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相关论文: Self-screening corrections beyond the random-phase…

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We use an all-electron implementation of the GW approximation to analyze several possible sources of error in the theory and its implementation. Among these are convergence in the polarization and Green's functions, the dependence of QP…

材料科学 · 物理学 2013-05-29 M. van Schilfgaarde , T. Kotani , S. Faleev

The self-screening error in electronic structure theory is the part of the self-interaction error that would remain within the $GW$ approximation if the exact dynamically screened Coulomb interaction, $W$, were used, causing each electron…

材料科学 · 物理学 2021-01-15 Jack Wetherell , Matthew Hodgson , Rex Godby

The $GW$ approximation is based on the neglect of vertex corrections, which appear in the exact self-energy and the exact polarizability. Here, we investigate the importance of vertex corrections in the polarizability only. We calculate the…

材料科学 · 物理学 2019-04-16 Alan M. Lewis , Timothy C. Berkelbach

We have implemented the so called GW approximation (GWA) based on an all-electron full-potential Projector Augmented Wave (PAW) method. For the screening of the Coulomb interaction W we tested three different plasmon-pole dielectric…

材料科学 · 物理学 2007-05-23 B. Arnaud , M. Alouani

This paper investigates the influence of the basis set on the GW self-energy correction in the full-potential linearized augmented-plane-wave (LAPW) approach and similar linearized all-electron methods. A systematic improvement is achieved…

材料科学 · 物理学 2007-05-23 Christoph Friedrich , Arno Schindlmayr , Stefan Blügel , Takao Kotani

We used our previously implemented GW approximation (GWA) based on the all-electron full-potential projector augmented wave (PAW) method to study the optical properties of small, medium and large-band-gap semiconductors: Si, GaAs, AlAs,…

材料科学 · 物理学 2016-08-31 B. Arnaud , M. Alouani

The self-consistent GW band gaps are known to be significantly overestimated. We show that this overestimation is, to a large extent, due to the neglect of the contribution of the lattice polarization to the screening of the…

材料科学 · 物理学 2015-06-15 Silvana Botti , Miguel A. L. Marques

The random phase approximation (RPA) is exact for the exchange energy of a many-electron ground state, but RPA makes the correlation energy too negative by about 0.5 eV/electron. That large short-range error, which tends to cancel out of…

计算物理 · 物理学 2020-06-24 Tim Gould , Adrienn Ruzsinszky , John P. Perdew

The equivalence of the covariant renormalization and the partial-wave renormaliz ation (PWR) approach is proven explicitly for the one-loop self-energy correction (SE) of a bound electron state in the presence of external perturbation…

高能物理 - 唯象学 · 物理学 2009-10-31 I. Goidenko , G. Plunien , S. Zschocke , L. Labzowsky , G. Soff

The \emph{GW} approximation takes into account electrostatic self-interaction contained in the Hartree potential through the exchange potential. However, it has been known for a long time that the approximation contains self-screening error…

强关联电子 · 物理学 2015-06-03 F. Aryasetiawan , R. Sakuma , K. Karlsson

The random phase approximation (RPA) to the correlation energy is extended to fractional occupations and its performance examined for exact conditions on fractional charges and fractional spins. RPA satisfies the constancy condition for…

其他凝聚态物理 · 物理学 2009-03-26 Paula Mori-Sánchez , Aron J. Cohen , Weitao Yang

The GW approximation is a well-known method to improve electronic structure predictions calculated within density functional theory. In this work, we have implemented a computationally efficient GW approach that calculates central…

Systematic errors are inevitable in most measurements performed in real life because of imperfect measurement devices. Reducing systematic errors is crucial to ensuring the accuracy and reliability of measurement results. To this end,…

量子物理 · 物理学 2017-06-29 Zhibo Hou , Huangjun Zhu , Guo-Yong Xiang , Chuan-Feng Li , Guang-Can Guo

We present an approach to calculate the electronic structure for a range of materials using the quasiparticle self-consistent GW method with vertex corrections included in the screened Coulomb interaction W. This is achieved by solving the…

材料科学 · 物理学 2023-10-10 Brian Cunningham , Myrta Gruening , Dimitar Pashov , Mark van Schilfgaarde

We investigate static correlation and delocalization errors in the self-consistent GW and random-phase approximation (RPA) by studying molecular dissociation of the H_2 and LiH molecules. Although both approximations contain topologically…

We study the convergence properties of the two-dimensional Rigorous Coupled Wave Approach (RCWA) for p-polarized monochromatic incident light. The RCWA is a semi-analytical numerical method that is widely used to solve the boundary-value…

数值分析 · 数学 2020-01-28 Benjamin J. Civiletti , Akhlesh Lakhtakia , Peter B. Monk

The band gaps of a few selected semiconductors/insulators are obtained from the self-consistent solution of the Hedin's equations. Two different schemes to include the vertex corrections are studied: (i) the vertex function of the…

强关联电子 · 物理学 2017-05-17 Andrey L. Kutepov

A new implementation of the GW approximation (GWA) based on the all-electron Projector-Augmented-Wave method (PAW) is presented, where the screened Coulomb interaction is computed within the Random Phase Approximation (RPA) instead of the…

材料科学 · 物理学 2009-11-10 S. Lebègue , B. Arnaud , M. Alouani , P. E. Bloechl

We report an all-electron, atomic orbital (AO) based, two-component (2C) implementation of the $GW$ approximation (GWA) for closed-shell molecules. Our algorithm is based on the space-time formulation of the GWA and uses analytical…

化学物理 · 物理学 2023-09-11 Arno Förster , Erik van Lenthe , Edoardo Spadetto , Lucas Visscher

Using seven semiconductors/insulators with band gaps covering the range from 1 eV to 10 eV we systematically explore the performance of two different variants of self-consistency associated with famous Hedin's system of equations: the full…

材料科学 · 物理学 2022-01-20 Andrey L. Kutepov
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