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The quasi-two-dimensional organic charge-transfer salt $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ is one of the prime candidates for a quantum spin-liquid due the strong spin frustration of its anisotropic triangular lattice in combination with…

Utilizing infrared vibrational spectroscopy we have investigated dimerized two-dimensional organic salts in order to search for possible charge redistribution that might cause electronic dipoles and ferroelectricity: the quantum spin liquid…

Recent discovery of superconductivity at a transition temperature of $73$K in the doped layered compound Ba$_{2}$CuO$_{3+x}$ for $x\sim 0.2$ has generated a lot of interest. Experiments in this alternately stacked oxygen octahedral and…

Quantum spin liquids (QSL) are novel phases of matter which remain quantum disordered even at the lowest temperature. They are characterized by emergent gauge fields and fractionalized quasiparticles. Here we show that the sub-Kelvin…

We describe a new possible route to the metal-insulator transition in doped semiconductors such as Si:P or Si:B. We explore the possibility that the loss of metallic transport occurs through Mott localization of electrons into a quantum…

强关联电子 · 物理学 2012-10-15 Andrew C. Potter , Maissam Barkeshli , John McGreevy , T. Senthil

The quantum spin liquid (QSL) state has been searched intensively in Kitaev-like materials, such as the Iridium oxides $A_2$IrO$_3$ and $\alpha$-RuCl$_3$. The half-filled Kitaev-Hubbard model with bond dependent hopping terms is used to…

强关联电子 · 物理学 2022-10-06 Shaojun Dong , Hao Zhang , Chao Wang , Meng Zhang , Yong-Jian Han , Lixin He

Mechanism of superconductivity (SC) in a purely interacting electron system has been one of the most challenging issues in condensed matter physics. In the BCS theory, the Landau's Fermi liquid is a normal state against which an SC…

强关联电子 · 物理学 2020-09-30 Hong-Chen Jiang , Shuai Chen , Zheng-Yu Weng

High-temperature superconductivity in cuprates emerges upon doping the parent Mott insulator. Robust signatures of the low-doped electronic state include a Hall carrier density that initially tracks the number of doped holes and the…

EtMe$_3$Sb[Pd(dmit)$_2$]$_2$, an organic Mott insulator with nearly isotropic triangular lattice, is a candidate material for a quantum spin liquid, in which the zero-point fluctuations do not allow the spins to order. The itinerant gapless…

强关联电子 · 物理学 2020-04-29 M. Yamashita , Y. Sato , T. Tominaga , Y. Kasahara , S. Kasahara , H. Cui , R. Kato , T. Shibauchi , Y. Matsuda

The Mott-insulator \kappa-(BEDT-TTF)_2Cu_2(CN)_3 is the prime candidate of a quantum spin liquid with puzzling magnetic properties. Our THz and infrared investigations reveal that also the charge dynamics does not follow the expectations…

强关联电子 · 物理学 2012-11-06 Sebastian Elsasser , Dan Wu , Martin Dressel , John A. Schlueter

We study the doping of a Mott insulator in the presence of quenched frustrating disorder in the magnetic exchange. A low doping regime $\delta<J/t$ is found, in which the quasiparticle coherent scale is low : $\epsilon_F^* = J…

强关联电子 · 物理学 2016-08-31 Olivier Parcollet , Antoine Georges

LK-99, with chemical formula Pb$_{10-x}$Cu$_x$(PO4)$_6$O, was recently reported to be a room-temperature superconductor. While this claim has met with little support in a flurry of ensuing work, a variety of calculations (mostly based on…

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…

Doping a Mott-insulating $\mathbb{Z}_2$ spin liquid can lead to a fractionalized Fermi liquid (FL*). Such a phase has several favorable features that make it a candidate for the pseudogap metal for the underdoped cuprates. We focus on a…

强关联电子 · 物理学 2016-11-15 Shubhayu Chatterjee , Subir Sachdev

Currently under active study in condensed matter physics, both theoretically and experimentally, are quantum spin liquid (QSL) states, in which no long-range magnetic ordering appears at low temperatures due to strong quantum fluctuations…

强关联电子 · 物理学 2019-07-04 Ruidan Zhong , Shu Guo , Guangyong Xu , Zhijun Xu , Robert J. Cava

Mott insulators with a half-filled band of electrons on the triangular lattice have been recently studied in a variety of organic compounds. All of these compounds undergo transitions to metallic/superconducting states under moderate…

强关联电子 · 物理学 2008-05-09 Yang Qi , Subir Sachdev

The molecular triangular lattice system, beta'-EtMe3Sb[Pd(dmit)2]2, is considered as a candidate material for the quantum spin liquid (QSL) state, although ongoing debates arise from recent controversial results. Here, the results of…

An unconventional superconducting phase is explored developing out of a non Fermi-liquid phase of the two-channel Anderson lattice model. It is characterized by a composite order parameter comprising of a local spin or orbital degree of…

强关联电子 · 物理学 2009-11-07 Frithjof B. Anders

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

强关联电子 · 物理学 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

We report the pressure study of a doped organic superconductor with Hall coefficient and conductivity measurements. We find that maximally enhanced superconductivity and a non-Fermi liquid appear around a certain pressure where mobile…

材料科学 · 物理学 2025-01-07 H. Oike , K. Miyagawa , H. Taniguchi , K. Kanoda