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In compound semiconductors and insulators, the polar electron-phonon coupling diverges at long range, known as the Fr\"ohlich interaction. Modern first-principles electron-phonon calculations treat the Fr\"ohlich interaction in a…

Starting from recent advances in the first-principles modeling of polarons, variational polaron equations in the strong-coupling adiabatic approximation are formulated in Bloch space. In this framework, polaron formation energy as well as…

材料科学 · 物理学 2022-06-09 Vasilii Vasilchenko , Andriy Zhugayevych , Xavier Gonze

The electron-phonon interaction causes thermal and zero-point motion shifts of electron quasiparticle (QP) energies $\epsilon_k(T)$. Other consequences of interactions, visible in angle-resolved photoemission spectroscopy (ARPES)…

材料科学 · 物理学 2018-03-28 Jean Paul Nery , Philip B. Allen , Gabriel Antonius , Lucia Reining , Anna Miglio , Xavier Gonze

We present the multi-channel Dyson equation that combines two or more many-body Green's functions to describe the electronic structure of materials. In this work we use it to model photoemission spectra by coupling the one-body Green's…

强关联电子 · 物理学 2023-10-03 Gabriele Riva , Pina Romaniello , J. Arjan Berger

We present a theoretical framework to describe polarons from first principles within a many-body Green's function formalism. Starting from a general electron-phonon Hamiltonian, we derive a self-consistent Dyson equation in which the…

The electronic structure of condensed matter can be significantly affected by the electron-phonon interaction, leading to important phenomena such as electrical resistance, superconductivity or the formation of polarons. This interaction is…

We perform a first-principles investigation of electron-phonon interactions in silicon and germanium, uncovering distinct non-polaronic spectral and transport fingerprints in these archetypal covalent semiconductors. Using many-body…

材料科学 · 物理学 2025-09-15 Raveena Gupta , Joao Abreu , Matthieu J. Verstraete

We present a method for solving impurity models with electron-phonon coupling, which treats the phonons efficiently and without approximations. The algorithm is applied to the Holstein-Hubbard model in the dynamical mean field…

强关联电子 · 物理学 2009-11-13 Philipp Werner , Andrew J. Millis

In model Hamiltonians, like Fr\"ohlich's, the electron-phonon interaction is assumed to be screened from the beginning. The same occurs when this interaction is obtained by using the state-of-the-art density functional perturbation theory…

材料科学 · 物理学 2022-12-14 Andrea Marini

We include the treatment of quadrupolar fields beyond the Fr\"ohlich interaction in the first-principles electron-phonon vertex in semiconductors. Such quadrupolar fields induce long-range interactions that have to be taken into account for…

Several photoemission spectroscopies and, in particular, Auger spectroscopy, involve double-ionization processes. For the numerical simulation of these spectroscopies it is convenient to use the particle-particle channel of the two-body…

强关联电子 · 物理学 2026-04-02 Pierre Sellié , J. Arjan Berger , Pina Romaniello

Polarons, that is, charge carriers correlated with lattice deformations, are ubiquitous quasiparticles in semiconductors, and play an important role in electrical conductivity. To date most theoretical studies of so-called large polarons,…

The Fr\"ohlich model describes the interaction of a mobile impurity with a surrounding bath of phonons which leads to the formation of a quasiparticle, the polaron. In this article an efficient renormalization group approach is presented…

量子气体 · 物理学 2016-04-27 Fabian Grusdt

A detailed study of the Frohlich polaron model is performed on the basis of diagrammatic quantum Monte Carlo method. The method is further developed both quantitatively (performance) and qualitatively (new estimators), and is enhanced by…

统计力学 · 物理学 2007-05-23 A. S. Mishchenko , N. V. Prokof'ev , A. Sakamoto , B. V. Svistunov

We analyze the effect of electron-phonon coupling on photoemission properties and ultrafast response of doped monolayer MoS2. The analysis is based on combined DFT and many-body (Eliashberg theory) approaches. In particular, we have…

材料科学 · 物理学 2015-02-02 Neha Nayyar , Duy Le , Volodymyr Turkowski , Talat S. Rahman

Within unitary transformed Hamiltonian of Fr\"ohlich type, using the Green's functions method, exact renormalized energy spectrum of quasiparticle strongly interacting with two-mode polarization phonons is obtained at $T=0$ K in a model of…

软凝聚态物质 · 物理学 2023-03-09 M. V. Tkach , Ju. O. Seti , O. M. Voitsekhivska , V. V. Hutiv

We study ground-state properties of a two-site, two-electron Holstein model describing two molecules coupled indirectly via electron-phonon interaction by using both exact diagonalization and self-consistent diagrammatic many-body…

强关联电子 · 物理学 2016-01-20 N. Säkkinen , Y. Peng , H. Appel , R. van Leeuwen

Many-polaron systems with finite charge-carrier density are often encountered experimentally. However, until recently, no satisfactory theoretical description of these systems was available even in the framework of simple models such as the…

强关联电子 · 物理学 2009-11-11 Martin Hohenadler , Georg Hager , Gerhard Wellein , Holger Fehske

The Frohlich interaction is one of the main electron-phonon intrinsic interactions in polar materials originating from the coupling of one itinerant electron with the macroscopic electric field generated by any longitudinal optical (LO)…

介观与纳米尺度物理 · 物理学 2009-11-11 C. Faugeras , G. Martinez , A. Riedel , R. Hey , K-J Friedland , Y. Bychkov

We describe an approach for calculations of phonon contributions to the electron spectral function, including both quasiparticle properties and satellites. The method is based on a cumulant expansion for the retarded one-electron Green's…

材料科学 · 物理学 2015-06-22 S. M. Story , J. J. Kas , F. D. Vila , M. J. Verstraete , J. J. Rehr
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