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Here we perform a series of time-resolved experiments where a 100 fs pump pulse is tuned between 528 nm and 555 nm, across the second indirect gap of intrinsic silicon at ~540 nm which involves electrons in a higher-lying conduction band…

光学 · 物理学 2017-01-24 Fabio Novelli , Jeffrey A Davis

Liquid crystal based technologies have found considerably diversified uses and areas of application over the last few decades, proving to be excellent materials for tunable optical elements from visible to near-infrared frequencies.…

化学物理 · 物理学 2023-10-25 Patrick Friebel , Daria Ruth Galimberti , Matteo Savoini , Laura Cattaneo

Advances in light sources and time resolved spectroscopy have made it possible to excite specific atomic vibrations in solids and to observe the resulting changes in electronic properties but the mechanism by which phonon excitation causes…

超导电性 · 物理学 2017-05-05 Dante M. Kennes , Eli Y. Wilner , David R. Reichman , Andrew J. Millis

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental…

Twisted bilayer graphene (tBLG) has recently emerged as a platform for hosting correlated phenomena, owing to the exceptionally flat band dispersion that results near interlayer twist angle $\theta\approx1.1^\circ$. At low temperature a…

强关联电子 · 物理学 2019-10-03 H. Polshyn , M. Yankowitz , S. Chen , Y. Zhang , K. Watanabe , T. Taniguchi , C. R. Dean , A. F. Young

We analyze the modification of the intersubband absorption of electrons in quantum wells under intense THz irradiation. An expression for the induced current is obtained, based on the adiabatic approach and the resonant approximation. We…

材料科学 · 物理学 2007-05-23 A. Hernanez-Cabrera , P. Aceituno , F. T. Vasko

The quantum dynamics of a system of Rb atoms, modeled by a V-type three-level system interacting with intense probe and pump pulses, are studied. The time-delay-dependent transient-absorption spectrum of an intense probe pulse is thus…

原子物理 · 物理学 2018-02-14 Vadim Becquet , Stefano M. Cavaletto

The temporal evolution of electromagnetically induced transparency (EIT) and absorption (EIA) coherence resonances in pump-probe spectroscopy of degenerate two-level atomic transition is studied for light intensities below saturation.…

量子物理 · 物理学 2009-11-07 P. Valente , H. Failache , A. Lezama

The advent of pump-probe spectroscopy techniques paved the way to the exploration of the ultrafast dynamics of electrons and phonons in crystalline solids. Following photo-absorption of a pump pulse and the initial electronic…

材料科学 · 物理学 2023-07-14 Fabio Caruso , Dino Novko

We investigated the pressure-dependent optical response of the low-dimensional Mott-Hubbard insulator TiOBr by transmittance and reflectance measurements in the infrared and visible frequency range. A suppression of the transmittance above…

The transient response of an intrinsic graphene, which is caused by the ultrafast interband transitions, is studied theoretically for the range of pumping correspondent to the saturated absorption regime. Spectral and temporal dependencies…

介观与纳米尺度物理 · 物理学 2015-05-20 F. T. Vasko

The large surface-to-volume ratio in atomically thin 2D materials allows to efficiently tune their properties through modifications of their environment. Artificial stacking of two monolayers into a bilayer leads to an overlap of…

介观与纳米尺度物理 · 物理学 2020-05-14 Samuel Brem , Kai-Qiang Lin , Roland Gillen , Jonas M. Bauer , Janina Maultzsch , John M. Lupton , Ermin Malic

Ultrafast carrier and phonon dynamics at the buried heterointerface of GaP/Si(001) are investigated by means of two-color pump-probe reflectivity measurements. The carrier-induced reflectivity signal exhibits a resonant enhancement at…

材料科学 · 物理学 2025-04-15 Gerson Mette , Kunie Ishioka , Steven Youngkin , Wolfgang Stolz , Kerstin Volz , Ulrich Höfer

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

High pressure is a proven effective tool for modulating inter-layer interactions in semiconducting transition metal dichalcogenides, which leads to significant band structure changes. Here, we present an extended infrared study of the…

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

材料科学 · 物理学 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

Femtosecond spectroscopy is applied to study transient electronic and lattice processes in bismuth. Components with relaxation times of 1 ps, 7 ps and ~ 1 ns are detected in the photoinduced reflectivity response of the crystal. To…

材料科学 · 物理学 2015-06-05 Alexey A. Melnikov , Oleg V. Misochko , Sergey V. Chekalin

We study the all-optical switching behavior of one-dimensional metal-dielectric photonic crystals due to the nonlinearity of the free metal electrons. A polychromatic pump-probe setup is used to determine the wavelength and pump intensity…

其他凝聚态物理 · 物理学 2015-05-13 Tolga Ergin , Tilman Höner zu Siederdissen , Harald Giessen , Markus Lippitz

The infrared reflectance of the transition metal chalcogenide 1T-TaS2 has been measured at temperatures from 30K to 360K over 30-45,000cm^-1 (4meV-5.5eV). The optical conductivity was obtained by Kramers-Kronig analysis. At 360K only modest…

凝聚态物理 · 物理学 2013-10-31 L. V. Gasparov , K. G. Brown , A. C. Wint , D. B. Tanner , H. Berger , R. Gaal , L. Forro , G. Margaritondo

Energy- and time-resolved spectroscopy reveals a photoinduced softening of the charge-transfer gap in the insulating copper oxide Sr2CuO2Cl2 that indicates rapid and efficient photoproduction of optical phonons. By relating the pump-probe…

强关联电子 · 物理学 2009-10-28 J. S. Dodge , A. B. Schumacher , L. L. Miller , D. S. Chemla