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We study the nature of photo-excited charge carriers in CsPbBr3 nanocrystal thin films by ultrafast optical pump - THz probe spectroscopy. We observe a deviation from a pure Drude dispersion of the THz dielectric response that is ascribed…

Using resonant 2-photon excitation of interlayer electrons in twisted bilayer graphene (tBLG), we resolve photoluminescence (PL) that tunes spectrally with stacking angle, {\theta}. This weak signal is 4- 5$\times$ larger than the…

介观与纳米尺度物理 · 物理学 2019-04-01 Hiral Patel , Lujie Huang , Cheol-Joo Kim , Jiwoong Park , Matt W. Graham

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…

Optical driving of materials has emerged as a versatile tool to control their properties, with photo-induced superconductivity being among the most fascinating examples. In this work, we show that light or lattice vibrations coupled to an…

We observe pronounced oscillations in the differential reflectivity of a ferromagnetic InMnAs/GaSb heterostructure using two-color pump-probe spectroscopy. Although originally thought to be associated with the ferromagnetism, our studies…

介观与纳米尺度物理 · 物理学 2015-06-25 J. Wang , Y. Hashimoto , J. Kono , A. Oiwa , H. Munekata , G. D. Sanders , C. J. Stanton

Enabling the light-control of complex systems on ultra-short timescales gives rise to rich physics with promising applications. While crucial, the quantitative determination of both the longitudinal and shear photo-induced strains still…

Hydrostatic pressure has been commonly applied to tune broadband light emissions from self-trapped excitons (STE) in perovskites for producing white light and study of basic electron-phonon interactions. However, a general theory is still…

We report on observation of the infrared photoresistance of twisted bilayer graphene under continuous quantum cascade laser illumination at a frequency of 57.1 THz. The photoresistance shows an intricate sign-alternating behavior under…

介观与纳米尺度物理 · 物理学 2022-08-04 S. Hubmann , G. Di Battista , I. A. Dmitriev , K. Watanabe , T. Taniguchi , D. K. Efetov , S. D. Ganichev

Simultaneous measurements of transient transmission and reflectivity were performed in the unintentionally doped InN film to reveal ultrafast optical bleaching and its recovery behavior under intense laser irradiation. The optical bleaching…

光学 · 物理学 2021-02-16 Junjun Jia , Takashi Yagi , Toshiki Makimoto

Recent theoretical studies showed that the electronic structure of 1$T$-TaS$_2$ in the low-temperature commensurate charge density wave phase exhibits a nontrivial interplay between band-insulating and Mott insulating behavior. This has…

强关联电子 · 物理学 2023-04-19 Francesco Petocchi , Jiyu Chen , Jiajun Li , Martin Eckstein , Philipp Werner

The characteristics of topological insulators are manifested in both their surface and bulk properties, but the latter remain to be explored. Here we report bulk signatures of pressure-induced band inversion and topological phase…

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

We developed a mid-infrared optical frequency comb-based Fourier-transform spectrometer and performed a line-shape study of the fundamental vibrational band of CO perturbed by N${_2}$, which is crucial for atmospheric science and…

In stark contrast to the conventional charge density wave (CDW) materials, the one-dimensional CDW on the In/Si(111) surface exhibits immediate damping of the CDW oscillation during the photoinduced phase transition. Here, by successfully…

材料科学 · 物理学 2023-04-11 Yu-Xiang Gu§ , Wen-Hao Liu§ , Zhi Wang , Shu-Shen Li , Lin-Wang Wang , Jun-Wei Luo

Utilizing femtosecond optical pump-probe technique, we have studied transient Fano-resonance in zinc. At high excitation levels the Fourier spectrum of the coherent E$_{2g}$ phonon exhibits strongly asymmetric line shape, which is well…

强关联电子 · 物理学 2007-05-23 Muneaki Hase , Jure Demsar , Masahiro Kitajima

Here we report an ultrafast optical spectroscopic study of the nodal-line semimetal ZrSiTe. Our measurements reveal that, converse to other compounds of the family, the sudden injection of electronic excitations results in a strongly…

We report on optical properties of reduced BaTiO3-d at different doping levels including insulating and metallic samples. In all the samples, including metallic one, we observe structural phase transitions from the changes in the…

强关联电子 · 物理学 2015-05-28 J. Hwang , T. Kolodiazhnyi , J. Yang , M. Couillard

Charge density wave (CDW) materials can undergo an ultrafast phase transition after an ultrashort laser pulse excitation, and the suggested underlying mechanisms have always been associated with two main features: excitonic…

材料科学 · 物理学 2021-12-24 Zhao-Jun Suo , Wen-Hao Liu , Zhi Wang , Hao-Wen Liu , Jun-Wei Luo , Shu-Shen Li , Lin-Wang Wang

The spectral functions of twisted bilayer graphene (TBG) in the absence of strain have recently been investigated in both the symmetric and symmetry-broken phases using dynamical mean-field theory (DMFT). The theoretically predicted…

We measure the photoionization cross-section of vibrationally excited levels in the S2 state of azulene by femtosecond pump-probe spectroscopy. At the wavelengths studied (349-265 nm in the pump) the transient signals exhibit two distinct…

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