相关论文: Determining Reaction Pathways at Low Temperatures …
A novel type of particle "cooling", called Ionization Cooling, is applicable to slow (v of the order of 0.1c) ions stored in a small ring. The many traversals through a thin foil enhance the nuclear reaction probability, in a steady…
Ion-atom interactions are a comparatively recent field of research that has drawn considerable attention due to its applications in areas including quantum chemistry and quantum simulations. In first experiments, atomic ions and neutral…
We report on a study of cold reactive collisions between sympathetically-cooled molecular ions and laser-cooled atoms in an ion-atom hybrid trap. Chemical reactions were studied at average collision energies <Ecoll>/k > 20 mK, about two…
We present a fully quantum mechanical description of a free $^6$Li atom scattering from a trapped $^{171}$Yb$^+$ ion in one dimension. By reformulating the system in polar coordinates and employing the adiabatic representation, we extract a…
Gas-solid reactions are cornerstones of many catalytic and redox processes that will underpin the energy and sustainability transition. The specific case of hydrogen-based iron oxide reduction is the foundation to render the global steel…
The trapped-ion quantum charge-coupled device (QCCD) architecture is a leading candidate for advanced quantum information processing. In current QCCD implementations, imperfect ion transport and anomalous heating can excite ion motion…
The direct photodissociation of trapped $^{85}$Rb$_2^+$ (rubidium) molecular ions by the cooling light for the $^{85}$Rb magneto-optical trap (MOT) is studied, both experimentally and theoretically. Vibrationally excited Rb$_{2}^{+}$ ions…
Tiny radiative losses below the 0.1% level can prove ruinous to the effective laser cooling of a molecule. In this paper the laser cooling of a hydride is studied with rovibronic detail using ab initio quantum chemistry in order to document…
In this theoretical work, we calculate potential energy curves, spectroscopic pa- rameters and transition dipole moments of molecular ions BeX^+ (X=Na, K, Rb) composed of alkaline ion Be and alkali atom X with a quantum chemistry approach…
Using the ab initio computed Potential Energy Surface (PES) for the electronic interaction of the MgH$^+$ ($^1\Sigma$) ion with the He($^1$S) atom, we calculate the relevant state-changing rotationally inelastic collision cross sections…
We describe a simple approach to the problem of incorporating the response time of an atom or ion being Doppler-cooled into the theory of the cooling process. The system being cooled does not in general respond instantly to the changing…
The two most widely used ion cooling methods are laser cooling and sympathetic cooling by elastic collisions (ECs). Here we demonstrate another method of cooling ions that is based on resonant charge exchange (RCE) between the trapped ion…
We have demonstrated transport of Be+ ions through a 2D Paul-trap array that incorporates an X-junction, while maintaining the ions near the motional ground-state of the confining potential well. We expand on the first report of the…
Low-energy light ion beams are an essential resource in lithography for nanopatterning magnetic materials and interfaces due to their ability to modify the structure and properties of metamaterials. Here we create…
Quantum tunneling reactions play a significant role in chemistry when classical pathways are energetically forbidden, be it in gas phase reactions, surface diffusion, or liquid phase chemistry. In general, such tunneling reactions are…
Gaseous H2O has been detected in several cold astrophysical environments, where the observed abundances cannot be explained by thermal desorption of H2O ice or by H2O gas phase formation. These observations hence suggest an efficient…
In the endeavour of developing quantum memories, Er$^{3+}$:CaWO$_4$ has emerged as a promising rare-earth ion-doped (REID) crystal platform due to its long optical coherence times and compatibility with the 1550 nm telecommunications band.…
We demonstrate precision laser spectroscopy of a trapped $^{173}$Yb$^+$ ion that is not directly laser cooled by coupling it to ultracold atoms. The atomic bath continuously cools the internal degrees of freedom of the ion to its hyperfine…
We describe a hybrid vacuum system in which a single ion or a well defined small number of trapped ions (in our case Ba$^+$ or Rb$^+$) can be immersed into a cloud of ultracold neutral atoms (in our case Rb). This apparatus allows for the…
We are developing a new hybrid atom-ion trap to study the interaction of ultracold rubidium atoms with mass-selected OH- molecules. The ions are trapped inside an octupole rf-trap made of thin wires instead of the commonly used rods. This…