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We combine ab-initio calculations based on many-body perturbation theory and the cumulant expansion with angle-resolved photoemission spectroscopy (ARPES) to quantify the electron-plasmon interaction in the highly-doped semiconducting…

强关联电子 · 物理学 2023-07-12 Christoph Emeis , Sanjoy Kr Mahatha , Sebastian Rohlf , Kai Rossnagel , Fabio Caruso

Electron-boson coupling is central to a comprehensive understanding of the diverse physical phenomena emerging from many-body interactions. Yet less attention has been paid to how plasmons, collective bosonic modes of electron density…

Harnessing electronic excitations involving coherent coupling to bosonic modes is essential for the design and control of emergent phenomena in quantum materials [1]. In situations where charge carriers induce a lattice distortion due to…

Two dimensional materials offer a path forward for smaller and more efficient devices. Their optical and electronic properties give way to beat the limits set in place by Moore's Law. Plasmon are the collective oscillations of electrons and…

介观与纳米尺度物理 · 物理学 2020-12-21 Eoin Moynihan , Stefan Rost , Eoghan O'Connell , Quentin Ramasse , Christoph Friedrich , Ursel Bangert

We develop a first-principles approach based on many-body perturbation theory to investigate the effects of the interaction between electrons and carrier plasmons on the electronic properties of highly-doped semiconductors and oxides.…

材料科学 · 物理学 2018-04-12 Fabio Caruso , Carla Verdi , Samuel Poncé , Feliciano Giustino

Plasmons in two-dimensional electron systems (2DES) feature ultra-strong confinement and are expected to efficiently mediate the interactions between light and charge carriers. Despite these expectations, the electromagnetic detectors…

介观与纳米尺度物理 · 物理学 2022-07-01 Dmitry Mylnikov , Dmitry Svintsov

Two-dimensional (2D) compounds provide unique building blocks for novel layered devices and hybrid photonic structures. However, large surface-to-volume ratio in thin films enhances the significance of surface interactions and charging…

Collective modes of doped two-dimensional crystalline materials, namely graphene, MoS$_2$ and phosphorene, both monolayer and bilayer structures, are explored using the density functional theory simulations together with the random phase…

介观与纳米尺度物理 · 物理学 2018-02-06 Zahra Torbatian , Reza Asgari

Transition metal dichalcogenide, especially MoS2 has attracted lot of attention recently owing to its tunable visible range band gap and anisotropic electronic and transport properties. Here, we report a comprehensive inelastic light…

材料科学 · 物理学 2020-08-26 Deepu Kumar , Birender Singh , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

Optical metasurfaces have great potential to form the platform for manipulation of surface waves. A plethora of advanced surface-wave phenomena utilizing negative refraction, self-collimation and channeling of 2D waves can be realized…

Based on first-principles calculations, we systematically study the electronic, dielectric, and plasmonic properties of two-dimensional (2D) electride materials X$_2$N (X=Ca, Sr). We show that both Ca$_2$N and Sr$_2$N are stable down to…

材料科学 · 物理学 2015-09-22 Shan Guan , Shengyuan A. Yang , Liyan Zhu , Junping Hu , Yu-Gui Yao

Two-dimensional (2D) metals can host gapless plasmonic excitations, which strongly couple to electrons and thus may significantly affect superconductivity in layered materials. To investigate the dynamical interplay of the electron-electron…

超导电性 · 物理学 2024-08-21 Yann in 't Veld , Mikhail I. Katsnelson , Andrew J. Millis , Malte Rösner

We reveal new aspects of the interaction between plasmons and phonons in 2D materials that go beyond a mere shift and increase in plasmon width due to coupling to either intrinsic vibrational modes of the material or phonons in a supporting…

We investigate the spectroscopic fingerprints of electron-plasmon coupling in integrated (PES) and angle-resolved photoemission spectroscopy (ARPES). To account for electron-plasmon interactions at a reduced computational cost, we derived…

强关联电子 · 物理学 2015-07-27 Fabio Caruso , Feliciano Giustino

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

We theoretically investigate the electric field-tuning plasmons and plasmon-phonon couplings of two-dimensional (2D) transition metal dichalcogenides (TMDs), such as monolayer MoS2, under the consideration of spin-orbit coupling. It is…

材料科学 · 物理学 2025-03-25 Chengxiang Zhao , Wenjun Zhang , Haotong Wang , Fangwei Han , and Haiming Dong

In reduced-dimensional semiconductors, doping-induced carrier plasmons can strongly couple with quasiparticle excitations, leading to a significant band gap renormalization. We develop a new plasmon-pole theory that efficiently and…

介观与纳米尺度物理 · 物理学 2015-02-11 Yufeng Liang , Li Yang

We analyze the effect of electron-phonon coupling on photoemission properties and ultrafast response of doped monolayer MoS2. The analysis is based on combined DFT and many-body (Eliashberg theory) approaches. In particular, we have…

材料科学 · 物理学 2015-02-02 Neha Nayyar , Duy Le , Volodymyr Turkowski , Talat S. Rahman

Interaction between electrons and phonons in solids is a key effect defining physical properties of materials such as electrical and thermal conductivity. In transitional metal dichalcogenides (TMDCs) the electron-phonon coupling results in…

We present a theoretical description of the coupling between longitudinal optical phonons and collective excitations of a two-dimensional electron gas. By diagonalizing the Hamiltonian of the system, including Coulomb electron-electron and…

介观与纳米尺度物理 · 物理学 2020-02-21 Sofia Ribeiro , Angela Vasanelli , Yanko Todorov , Carlo Sirtori
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