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Hole doping in Nd${}_{2}$NiO${}_{4.00}$ can be either achieved by substituting the trivalent Nd atoms by bivalent alkaline earth metals or by oxygen doping, yielding Nd${}_{2}$NiO${}_{4+\delta}$. In this study, we investigated the interplay…

Anion exchange membranes are used in alkaline fuel cells and offer a promising alternative to the more expensive proton exchange membrane fuel cells. However, hydroxide ion conductivity in anion exchange membranes is low, and the quest for…

软凝聚态物质 · 物理学 2024-04-16 Mohammed Al Otmi , Ping Lin , William Schertzer , Coray M. Colina , Rampi Ramprasad , Janani Sampath

The recent discovery of superconductivity in La3Ni2O7-{\delta} under high pressure with a transition temperature around 80 K has sparked extensive experimental and theoretical efforts. Several key questions regarding the pairing mechanism…

超导电性 · 物理学 2024-07-26 Zehao Dong , Mengwu Huo , Jie Li , Jingyuan Li , Pengcheng Li , Hualei Sun , Yi Lu , Meng Wang , Yayu Wang , Zhen Chen

Understanding and predicting the dominant diffusion processes in Cr2O3 is essential to its optimization for anti-corrosion coatings, spintronics, and other applications. Despite significant theoretical effort in modeling defect mediated…

Recent discovery of giant electrostriction in rare earth (RE (III)) substituted ceria (CeO2) thin films driven by electroactive defect complexes and their coordinated elastic response, expands the material spectrum for electrostrain…

材料科学 · 物理学 2023-09-26 Soumyajyoti Mondal , Pooja Punetha , Rajeev Ranjan , Pavan Nukala

CeO$_2$ (ceria) is an attractive material for heterogeneous catalysis applications involving hydrogen due to its favorable redox activity combined with its relative impermeability to hydrogen ions and molecules. However, to date, many bulk…

材料科学 · 物理学 2024-11-12 Jared C. Stimac , Nir Goldman

Oxide heterostructures exhibit a vast variety of unique physical properties. Examples are unconventional superconductivity in layered nickelates and topological polar order in (PbTiO$_3$)$_n$/(SrTiO$_3$)$_n$ superlattices. Although it is…

A series of CaxCoO2 (0.15 <= x <= 0.40) materials have been prepared by means of ion exchange reaction from NaxCoO2. Transmission electron microscopy (TEM) measurements revealed a rich variety of structural phenomena resulting from cation…

强关联电子 · 物理学 2009-11-11 H. X. Yang , Y. G. Shi , X. Liu , R. J. Xiao , H. F. Tian , J. Q. Li

A two-dimensional small bias model has been developed for a patterned metal current collector $|$ mixed oxygen ion and electronic conductor (MIEC) $|$ patterned metal current collector electrochemical cell in a symmetric gas environment.…

化学物理 · 物理学 2009-03-20 Francesco Ciucci , William C. Chueh , Sossina M. Haile , David G. Goodwin

Disorder, primarily in the form of oxygen vacancies, cation stoichiometry and atomic inter-diffusion, appear to play vital roles in the electronic and transport properties of the metallic electron liquid at the oxide hetero-interfaces.…

强关联电子 · 物理学 2018-07-05 Urmimala Dey , Swastika Chatterjee , A. Taraphder

The structure property of non-ideal Si/GaAs heterostructures that were integrated with the ultra-thin oxide (UO) tunneling interfacial layer has been systematically investigated. Si nanomembranes (NMs) were oxidized in different time…

In recent years, the Na-ion SuperIonic CONductor (NASICON) based polyanionics are considered the pertinent cathode materials in sodium-ion batteries due to their 3D open framework, which can accommodate a wide range of Na content and can…

化学物理 · 物理学 2024-05-10 Simranjot K. Sapra , Jeng-Kuei Chang , Rajendra S. Dhaka

Sodium-titanate \ce{Na2Ti3O7} (NTO) is regarded as a highly promising anode material with a very low voltage for Na-ion batteries and capacitors, but suffered from relatively low specific capacity and poor electron conductivity. Here we…

材料科学 · 物理学 2020-06-19 Chol-Jun Yu , Suk-Gyong Hwang , Yong-Chol Pak , Song-Hyok Choe , Jin-Song Kim , Kum-Chol Ri

Carbon contamination is a significant concern for proton-conducting oxides in the cerate and zirconate family, particularly for BaCeO$_3$. Here, we use first-principles calculations to evaluate carbon stability in SrCeO$_3$, BaCeO$_3$,…

材料科学 · 物理学 2021-06-25 Andrew J. E. Rowberg , Michael W. Swift , Chris G. Van de Walle

Lead-free materials based on the $\text{(Ba,Ca)(Zr,Ti)O}_{3}$ (BCZT) system exhibit excellent electromechanical properties that can be strongly modified by small amounts of dopants. Here, we use a high throughput strategy to unravel the…

To design and discover new materials for next-generation energy materials such as solid-oxide fuel cells (SOFCs), a fundamental understanding of their ionic properties and behaviors is essential. The potential applicability of a material…

材料科学 · 物理学 2014-09-01 Chandrima Mitra , Tricia Meyer , Ho Nyung Lee , Fernando A. Reboredo

There is considerable interest in the pH-dependent switchable biocatalytic properties of cerium oxide nanoparticles (CeNPs) in biomedicine, where these materials exhibit beneficial antioxidant activity against reactive oxygen species at…

材料科学 · 物理学 2021-04-23 Hongyang Ma , Hangjuan Ren , Zhao Liu , Pramod Koshy , Charles C. Sorrell , Judy N. Hart

The effect of substituting iron and zinc for cobalt in CaBaCo$_4$O$_7$ has been investigated using neutron diffraction and x-ray absorption spectroscopy. The orthorhombic distortion present in the parent compound CaBaCo$_4$O$_7$ decreases…

材料科学 · 物理学 2020-09-01 V. Cuartero , J. Blasco , G. Subías , J. García , J. A. Rodríguez-Velamazán , C. Ritter

The presence of oxygen vacancy, as well as ordering of vacancies plays an important role in determining the electronic, ionic and thermal transport properties of many transition metal oxide materials. Controlling the concentration of oxygen…

介观与纳米尺度物理 · 物理学 2018-12-05 Xue Rui , Robert Klie

The electronic properties of single- and multi-cation transparent conducting oxides (TCOs) are investigated using first-principles density functional approach. A detailed comparison of the electronic band structure of stoichiometric and…

材料科学 · 物理学 2015-05-18 Julia E. Medvedeva , Chaminda L. Hettiarachchi