相关论文: High frequency limit of spectroscopy

The interaction of coherent nonlinear structures (such as sub-cycle solitons, electron vortices and wake Langmuir waves) with a strong wake wave in a collisionless plasma can be exploited in order to produce ultra-short electromagnetic…

We develop the theory of pure dephasing in a solid exposed to an ultrashort laser pulse beyond the commonly used Markov approximation. This approach takes into account the finite cutoff energy of the bath and can be applied to both…

The Heisenberg limit is the superior precision available by entanglement sensors. However, entanglementis fragile against dephasing, and there is no known quantum metrology protocol that can achieve Heisenberg limited sensitivity with the…

Molecular absorption and photo-electron spectra can be efficiently predicted with real-time time-dependent density-functional theory (TDDFT). We show here how these techniques can be easily extended to study time-resolved pump-probe…

Ultrashort light pulses are ubiquitous in modern research, but the electromagnetic field of the optical cycles is usually not easy to obtain as a function of time. Field-resolved pulse characterization requires either a nonlinear-optical…

The analysis of nonlinear spectroscopy, widely used to study the dynamics and structures of condensed-phase matter, typically employs a perturbative approach noticing the weak interaction between the laser and the matter of interest.…

We treat the case of a flat stress-free surface (i.e., the ground in seismological applications) separating air from a homogeneous, isotropic, solid substratum overlain by a homogeneous, isotropic, solid layer (in contact with the ground)…

A long range phase-sensitive optical time domain reflectometer (phi-OTDR) with a multi-frequency non-linear frequency modulation (NLFM) optical pulse is proposed in this Letter. To boost the pulse energy while suppressing the optical…

The success of non-linear optics relies largely on pulse-to-pulse consistency. In contrast, covariance based techniques used in photoionization electron spectroscopy and mass spectrometry have shown that wealth of information can be…

Simultaneous observations at four different frequencies viz. 313, 607, 1380 and 4850 MHz, for three pulsars, PSRs B0031-07, B0809+74 and B2319+60, are reported in this paper. Identified null and burst pulses are highly concurrent across…

Absorbing a focused, femtosecond X-ray pulse from a Free-Electron Laser (FEL) can lead to extreme electronic excitations in solids. This excitation drives changes of the electronic system over the course of the pulse duration and the…

The theory for time-resolved photoemission spectroscopy as applied to pump-probe experiments is developed and solved for the generic case of a strongly correlated material. The formal development incorporates all of the nonequilibrium…

Resistive Pulse Sensing (RPS) is a key label-free technology to measure particles and single-cell size distribution. As a growing corpus of evidence supports that cancer cells exhibit distinct mechanical phenotypes from healthy cells,…

Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…

In the framework of linear optics, light fields do not interact with each other in a medium. Yet, when their field amplitude becomes comparable to the electron binding energies of matter, the nonlinear motion of these electrons emits new…

The spectral response and physical features of the 2D Hubbard-Holstein model are calculated both in equilibrium at zero and low chemical dopings, and after an ultra short powerful light pulse, in undoped systems. At equilibrium and at…

We show that, in optical pump-probe experiments on bulk samples, the statistical distribution of the intensity of ultrashort light pulses after the interaction with a nonequilibrium complex material can be used to measure the time-dependent…

In this paper, single-molecule spectroscopy experiments based on continuous laser excitation are characterized through an open quantum system approach. The evolution of the fluorophore system follows from an effective Hamiltonian…

A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…

Spectral/hp element methods and an arbitrary Lagrangian-Eulerian (ALE) moving-boundary technique are used to investigate planar Newtonian extrudate swell. Newtonian extrudate swell arises when viscous liquids exit long die slits. The…