相关论文: High frequency limit of spectroscopy
Ultra-fast and multi-dimensional spectroscopy gives a powerful looking glass into the dynamics of molecular systems. In particular two-dimensional electronic spectroscopy (2DES) provides a probe of coherence and the flow of energy within…
We propose theoretically a method for the control of the frequency of the nonlinear optical response of a model nonlinear medium driven by an electric field and suggest an experimental realization on the basis of isotropic LiF, or NaCl…
Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…
We revisit the phenomenon of pulse nulling using high-quality single-pulse data of PSR B1133+16 from simultaneous multifrequency observations. Observations were made at 325, 610, 1400 and 4850 MHz as part of a joint program between the…
We study the non-linear response of a 2+1 dimensional holographic model with weak momentum relaxation and finite charge density to an oscillatory electric field pump pulse. Following the time evolution of one point functions after the…
Frequency conversion of non-classical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic…
The computation and analysis of photoelectron spectra (PES) is a fundamental technique in atomic and molecular physics to study the structural and dynamical properties of a target system, and to gain insight into the process of its…
In this paper we develop a method capable of modeling the space-time focusing of nondiffracting pulses. The new pulses can possess arbitrary peak velocities and, in addition to being resistant to diffraction, can have their peak intensities…
Spatiotemporal control of laser pulses at relativistic intensities is a longstanding goal with broad implications in laser-plasma acceleration, high-brightness radiation sources, and extreme-field science. Laser pulses with helical…
This paper proposes a high-precision time measurement method based on digital frequency-domain phase-fitting (DFPF) by using the digitized nuclear pulses. The averaging effect inherent in the frequency-domain cross-correlation and…
We present an effective linear response approach to pump-probe femtosecond coherence spectroscopy in the well separated pulse limit. The treatment presented here is based on a displaced and squeezed state representation for the…
The round trip time of the light pulse limits the maximum detectable frequency response range of vibration in phase-sensitive optical time domain reflectometry ({\phi}-OTDR). We propose a method to break the frequency response range…
We present a novel spectroscopy protocol based on optimal control of a single quantum system. It enables measurements with quantum-limited sensitivity (\eta_\omega ~ 1/sqrt(T_2^*),T_2^* denoting the system's coherence time) but has an…
Nonlinear phenomena are inherent in most systems in nature. Second or higher-order harmonic generations, three-wave and four-wave mixing are typical phenomena in nonlinear optics. To obtain a nonzero signal for second-harmonic generation in…
The fractional discrete nonlinear Schr\"odinger equation (fDNLS) is studied on a periodic lattice from the analytic and dynamic perspective by varying the mesh size $h>0$ and the nonlocal L\'evy index $\alpha \in (0,2]$. We show that the…
Nanoelectromechanical Systems (NEMS) have emerged as a promising technology for performing the mass spectrometry of large biomolecules and nanoparticles. As nanoscale objects land on NEMS sensor one by one, they induce resolvable shifts in…
Frequency sum rules are derived in extended quantum systems of non relativistic fermions from a minimal set of assumptions on dynamics in infinite volume, for ground and thermal states invariant under space translations or a lattice…
A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…
We introduce a numerically exact and computationally feasible nonlinear-response theory developed for lossy superconducting quantum circuits based on a framework of quantum dissipation in a minimally extended state space. Starting from the…
Coherent time is a characteristic time in the extreme nonlinear optics regime and thus generally introduced as the dephasing time in the simulations of the solid-state high-harmonic generation. This characteristic time linked with the…