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We study theoretically weak localization of excitons in atomically-thin transition metal dichalcogenides. The constructive interference of excitonic de Broglie waves on the trajectories forming closed loops results in a decrease of the…

介观与纳米尺度物理 · 物理学 2020-04-27 M. M. Glazov

Two-dimensional transition metal dichalcogenides exhibit strong optical transitions with significant potential for optoelectronic devices. In particular they are suited for cavity quantum electrodynamics in which strong coupling leads to…

Exciton-polariton modes arising from interaction between bound excitons in monolayer thin semiconductor sheets and photons in a Fabry-Perot microcavity are considered theoretically. We calculate the dispersion curves, mode lifetimes, Rabi…

介观与纳米尺度物理 · 物理学 2015-12-30 Mikhail I. Vasilevskiy , Darío G. Santiago-Pérez , Carlos Trallero-Giner , Nuno M. R. Peres , Alexey Kavokin

Condensed-matter emitters offer enriched cavity quantum electrodynamical effects due to the coupling to external degrees of freedom. In the case of carbon nanotubes a very peculiar coupling between localized excitons and the one-dimensional…

The properties of excitons, or correlated electron-hole pairs, are of paramount importance to optoelectronic applications of materials. A central component of exciton physics is the electron-hole interaction, which is commonly treated as…

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

材料科学 · 物理学 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge density wave order,…

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation…

材料科学 · 物理学 2015-11-05 G. Wang , I. C. Gerber , L. Bouet , D. Lagarde , A. Balocchi , M. Vidal , E. Palleau , T. Amand , X. Marie , B. Urbaszek

Excitons, trions, biexcitons, and exciton-trion complexes in two-dimensional transition metal dichalcogenide sheets of MoS$_2$, MoSe$_2$, MoTe$_2$, WS$_2$ and WSe$_2$ are studied by means of density functional theory and path integral Monte…

介观与纳米尺度物理 · 物理学 2015-11-23 Ilkka Kylänpää , Hannu-Pekka Komsa

Explaining the mechanism of superconductivity in the high-$T_c$ cuprates requires an understanding of what causes electrons to form Cooper pairs. Pairing can be mediated by phonons, the screened Coulomb force, spin or charge fluctuations,…

Bilayer van der Waals (vdW) heterostructures such as MoS2/WS2 and MoSe2/WSe2 have attracted much attention recently, particularly because of their type II band alignments and the formation of interlayer exciton as the lowest-energy…

介观与纳米尺度物理 · 物理学 2017-12-14 Shiyuan Gao , Li Yang , Catalin D. Spataru

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

The optical properties of the two-dimensional (2D) crystals are dominated by tightly bound electron-hole pairs (excitons) and lattice vibration modes (phonons). The exciton-phonon interaction is fundamentally important to understand the…

材料科学 · 物理学 2021-02-09 Qing-Hai Tan , Yu-Jia Sun , Xue-Lu Liu , Yanyuan Zhao , Qihua Xiong , Ping-Heng Tan , Jun Zhang

We investigate phase-dependent electronic and excitonic phenomena in monolayer Y2TeO2 MOenes in the 1T and 2H polymorphs using first-principles theory and an effective many-body framework. Phonon spectra and elastic stability criteria…

We report resonant Raman spectroscopy of neutral excitons X$^0$ and intravalley trions X$^-$ in hBN-encapsulated MoS$_2$ monolayer embedded in a nanobeam cavity. By temperature tuning the detuning between Raman modes of MoS$_2$ lattice…

介观与纳米尺度物理 · 物理学 2023-03-24 Chenjiang Qian , Viviana Villafañe , Marko M. Petrić , Pedro Soubelet , Andreas V. Stier , Jonathan J. Finley

The strength of the electron-phonon coupling parameter and its evolution throughout a solid's phase diagram often determines phenomena such as superconductivity, charge- and spin-density waves. Its experimental determination relies on the…

Electron-phonon coupling (EPC) is foundational in condensed matter physics, determining intriguing phenomena and properties in both conventional and quantum materials. In this manuscript, we propose and demonstrate a novel two dimensional…

材料科学 · 物理学 2025-04-09 Sheng Qu , Vishal K. Sharma , Jaco Geuchies , Maksim Grechko , Mischa Bonn , Falko Pientka , Heejae Kim

Monolayers of transition metal dichalcogenide materials emerged as a new material class to study excitonic effects in solid state, since they benefit from enormous coulomb correlations between electrons and holes. Especially in WSe2, sharp…

Atomically thin layer transition metal dichalcogenides have been intensively investigated for their rich optical properties and potential applications in nano-electronics. In this work, we study the incoherent optical phonon and exciton…

Light emitters in vicinity of a hyperbolic metamaterial (HMM) show a range of quantum optical phenomena from spontaneous decay rate enhancement to strong coupling. In this study, we integrate monolayer Molybdenum disulfide (MoS$_2$) emitter…

光学 · 物理学 2022-08-05 Harshavardhan R. Kalluru , Jaydeep K. Basu