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Exciton dynamics can be strongly affected by lattice vibrations through electron-phonon coupling. This is rarely explored in two-dimensional magnetic semiconductors. Focusing on bilayer CrI3, we first show the presence of strong…

Synthetic powder, ore samples and mineral single crystals of goethite ($\alpha-$FeOOH) were investigated with polarized Raman spectroscopy at temperatures from 300 K to 473 K. The symmetry of the vibrational modes, observed in different…

材料科学 · 物理学 2020-06-24 M. V. Abrashev , V. G. Ivanov , B. S. Stefanov , N. D. Todorov , J. Rosell , V. Skumryev

The polycrystalline co-doped samples of Sm0.5Y0.5Fe0.58Mn0.42O3 were prepared by solid-state reaction route and its various physical properties with their correlations have been investigated. The dc magnetization measurements on the sample…

Quasi-2D van der Waals ferromagnet Fe$_4$GeTe$_2$, featuring the simultaneous presence of high Curie temperature ($T_\mathrm{C}$ $\sim 270$ K) and a spin-reorientation transition at $T_\mathrm{SR}$ $\sim 110$ K, is a rare system where…

In this study, we propose that the signatures of spin fractionalization in quantum magnets can be identified through a detailed analysis of the temperature dependence of the asymmetric Fano lineshape of optical phonons overlapping with a…

强关联电子 · 物理学 2024-10-15 Swetlana Swarup , Susmita Singh , Natalia B. Perkins

We report low-temperature Raman signatures of the Heisenberg quantum magnet Ca$_{10}$Cr$_7$O$_{28}$, showing clear anomalies in phonon mode frequencies and linewidths below $\sim$100 K. This crossover temperature lies in between the…

强关联电子 · 物理学 2023-12-12 Srishti Pal , Arnab Seth , Anzar Ali , Yogesh Singh , D. V. S. Muthu , Subhro Bhattacharjee , A. K. Sood

We have carried out an extensive phonon study on multiferroic GaFeO3 to elucidate its dynamical behavior. Inelastic neutron scattering measurements are performed over a wide temperature range, 150 to 1198 K. First principles lattice…

材料科学 · 物理学 2015-06-19 M. K. Gupta , R. Mittal , M. Zbiri , Ripandeep Singh , S. Rols , H. Schober , S. L. Chaplot

We used Raman scattering to study the lattice and magnetic excitations in the hexagonal HoMnO3 single crystals. The E2 phonon mode at 237 cm-1 is affected by the magnetic order. This mode is related to the displacement of Mn and O ions in…

强关联电子 · 物理学 2018-10-17 J. Liu , Y. Gallais , M-A. Measson , A. Sacuto , S. W. Cheong , M. Cazayous

The symmetric splitting of two spin-wave branches in an antiferromagnetic resonance (AFR) experiment has been an essential measurement of antiferromagnets for over half a century. In this work, circularly polarized time-domain THz…

强关联电子 · 物理学 2017-12-05 N. J. Laurita , Yi Luo , Rongwei Hu , Meixia Wu , S. W. Cheong , O. Tchernyshyov , N. P. Armitage

The temperature and magnetic field dependence of lattice and carrier excitations in MnSi is studied in detail using inelastic light scattering. The pure symmetry components of the electronic response are derived from the polarization…

强关联电子 · 物理学 2014-07-23 H. -M. Eiter , P. Jaschke , R. Hackl , A. Bauer , M. Gangl , C. Pfleiderer

Inelastic light scattering studies on single crystal of electron-doped Ca(Fe0.95Co0.05)2As2 superconductor, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at TSM ~ 140 K and superconducting…

Two-dimensional (2D) van der Waals (vdW) magnets with spin-phonon coupling are crucial for next-generation spintronics. Among them, Fe3GaTe2 has attracted widespread attention due to above-room-temperature intrinsic ferromagnetism and large…

材料科学 · 物理学 2024-12-02 Gaojie Zhang , Hao Wu , Li Yang , Wen Jin , Bichen Xiao , Wenfeng Zhang , Haixin Chang

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

强关联电子 · 物理学 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado

Raman scattering spectra of zigzag spin chain TaFe$_{1.25}$Te$_3$ single crystal are presented in a temperature range from 80 to 300 K. Nine Raman active modes of $A_g$ and $B_g$ symmetry are clearly observed and assigned by probing…

The lattice dynamics of the $\rm YMnO_3$ magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data…

材料科学 · 物理学 2012-03-09 Julien Varignon , Sébastien Petit , Marie-Bernadette Lepetit

Fe3GeTe2 has emerged as one of the most fascinating van der Waals crystals due to its two-dimensional (2D) itinerant ferromagnetism, topological nodal lines and Kondo lattice behavior. However, lattice dynamics, chirality of phonons and…

In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman and dielectric spectroscopic study. Pr$_2$CoMnO$_6$ is a manganite compound , it undergoes a paramagnetic to…

强关联电子 · 物理学 2021-04-13 Ilyas Noor Bhatti , Imtiaz Noor Bhatti

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

强关联电子 · 物理学 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

The magneto-electric (ME) coupling on spin-wave resonances in single-crystal Cu2OSeO3 was studied by a novel technique using electron spin resonance combined with electric field modulation. An external electric field E induces a magnetic…

强关联电子 · 物理学 2015-06-04 A. Maisuradze , A. Shengelaya , H. Berger , D. M. Djokić , H. Keller

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

材料科学 · 物理学 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch