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This work presents methods of controlling the density of self-assembled CdTe quantum dots (QDs) grown by molecular beam epitaxy. Two approaches are discussed: increasing the deposition temperature of CdTe and the reduction of CdTe layer…

介观与纳米尺度物理 · 物理学 2016-10-20 J. Kobak , J. -G. Rousset , R. Rudniewski , E. Janik , Słupiński , P. Kossacki , A. Golnik , W. Pacuski

In this paper, we study theoretically the electron and spectral properties of Ge1-xSnx systems, including alloys, cubic- and spherical quantum dots. The single-particle electron and hole states are calculated within the sp3d5s*…

介观与纳米尺度物理 · 物理学 2024-06-21 Krzysztof Gawarecki , Jakub Ziembicki , Paweł Scharoch , Robert Kudrawiec

Semiconductor nanocrystals, quantum dots, are known to exhibit the quantum-confined Stark effect which reveals itself in the shift of their photoluminescence spectra in response to external electric field. It was, therefore, proposed to use…

等离子体物理 · 物理学 2022-04-04 Mikhail Pustylnik

Giant shell CdSe/CdS quantum dots are bright and flexible emitters, with near-unity quantum yield and suppressed blinking, but their single photon purity is reduced by efficient multiexcitonic emission. We report the observation, at the…

Images of a single-electron quantum dot were obtained in the Coulomb blockade regime at liquid He temperatures using a cooled scanning probe microscope (SPM). The charged SPM tip shifts the lowest energy level in the dot and creates a ring…

Systematic ensemble photoluminescence studies have been performed on type-I InP-quantum dots in Al0.20Ga0.80InP barriers, emitting at approximately 1.85 eV at 5 K. The influence of different barrier configurations as well as the…

Fluorophores emitting in the NIR-IIb wavelength range (1.5 micron - 1.7 micron) show great potential for bioimaging due to their large tissue penetration. However, current fluorophores suffer from poor emission with quantum yields ~2% in…

材料科学 · 物理学 2023-01-26 Ananth Kamath , Richard D. Schaller , Philippe Guyot-Sionnest

The strong confinement of semiconductor excitons in a quantum dot gives rise to atom-like behavior. The full benefit of such a structure is best observed in resonant excitation where the excited state can be deterministically populated and…

Electronic coupling and hence hybridization of atoms serve as the basis for the rich properties of the endless library of naturally occurring molecules. Colloidal quantum dots (CQDs) manifesting quantum strong confinement, possess atomic…

介观与纳米尺度物理 · 物理学 2021-03-09 Somnath Koley , Jiabin Cui , Yossef E. Panfil , Uri Banin

Hot electrons play a crucial role in enhancing the efficiency of photon-to-current conversion or photocatalytic reactions. In semiconductor nanocrystals, energetic hot electrons capable of photoemission can be generated via the upconversion…

化学物理 · 物理学 2022-09-07 Chih-Wei Wang , Xiaohan Liu , Tian Qiao , Mohit Khurana , Alexey V. Akimov , Dong Hee Son

Carbon quantum dots (CQDs) are known for their antibacterial properties and ability to inhibit bacteria growth. In the current study, we observed a dopant and concentration-dependency on the antibacterial effect of CQDs. High concentrations…

Coherent interaction between matter and periodic light field induces both optical Stark effect (OSE) and Bloch-Siegert shift (BSS). Observing the BSS has been historically challenging, not only because it is weak but it is often accompanied…

介观与纳米尺度物理 · 物理学 2022-10-12 Yuxuan Li , Yaoyao Han , Wenfei Liang , Boyu Zhang , Yulu Li , Yuan Liu , Yupeng Yang , Jingyi Zhu , Kaifeng Wu

We report the colloidal synthesis of strongly fluorescent CsPbBr3 perovskite nanowires (NWs) with rectangular section and with tuneable width, from 20 nm (exhibiting no quantum confinement, hence emitting in the green) down to around 3 nm…

Quantum droplets, stabilized by beyond-mean-field effects, represent a novel state of matter in quantum many-body systems. While previous studies have focused primarily on dipolar and contact-interacting systems, quadrupolar condensates…

量子气体 · 物理学 2025-10-16 Wei-qi Xia , Xiao-ting Zheng , Xiao-wei Chen , Gui-hua Chen

We report highly tunable control of holes in Ge/Si core/shell nanowires (NWs). We demonstrate the ability to create single quantum dots (QDs) of various sizes, with low hole occupation numbers and clearly observable excited states. For the…

Lead halide perovskites possess high photoluminescence (PL) efficiency and strong electron-phonon interactions, and therefore the optical cooling using up-conversion PL has been expected. We investigate anti-Stokes PL from green-luminescent…

Dilute arrays of GaAs/AlGaAs modulation-doped quantum dots (QDs) fabricated by electron-beam lithography and low impact reactive-ion etching exhibit highly homogeneous luminescence. Single quantum dots display spectral emission with peak…

We study the formation of quantum droplets in the mixture of a single-component Bose-Einstein condensate (BEC), and a two-species Fermi superfluid across a wide Feshbach resonance. With repulsive boson-boson and attractive boson-fermion…

量子气体 · 物理学 2020-07-07 Jing-Bo Wang , Jian-Song Pan , Xiaoling Cui , Wei Yi

A sequence of photoluminescence spectroscopy based methods are used to rigorously identify and study all the main spectral features (more than thirty emission lines) of site controlled InGaAs/AlGaAs quantum dots (QDs) grown along [111]B in…

An experimental observation on irreversible thermal quenching and antiquenching behavior is reported for photoluminescence (PL) of ZnS/CdS:Mn/ZnS quantum well quantum dots (QWQDs) prepared with a reverse micelle method. The dual-color…

材料科学 · 物理学 2013-09-20 X. Ding , R. C. Dai , Z. Zhao , Z. P. Wang , Z. Q. Sun , Z. M. Zhang , Z. J. Ding