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In this work, we investigate crystallization from droplets formed on micro-patterned surfaces. By solvent exchange in a micro-chamber, a ternary solution consisting of a model compound beta-alanine, water, and isopropanol, was displaced by…

软凝聚态物质 · 物理学 2021-04-16 Howon Choi , Zixiang Wei , Jae Bem You , Huaiyu Yang , Xuehua Zhang

Solvent shifting is a process in which a non-solvent is added to a solvent/solute mixture and extracts the solvent. The solvent and the non-solvent are miscible. Because of solution supersaturation a portion of the solute transforms to…

流体动力学 · 物理学 2014-09-30 Ramin Hajian , Steffen Hardt

Nanodroplets on a solid surface (i.e. surface nanodroplets) have practical implications for high-throughput chemical and biological analysis, lubrications, lab-on-chip devices, and near-field imaging techniques. Oil nanodroplets can be…

流体动力学 · 物理学 2017-06-07 Xuehua Zhanga , Ziyang Lu , Huanshu Tan , Lei Bao , Yinghe He , Chao Sun , Detlef Lohse

Solvent exchange is a process involving mixing between a good solvent with dissolved solute and a poor solvent. The process creates local oversaturation which causes the nucleation of minute solute droplets. Such ternary systems on a…

流体动力学 · 物理学 2022-06-07 You-An Lee , Chao Sun , Sander G. Huisman , Detlef Lohse

Recently, there has been much interest in using lubricated flat and nano-/micro-structured surfaces to achieve extreme liquid-repellency: any foreign droplet immiscible with the underlying lubricant layer was shown to slide off at a small…

流体动力学 · 物理学 2017-07-26 Dan Daniel , Jaakko V. I. Timonen , Ruoping Li , Seneca J. Velling , Joanna Aizenberg

The sensitive and reliable in-droplet chemical analysis benefits from the enhanced partition of an analyte into the droplets. This work, we will show that chemical reactions in surface nanodroplets can shift the partition of analytes from a…

软凝聚态物质 · 物理学 2021-10-04 Zixiang Wei , Jae Bem You , Hongbo Zeng , Xuehua Zhang

Solvent exchange is a controlled process for dilution-induced phase separation. This work utilizes the solvent exchange method to reveal the effect of the mixing dynamics on the asphaltene precipitation process under 20 different mixing…

流体动力学 · 物理学 2022-09-02 Jia Meng , Chiranjeevi Kanike , Somasekhara Goud Sontti , Arnab Atta , Xiaoli Tan , Xuehua Zhang

The evaporation of a droplet induces variety of ordered patterns near the contact line between the droplet and a substrate. This pattern formation involves both the behavior of colloidal suspensions and interactions between a droplet and a…

软凝聚态物质 · 物理学 2024-08-05 Yusaku Abe , Yu Matsuda

Solvent exchange (also called solvent shifting or Ouzo effect) is a generally used bottom-up process to mass-produce nanoscale droplets. In this process, a good solvent for some oil is displaced by a poor one, leading to oil nanodroplet…

软凝聚态物质 · 物理学 2020-02-11 Binglin Zeng , Yuliang Wang , Xuehua Zhang , Detlef Lohse

The growth of surface plasmonic microbubbles in binary water/ethanol solutions is experimentally studied. The microbubbles are generated by illuminating a gold nanoparticle array with a continuous wave laser. Plasmonic bubbles exhibit…

How liquid transport occurs in confined spaces is relevant to many industrial and lab-scale processes, ranging from enhanced oil recovery to drug delivery systems. In this work, we investigate propelling microdroplets that form from…

软凝聚态物质 · 物理学 2021-06-15 Gilmar F. Arends , John M. Shaw , Xuehua Zhang

Solvent exchange is a simple method to produce surface nanodroplets on a substrate for a wide range of applications by displacing a solution of good solvent, poor solvent and oil (Solution A) by a poor solvent (Solution B). In this work, we…

软凝聚态物质 · 物理学 2020-05-19 Jia Meng , Jae Bem You , Xuehua Zhang

Ethanol is a common protein crystallization agent, precipitant, and denaturant, but also alters the dielectric properties of solutions. While ethanol-induced unfolding is largely ascribed to its hydrophobic parts, its effect on protein…

软凝聚态物质 · 物理学 2021-11-03 Jan Hansen , Rajeevann Uthayakumar , Jan Skov Pedersen , Stefan U. Egelhaaf , Florian Platten

This study investigates the interfacial tension, fluid mobility, and crystallization behavior of various saline and additive-modified solutions in a microfluidic chip environment, simulating pore-scale processes during CO2 injection. The…

The evaporation of particle-laden droplets on engineered surfaces underpins a wide range of technologies, from printed electronics to biosensing. While the influence of substrate topography on passive particle deposition is well…

软凝聚态物质 · 物理学 2025-12-01 Meneka Banik , Ranjini Bandyopadhyay

Segregation at surfaces of metal-covalent binary liquids is often non-classical and in extreme cases such as AuSi, the surface crystallizes above the melting point. In this study, we employ atomic-scale computational frameworks to study the…

材料科学 · 物理学 2021-07-21 Hailong Wang , Alireza Shahabi , Alain Karma , Moneesh Upmanyu

Droplet-based microfluidics has emerged as a powerful technology for the miniaturization and automation of biochemical assays. The replacement of surfactants by nanoparticles as interfacial stabilizers has gained increasing interest.…

软凝聚态物质 · 物理学 2019-06-21 Laura Andreina Chacon Orellana , Jean-Christophe Baret

The removal of liquid droplets from solid surfaces is central to cleaning, coatings and oil recovery. Here we investigate liquid droplets capillary lifted by an immiscible working liquid. The rising working liquid triggers the formation of…

软凝聚态物质 · 物理学 2025-08-05 Ke Sun , Jack R. Panter , Alvin C. M. Shek , Yonas Gizaw , Kislon Voïtchovsky , Halim Kusumaatmaja

We delineate and examine the distinct breakup modes of evaporating water-in-oil emulsion droplets under acoustic levitation. The emulsion droplets consist of decane/dodecane/tetradecane as oil, while the water concentration is varied from…

流体动力学 · 物理学 2020-02-21 D Chaitanya Kumar Rao , Saptarshi Basu

The behavior of an oil droplet pinned at the entrance of a micropore and subject to clossflow-induced shear is investigated numerically by solving the Navier-Stokes equation. We found that in the absence of crossflow, the critical…

流体动力学 · 物理学 2013-09-04 Tohid Darvishzadeh , Volodymyr V. Tarabara , Nikolai V. Priezjev
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