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We develop a general theory of electron--hole recombination in organic light emitting diodes that leads to formation of emissive singlet excitons and nonemissive triplet excitons. We briefly review other existing theories and show how our…

材料科学 · 物理学 2009-11-07 K. Tandon , S. Ramasesha , S. Mazumdar

It is well-known that exciton effects are determinant to understand the optical absorption spectrum of low-dimensional materials. However, the role of excitons in nonlinear optical responses has been much less investigated at an…

介观与纳米尺度物理 · 物理学 2024-06-21 J. J. Esteve-Paredes , M. A. García-Blázquez , A. J. Uría-Álvarez , M. Camarasa-Gómez , J. J. Palacios

Monolayers of transition metal dichalcogenides (TMDCs) feature exceptional optical properties that are dominated by excitons, tightly bound electron-hole pairs. Forming van der Waals heterostructures by deterministically stacking individual…

Exciton dissociation via the excitonic Mott transition (EMT) governs the high-density optical response of semiconductors and sets fundamental limits for optoelectronic devices. The EMT is conventionally linked to the onset of population…

Exciton condensation in an electron-hole bilayer system of monolayer transition metal dichalcogenides is analyzed at three different levels of theory to account for screening and quasiparticle renormalization. The large effective masses of…

介观与纳米尺度物理 · 物理学 2017-11-15 Bishwajit Debnath , Yafis Barlas , Darshana Wickramaratne , Mahesh R. Neupane , Roger K. Lake

The giant exciton binding energy and the richness of degrees of freedom make monolayer transition metal dichalcogenide an unprecedented playground for exploring exciton physics in 2D systems. Thanks to the well energetically separated…

介观与纳米尺度物理 · 物理学 2023-07-26 Bairen Zhu , Ke Xiao , Siyuan Yang , Kenji Watanabe , Takashi Taniguchi , Xiaodong Cui

Heterostructures of atomically thin van der Waals bonded monolayers have opened a unique platform to engineer Coulomb correlations, shaping excitonic, Mott insulating, or superconducting phases. In transition metal dichalcogenide…

Identifying materials hosting an excitonic insulator ground state has been one of the major pursuits in condensed matter physics in recent years. Promising candidates in transition metal chalcogenide compounds (TMC), including…

强关联电子 · 物理学 2026-03-20 Yao Zeng , Shi-Cong Mo , Wéi Wú

Interlayer excitons (IXs) in hetero-bilayers of transition metal dichalcogenides (TMDs) represent an exciting emergent class of long-lived dipolar composite bosons in an atomically thin, near-ideal two-dimensional (2D) system. The…

Motivated by the gigantic nonlinear optical response in the halogen-bridged Ni-compounds, the underlying electronic states of the compounds are examined in the one-dimensional two-band Hubbard model, by studying the current-current…

强关联电子 · 物理学 2009-11-10 H. Matsueda , T. Tohyama , S. Maekawa

We present a systematic theory of Coulomb interaction effects in the nonlinear optical processes in semiconductors using a perturbation series in the exciting laser field. The third-order dynamical response consists of phase-space filling…

凝聚态物理 · 物理学 2009-10-31 Th. Oestreich , K. Schoenhammer , L. J. Sham

The monolayer transition metal dichalcogenides are an emergent semiconductor platform exhibiting rich excitonic physics with coupled spin-valley degree of freedom and optical addressability. Here, we report a new series of low energy…

We study the coherent light-matter interactions of GaAs quantum wells associated with excitons, biexcitons and many-body effects. For most polarization configurations, excitonic features dominate the phase-resolved two-dimensional…

其他凝聚态物理 · 物理学 2011-12-13 Alan D. Bristow , Denis Karaiskaj , Xingcan Dai , Richard. P. Mirin , Steven T. Cundiff

Moir\'{e} superlattices in transition metal dichalcogenides (TMDs) heterobilayers exhibit various correlated insulating states driven by long-range Coulomb interactions, and these states crucially alter exciton resonances, particularly at…

材料科学 · 物理学 2025-11-04 Junghwan Kim , Dinh Van Tuan , Hanan Dery

The region surrounding the excitonic insulator phase is a three-component plasma composed of electrons, holes, and excitons. Due to the extended nature of the excitons, their presence influences the surrounding electrons and holes. We…

强关联电子 · 物理学 2015-06-22 B Zenker , D Ihle , F X Bronold , H Fehske

The electronic and optical properties of monolayer transition-metal dichalcogenides (TMDs) and van der Waals heterostructures are strongly subject to their dielectric environment. In each layer the field lines of the Coulomb interaction are…

Charge separated interlayer excitons in transition metal dichalcogenide (TMDC) heterobilayers are being explored for moir\'e exciton lattices and exciton condensates. The presence of permanent dipole moments and the poorly screened Coulomb…

介观与纳米尺度物理 · 物理学 2021-03-17 Jue Wang , Qianhui Shi , En-Min Shih , Lin Zhou , Wenjing Wu , Yusong Bai , Daniel A. Rhodes , Katayun Barmak , James Hone , Cory R. Dean , X. -Y. Zhu

It is shown that the strong Coulomb coupling in intrinsic suspended semiconducting transition metal dichalcogenides can exceed the critical value needed for an excitonic ground state. The dipole-allowed optical excitations then correspond…

材料科学 · 物理学 2015-09-02 Tineke Stroucken , Stephan W. Koch

Exciton-exciton annihilation (EEA), in which two excitons interact to generate high-energy excitations, is an important non-radiative channel in light-induced excited-state relaxation. When efficient, this process offers an alternative…

材料科学 · 物理学 2025-06-06 Guy Vosco , Sivan Refaely-Abramson

Excitons, the bosonic quasiparticle emerging from Coulomb interaction between electrons and holes, will undergo a Bose-Einstein condensation(BEC) and transition into a superfluid state with global phase coherence at low temperatures. An…