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Alkali metal dimers attached to the surface of helium nanodroplets are found to be efficiently doubly ionized by electron transfer-mediated decay (ETMD) when photoionizing the helium droplets. This process is evidenced by detecting in…

We describe an experimental setup comprised of a discharge source for supersonic beams of metastable helium atoms and a magneto-optical trap (MOT) for ultracold lithium atoms that makes it possible to study Penning ionization and…

化学物理 · 物理学 2020-10-22 Jonas Grzesiak , Takamasa Momose , Frank Stienkemeier , Marcel Mudrich , Katrin Dulitz

We develop a microscopic calculation scheme for the excitation spectrum of a single-electron atom localized near a dielectric nanostructure. The atom originally has an arbitrary degenerate structure of its Zeeman sublevels on its closed…

量子物理 · 物理学 2024-02-02 N. A. Moroz , L. V. Gerasimov , A. D. Manukhova , D. V. Kupriyanov

Rotation of molecules embedded in He nanodroplets is explored by a combination of fs laser-induced alignment experiments and angulon quasiparticle theory. We demonstrate that at low fluence of the fs alignment pulse, the molecule and its…

Two-dimensional dilute magnetic semiconductors has been recently reported in semiconducting transition metal dichalcogenides by the introduction of spin-polarized transition metal atoms as dopants. This is the case of vanadium-doped WS$_2$…

Colloidal semiconductor nanoplatelets, in which carriers are strongly confined only along one dimension, present fundamentally different excitonic properties than quantum dots, which support strong confinement in all three dimensions. In…

介观与纳米尺度物理 · 物理学 2020-01-08 Daniel Amgar , Gaoling Yang , Ron Tenne , Dan Oron

We observe the low-lying excitations of a molecular dimer formed by two electrons in a GaAs semiconductor quantum dot in which the number of confined electrons is tuned by optical illumination. By employing inelastic light scattering we…

介观与纳米尺度物理 · 物理学 2010-06-16 Achintya Singha , Vittorio Pellegrini , Aron Pinczuk , Loren N. Pfeiffer , Ken W. West , Massimo Rontani

Inelastic x-ray scattering (IXS) with very high (meV) energy resolution has become a valuable spectroscopic tool, complementing the well established coherent inelastic neutron scattering (INS) technique for phonon dispersion investigations.…

强关联电子 · 物理学 2009-11-07 M. d'Astuto , P. K. Mang , P. Giura , A. Shukla , A. Mirone , M. Krisch , F. Sette , P. Ghigna , M. Braden , M. Greven

We have experimentally studied the electronic $3p\leftarrow 3s$ excitation of Na atoms attached to $^3$He droplets by means of laser-induced fluorescence as well as beam depletion spectroscopy. From the similarities of the spectra…

凝聚态物理 · 物理学 2009-11-10 F. Stienkemeier , O. Bunermann , R. Mayol , F. Ancilotto , M. Barranco , M. Pi

We investigate the electronic band structure of modulation-doped GaAs/AlGaAs core-shell nanowires for both n- and p-doping. We developed an 8-band Burt-Foreman k.p Hamiltonian approach to describe coupled conduction and valence bands in…

介观与纳米尺度物理 · 物理学 2022-06-13 Andrea Vezzosi , Andrea Bertoni , Guido Goldoni

In the presence of an active medium incorporated in a Penning trap, the moving electrons can become bunched, as they get enough energy, they escape the trap forming an optical injector. These bunched electrons can enter next PASER section…

加速器物理 · 物理学 2016-01-20 Xiu-fang Tian , Cong-feng Wu , Qika Jia

Doped clusters in the gas phase provide nanoconfined model systems for the study of system-bath interactions. To gain insight into interaction mechanisms between chromophores and their environment, the ensemble inhomogeneity has to be…

化学物理 · 物理学 2022-06-14 Ulrich Bangert , Frank Stienkemeier , Lukas Bruder

Resonances are among the clearest quantum mechanical signatures of scattering processes. Previously, shape resonances and Feshbach resonances have been observed in inelastic and reactive collisions involving atoms or diatomic molecules.…

化学物理 · 物理学 2015-05-05 Justin Jankunas , Krzysztof Jachymski , Michal Hapka , Andreas Osterwalder

Molecular dynamics simulations were employed to study the wetting behavior of nanoscale aqueous hydrophilic and hydrophobic Imidazolium based ionic liquid (IL) droplets on a solid graphite substrate subjected to the perpendicular electric…

软凝聚态物质 · 物理学 2020-12-09 Sanchari Bhattacharjee , Sandip Khan

Helium atom scattering (HAS) studies of the H-covered Mo(110) and W(110) surfaces reveal a twofold anomaly in the respective dispersion curves. In order to explain this unusual behavior we performed density functional theory calculations of…

mtrl-th · 物理学 2009-10-30 Bernd Kohler , Paolo Ruggerone , Matthias Scheffler

The relaxation of photoexcited nanosystems is a fundamental process of light-matter interaction. Depending on the couplings of the internal degrees of freedom, relaxation can be ultrafast, converting electronic energy in a few fs, or slow,…

Plasmons and polar phonons are elementary electrodynamic excitations of matter. In 2d and at long wavelengths, they couple to light and act as the system polaritons. They also dictate the scattering of charged carriers. Van der Waals…

材料科学 · 物理学 2025-06-10 Francesco Macheda , Francesco Mauri , Thibault Sohier

The study of phonon coupling in doped semiconductors via electrical transport measurements is challenging due to unwanted temperature-induced effects such as dopant ionisation and parallel conduction. Here, we study phonon scattering in 2D…

介观与纳米尺度物理 · 物理学 2025-03-03 Y. Ashlea Alava , K. Kumar , C. Harsas , P. Mehta , P. Hathi , C. Chen , D. A. Ritchie , A. R. Hamilton

We report spectra of various benzene isotopomers and their dimers in helium nanodroplets in the region of the first Herzberg-Teller allowed vibronic transition 610 1B2u<-1A1g (the A00 transition) at ~260 nm. Excitation spectra have been…

In this work, the electronic and optical properties of a Nitrogen (N) or a Boron (B) doped BeO monolayer are investigated in the framework of density functional theory. It is known that the band gap of a BeO monolayer is large leading to…