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Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

A model of a finite cylindrical ion channel through a phospholipid membrane of width $L$ separating two electrolyte reservoirs is studied. Analytical solution of the Poisson equation is obtained for an arbitrary distribution of ions inside…

软凝聚态物质 · 物理学 2009-11-11 Yan Levin

Statistically studied are the equilibrium characteristics of a subsystem of mobile charges of one sort, taking into account the subsystem of fixed charges of the opposite sign creating a compensating electric background. The distribution of…

其他凝聚态物理 · 物理学 2019-02-07 H. S. Bokun , D. di Caprio

We study the response of a model micro-electrochemical cell to a large ac voltage of frequency comparable to the inverse cell relaxation time. To bring out the basic physics, we consider the simplest possible model of a symmetric binary…

流体动力学 · 物理学 2013-12-12 Laurits H. Olesen , Martin Z. Bazant , Henrik Bruus

Effects of the adsorption-desorption process on the immittance response of an electrolytic cell are theoretically investigated in the framework of the diffusional Poisson-Nernst-Planck (PNP) continuum model, when the generation and…

On the elementary level, electronic current consists of individual electron tunnelling events that are separated by random time intervals. The waiting time distribution is a probability to observe the electron transfer in the detector…

介观与纳米尺度物理 · 物理学 2017-02-21 Daniel S. Kosov

Understanding the behaviour of vortices under nanoscale confinement in superconducting circuits is of importance for development of superconducting electronics and quantum technologies. Using numerical simulations based on the…

超导电性 · 物理学 2022-10-19 Benjamin A. McNaughton , Nicola Pinto , Andrea Perali , Milorad V. Milosevic

Porous electrodes are found in energy storage devices such as supercapacitors and pseudocapacitors. However, the effect of electrode-pore-size distribution over their energy storage properties remains unclear. Here, we develop a model for…

化学物理 · 物理学 2021-12-03 Filipe Henrique , Pawel J. Zuk , Ankur Gupta

We reformulate and extend porous electrode theory for non-ideal active materials, including those capable of phase transformations. Using principles of non-equilibrium thermodynamics, we relate the cell voltage, ionic fluxes, and Faradaic…

化学物理 · 物理学 2012-08-24 Todd R. Ferguson , Martin Z. Bazant

Linear sweep and cyclic voltammetry techniques are important tools for electrochemists and have a variety of applications in engineering. Voltammetry has classically been treated with the Randles-Sevcik equation, which assumes an…

化学物理 · 物理学 2017-03-15 David Yan , Martin Z. Bazant , P. M. Biesheuvel , Mary C. Pugh , Francis P. Dawson

Warming in complex physical systems, in particular global warming, attracts significant contemporary interest. It is essential, therefore, to understand basic physical mechanisms leading to overheating. It is well known that application of…

介观与纳米尺度物理 · 物理学 2008-07-04 N. Romero Kalmanovitz , A. A. Bykov , S. A. Vitkalov , A. I. Toropov

Recent experiments suggest the possibility to tune superconductivity in metallic nanowires by application of modest gate voltages. It is largely debated whether the effect is due to an electric field at the superconductor surface or small…

超导电性 · 物理学 2022-04-13 M. F. Ritter , N. Crescini , D. Z. Haxell , M. Hinderling , H. Riel , C. Bruder , A. Fuhrer , F. Nichele

Neurons regulate the distribution of signaling components across an extended tree-like cellular structure using both local and global feedback control. This is hypothesized to allow homeostatic control of the electrical activity of a neuron…

适应与自组织系统 · 物理学 2021-04-27 Saeed Aljaberi , Adriano Bellotti , Timothy O'Leary , Fulvio Forni

We scrutinize the diagrammatic perturbation theory of noninteracting electrons in a random potential with the aim to accomplish a consistent comprehensive theory of quantum diffusion. Ward identity between the one-electron self-energy and…

无序系统与神经网络 · 物理学 2017-01-17 V. Janiš , J. Kolorenč

A system of drift-diffusion equations for the electron, hole, and oxygene vacancy densities in a semiconductor, coupled to the Poisson equation for the electric potential, is analyzed in a bounded domain with mixed Dirichlet-Neumann…

偏微分方程分析 · 数学 2022-04-08 Clément Jourdana , Ansgar Jüngel , Nicola Zamponi

This work is concerned with the stationary Poisson--Nernst--Planck equation with a large parameter which describes a huge number of ions occupying an electrolytic region. Firstly, we focus on the model with a single specie of positive…

偏微分方程分析 · 数学 2023-11-20 Jhih-Hong Lyu , Chiun-Chang Lee , Tai-Chia Lin

Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

化学物理 · 物理学 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

The role of kinetic electrons in the excitation and sustainment of ion-bulk electrostatic waves in collisionless plasmas is investigated, with a focus on the physical mechanisms responsible for the generation of small-scale structures in…

We use a 30-nm x-ray beam to study the spatially resolved properties of a SmNiO$_3$-based nanodevice that is doped with protons. The x-ray absorption spectra supported by density-functional theory (DFT) simulations show partial reduction of…

A model is constructed to describe the arbitrary deformation of a drop or vesicle that contains and is embedded in an electrolyte solution, where the deformation is caused by an applied electric field. The applied field produces an…

流体动力学 · 物理学 2022-07-13 Manman Ma , Michael R. Booty , Michael Siegel