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Selected configuration interaction (SCI) methods, when complemented with a second-order perturbative correction, provide near full configuration interaction (FCI) quality energies with only a small fraction of the Slater determinants of the…

We show that a naive treatment of open-shell systems in hybrid density functional calculations ignoring the spin dependence causes significant errors due to a kind of self interaction that is not emerged in spin-dependent calculations. As…

材料科学 · 物理学 2016-05-03 Jun-Ichi Iwata , Keisuke Sawada , Atsushi Oshiyama

We discuss various ways to handle self-interaction corrections (SIC) to Density Functional Theory (DFT) calculations. To that end, we use a simple model of few particles in a finite number of states together with a simple zero-range…

其他凝聚态物理 · 物理学 2009-11-13 P. M. Dinh , J. Messud , P. -G. Reinhard , E. Suraud

The small magnitude and long-range character of non-covalent interactions pose a significant challenge for computational quantum chemical and electronic-structure methods alike. State-of-the-art coupled cluster (CC) theory and…

化学物理 · 物理学 2026-01-22 S. Lambie , P. López-Ríos , D. Kats , Ali Alavi

The newly developed "strongly constrained and appropriately normed" (SCAN) meta-generalized-gradient approximation (meta-GGA) can generally improve over the non-empirical Perdew-Burke-Ernzerhof (PBE) GGA not only for strong chemical…

材料科学 · 物理学 2016-10-19 Haowei Peng , Zeng-Hui Yang , Jianwei Sun , John P. Perdew

Molecular dynamics simulations of water, liquid beryllium fluoride and silica melt are used to study the accuracy with which the entropy of ionic and molecular liquids can be estimated from atom-atom radial distribution function data. All…

软凝聚态物质 · 物理学 2009-11-13 Ruchi Sharma , Manish Agarwal , Charusita Chakravarty

High-throughput DFT calculations are key to screening existing/novel materials, sampling potential energy surfaces, and generating quantum mechanical data for machine learning. By including a fraction of exact exchange (EXX), hybrid…

Self interaction error remains an impotrant problem in density functional theory. A number of approximations to exact exchange aimed to correct for this error while retainining computational efficiency had been suggested recently. We…

化学物理 · 物理学 2012-01-31 Valentin V. Karasiev , Eduardo V. Ludeña , Artëm E. Masunov

The study of defects in materials is of utmost importance for technological applications and the design of new materials. In this work, we analyze the performance of density functional approximations on two prototypical sets of defective…

Side-scan sonar (SSS) images are susceptible to motion-induced geometric distortion, which degrades their reliability for seabed interpretation and downstream tasks. Existing correction methods either exploit image-domain consistency…

大气与海洋物理 · 物理学 2026-04-23 Can Lei , Valerio Franchi , Hayat Rajani , Nuno Gracias , Rafael Garcia , Huigang Wang

Recent investigations have found that the strongly constrained and appropriately normed (SCAN) meta-GGA exchange-correlation functional significantly over-magnetizes elemental Fe, Co, and Ni solids. For the paradigmatic case, bcc Fe, the…

材料科学 · 物理学 2019-07-24 Daniel Mejia-Rodriguez , S. B. Trickey

Electronic resonances are metastable states with finite lifetimes, encountered in processes such as photodetachment, electron transmission, and Auger decay. Resonances appear in Hermitian quantum mechanics as increased density of states in…

化学物理 · 物理学 2025-11-10 Cansu Utku , Garrette Pauley Paran , Thomas-C. Jagau

This paper studies the joint digital self-interference (SI) cancellation and data detection in an orthogonal-frequency-division-multiplexing (OFDM) full-duplex (FD) system, considering the effect of phase noise introduced by the oscillators…

信息论 · 计算机科学 2023-08-11 Meng He , Chuan Huang

This paper investigates a robust joint power allocation and beamforming scheme for in-band full-duplex multi-cell multi-user (IBFD-MCMU) networks. A mean-squared error (MSE) minimization problem is formulated with constraints on the power…

信息论 · 计算机科学 2024-03-19 Haifeng Luo , Navneet Garg , Mark Holm , Tharmalingam Ratnarajah

Previous approaches for blind image super-resolution (SR) have relied on degradation estimation to restore high-resolution (HR) images from their low-resolution (LR) counterparts. However, accurate degradation estimation poses significant…

图像与视频处理 · 电气工程与系统科学 2024-03-13 Haochen Sun , Yan Yuan , Lijuan Su , Haotian Shao

The smoothed-particle hydrodynamics (SPH) technique is a numerical method for solving gas-dynamical problems. It has been applied to simulate the evolution of a wide variety of astrophysical systems. The method has a second-order accuracy,…

天体物理仪器与方法 · 物理学 2016-08-08 Domingo García-Senz , Rubén M. Cabezón , José A. Escartín , Kevin Ebinger

We report calculations of the surface tension of the water-air interface using ab initio molecular dynamics (AIMD) simulations. We investigate the simulation cell size dependence of the surface tension of water from force field molecular…

化学物理 · 物理学 2016-06-22 Yuki Nagata , Tatsuhiko Ohto , Mischa Bonn , Thomas D Kühne

The development of novel materials for vacuum electron sources in particle accelerators is an active field of research that can greatly benefit from the results of \textit{ab initio} calculations for the characterization of the electronic…

材料科学 · 物理学 2021-06-01 Holger-Dietrich Saßnick , Caterina Cocchi

The cluster-in-molecule (CIM) local correlation approach with an accurate distant pair correlation energy correction is presented. For large systems, the inclusion of distant pair correlation energies is essential for the accurate…

化学物理 · 物理学 2020-08-06 Zhigang Ni , Yang Guo , Frank Neese , Wei Li , Shuhua Li

We present a modification to our recently published SAFT-based classical density functional theory for water. We have recently developed and tested a functional for the averaged radial distribution function at contact of the hard-sphere…

软凝聚态物质 · 物理学 2015-06-17 Eric J. Krebs , Jeff B. Schulte , David Roundy