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The direct manipulation of individual atoms in materials using scanning probe microscopy has been a seminal achievement of nanotechnology. Recent advances in imaging resolution and sample stability have made scanning transmission electron…

The burgeoning field of atomic level material control holds great promise for future breakthroughs in quantum and memristive device manufacture and fundamental studies of atomic-scale chemistry. Realization of atom-by atom control of matter…

材料科学 · 物理学 2018-08-06 Ondrej Dyck , Songkil Kim , Sergei V. Kalinin , Stephen Jesse

Electron-beam (e-beam) manipulation of single dopant atoms in an aberration-corrected scanning transmission electron microscope is emerging as a method for directed atomic motion and atom-by-atom assembly. Until now, the dopant species have…

We demonstrate assembly of di-, tri- and tetrameric Si clusters on the graphene surface using sub-atomically focused electron beam of a scanning transmission electron microscope. Here, an electron beam is used to introduce Si substitutional…

Despite decades of research, the ultimate goal of nanotechnology--top-down manipulation of individual atoms--has been directly achieved with only one technique: scanning probe microscopy. In this Review, we demonstrate that scanning…

We demonstrate high-resolution modification of suspended multi-layer graphene sheets by controlled exposure to the focused electron beam of a transmission electron microscope. We show that this technique can be used to realize, on…

介观与纳米尺度物理 · 物理学 2009-11-13 Michael D. Fischbein , Marija Drndic

Direct-write processes enable the alteration or deposition of materials in a continuous, directable, sequential fashion. In this work we demonstrate an electron beam direct-write process in an aberration-corrected scanning transmission…

材料科学 · 物理学 2023-03-22 Ondrej Dyck , Andrew R. Lupini , Stephen Jesse

We demonstrate that the sub-atomically focused beam of a scanning transmission electron microscope (STEM) can be used to controllably manipulate individual dopant atoms in a 2D graphene lattice. We demonstrate the manipulation of adsorbed…

材料科学 · 物理学 2018-08-06 Ondrej Dyck , Songkil Kim , Sergei V. Kalinin , Stephen Jesse

The directed self-assembly of colloidal nanoparticles (NPs) using external fields guides the formation of sophisticated hierarchical materials but becomes less effective with decreasing particle size. As an alternative, electron-beam-driven…

软凝聚态物质 · 物理学 2024-09-13 Jonathan G. Raybin , Ethan J. Dunsworth , Veronica Guo , Naomi S. Ginsberg

We demonstrate a method by which few-layer graphene samples can be etched along crystallographic axes by thermally activated metallic nanoparticles. The technique results in long (>1 micron) crystallographic edges etched through to the…

材料科学 · 物理学 2009-05-08 Sujit S. Datta , Douglas R. Strachan , Samuel M. Khamis , A. T. Charlie Johnson

Directed atomic fabrication using an aberration-corrected scanning transmission electron microscope (STEM) opens new pathways for atomic engineering of functional materials. In this approach, the electron beam is used to actively alter the…

Using electron beam manipulation, we enable deterministic motion of individual Si atoms in graphene along predefined trajectories. Structural evolution during the dopant motion was explored, providing information on changes of the Si atom…

材料科学 · 物理学 2020-07-15 Maxim Ziatdinov , Stephen Jesse , Bobby G. Sumpter , Sergei V. Kalinin , Ondrej Dyck

Controlled fabrication of nanopores in atomically thin two-dimensional material offers the means to create robust membranes needed for ion transport, nanofiltration, and DNA sensing. Techniques for creating nanopores have relied upon either…

We report on the etching of graphene devices with a helium ion beam, including in situ electrical measurement during lithography. The etching process can be used to nanostructure and electrically isolate different regions in a graphene…

介观与纳米尺度物理 · 物理学 2009-10-08 M. C. Lemme , D. C. Bell , J. R. Williams , L. A. Stern , B. W. H. Baugher , P. Jarillo-Herrero , C. M. Marcus

Electromagnetically induced transparency (EIT) analogue in all-dielectric metamaterials with a high quality factor provides an effective route to enhance light-matter interaction at the nanoscale. In particular, the active control applied…

光学 · 物理学 2020-10-15 Tingting Liu , Huaixing Wang , Chaobiao Zhou , Xiaoyun Jiang , Shuyuan Xiao

Investigating the interaction of electron beams with materials and light has been a field of research since more than a century. The field was advanced theoretically by the raise of quantum mechanics and technically by the introduction of…

光学 · 物理学 2017-10-11 Nahid Talebi

Attosecond science has leveraged the highly nonlinear interactions between intense few-cycle laser pulses and matter, allowing for unprecedented observation and control of electron motion with remarkable temporal resolution. However, most…

介观与纳米尺度物理 · 物理学 2024-11-06 Mingrui Yuan , Husain Alqattan , Dandan Hui , Mohamed Sennary , Vladimir Pervak , Nikolay V. Golubev , Mohammed Th. Hassan

Chromium atoms in graphene have been proposed to exhibit magnetic moments and spin-selective conducting states depending on the local bonding geometry within the graphene structure, which could lead to interesting applications in…

材料科学 · 物理学 2023-07-13 Ondrej Dyck , Mina Yoon , Lizhi Zhang , Andrew R. Lupini , Jacob L. Swett , Stephen Jesse

In order to harvest the many promising properties of graphene in (electronic) applications, a technique is required to cut, shape or sculpt the material on a nanoscale without damage to its atomic structure, as this drastically influences…

材料科学 · 物理学 2011-09-01 Bo Song , Grégory F. Schneider , Qiang Xu , Grégory Pandraud , Cees Dekker , Henny Zandbergen

Recent advances in scanning transmission electron microscopy (STEM) instrumentation have made it possible to focus electron beams with sub-atomic precision and to identify the chemical structure of materials at the level of individual…

材料科学 · 物理学 2017-03-08 T. Susi , J. C. Meyer , J. Kotakoski
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