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The origin of the variation of photoluminescence (PL) spectra of monolayer tungsten disulfide (WS2) is investigated systematically. Dependence of the PL spectrum on the excitation power show that the relatively sharp component corresponds…

介观与纳米尺度物理 · 物理学 2018-06-01 Yongjae Kwon , Kangwon Kim , Wontaek Kim , Sunmin Ryu , Hyeonsik Cheong

The decay time of the linear polarization degree of the luminescence in strongly confined semiconductor quantum dots with asymmetrical shape is calculated in the frame of second-order quasielastic interaction between quantum dot charge…

介观与纳米尺度物理 · 物理学 2009-11-07 E. Tsitsishvili , R. v. Baltz , H. Kalt

We present a systematic study of the exciton/electron-hole plasma photoluminescence dynamics in bulk GaAs for various lattice temperatures and excitation densities. The competition between the exciton and electron-hole pair recombination…

材料科学 · 物理学 2009-11-22 A. Amo , M. D. Martin , L. Vina , A. I. Toropov , K. S. Zhuravlev

To provide physical insight into the recently observed photoluminescence saturation behaviors in single-walled carbon nanotubes implying the existence of an upper limit of exciton densities, we have performed a time-dependent theoretical…

介观与纳米尺度物理 · 物理学 2015-05-13 Ajit Srivastava , Junichiro Kono

The optical properties of C$_{60}$ single crystals, intercalated with nitrogen molecules, were investigated by the spectral-luminescence method in the temperature range 20 - 230 K. The saturation was carried out under the pressure of 30…

介观与纳米尺度物理 · 物理学 2021-09-29 P. V. Zinoviev , V. N. Zoryansky

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

材料科学 · 物理学 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

We present the micro-photoluminescence ($\mu$PL) and micro-reflectance contrast spectroscopy studies on thin films of MoSe2 with layer thicknesses ranging from a monolayer (1L) up to 5L. The thickness dependent evolution of the ground and…

介观与纳米尺度物理 · 物理学 2016-01-20 Ashish Arora , Karol Nogajewski , Maciej R. Molas , Maciej Koperski , Marek Potemski

Transition metal dichalcogenides hold promise for applications in novel optoelectronic devices. There is therefore a need for materials that can be obtained in large quantities and with well understood optical properties. In this report, we…

介观与纳米尺度物理 · 物理学 2018-01-04 Ł. Kłopotowski , C. Backes , A. A. Mitioglu , V. Vega-Mayoral , D. Hanlon , J. N. Coleman , V. Y. Ivanov , D. K. Maude , P. Plochocka

Two-dimensional transition metal di-chalcogenide semiconductors provide unique possibilities to investigate strongly confined excitonic physics and a plasmonic platform integrable to such materials constitutes a hybrid system that can be of…

介观与纳米尺度物理 · 物理学 2022-05-26 Bidisha Roy , Maex Blauth , Siddharth Dhomkar , Michael Kaniber , Vinod M. Menon , Jonathan. J. Finley

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

介观与纳米尺度物理 · 物理学 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

In this letter, we address the chiral properties of valley exciton-polaritons in a monolayer of WS2 in the regime of strong light-matter coupling with a Tamm-Plasmon resonance. We observe that the valley polarization, which manifests in the…

介观与纳米尺度物理 · 物理学 2017-12-13 N. Lundt , S. Stoll , P. Nagler , A. Nalitov , S. Klembt , S. Betzold , J. W. Goddard , E. Frieling , A. V. Kavokin , C. Schüller , T. Korn , S. Höfling , C. Schneider

The fine structure of the exciton spectrum, containing optically allowed (bright) and forbidden (dark) exciton states, determines the radiation efficiency in nanostructures. We study time-resolved micro-photoluminescence in MoS$_2$…

We develop a non-local dielectric response theory to describe the temperature dependence of exciton lifetime in metal-semiconductor heterostructures. Coupling between excitons and surface plasmons results in a strongly nonmonotonous…

介观与纳米尺度物理 · 物理学 2015-05-07 M. V. Durnev , A. V. Kavokin , B. Gil

Newly measured optical absorption and photoluminescence spectra reveal substantial frequency shifts of both exciton and trion peaks as monolayer MoS2 is cooled from 363 K to 4 K. First-principles simulations using the GW-Bethe-Salpeter…

介观与纳米尺度物理 · 物理学 2014-05-22 Ryan Soklaski , Yufeng Liang , Changjian Zhang , Haining Wang , Farhan Rana , Li Yang

The photoluminescence (PL) spectrum of transition metal dichalcogenides (TMDs) shows a multitude of emission peaks below the bright exciton line and not all of them have been explained yet. Here, we study the emission traces of…

Achieving localized light emission from monolayer two-dimensional (2D) transition metal dichalcogenides (TMDs) embedded in the matrix of another TMD has been theoretically proposed but not experimentally proven. In this study, we used…

We have investigated the steady-sate valley polarization and valley coherence of encapsulated MoS2 monolayer as a function of the temperature and the power density with a continuous wave laser excitation. Both valley polarization and…

材料科学 · 物理学 2021-11-01 Fabian Cadiz , Stefan Gerl , Takashi Taniguchi , Kenji Watanabe

We investigate effects of the local structure on the excitonic transport in C60 thin films by means of temperature-dependent photoluminescence quenching studies in a range of 5 to 300 K. Exciton motion in the X-ray amorphous layers…

材料科学 · 物理学 2013-10-30 A. K. Topczak , M. Gruber , W. Brütting , J. Pflaum

We have combined spatially-resolved steady-state micro-photoluminescence ($\mu$PL) with time-resolved photoluminescence (TRPL) to investigate the exciton diffusion in a WSe$_2$ monolayer encapsulated with hexagonal boron nitride (hBN). At…

介观与纳米尺度物理 · 物理学 2018-05-09 F. Cadiz , C. Robert , E. Courtade , M. Manca , L. Martinelli , T. Taniguchi , K. Watanabe , T. Amand , A. C. H. Rowe , D. Paget , B. Urbaszek , X. Marie

We report a photoluminescence (PL) and transient reflection spectroscopy study of exciton dynamics in monolayer transition transition-metal dichalcogenides (TMDs). PL saturation in monolayer MoSe2 occurs an excitation intensity more than…

介观与纳米尺度物理 · 物理学 2015-06-22 Min Ju Shin , Dong Hak Kim , D. Lim