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相关论文: Ballistic and shift currents in the bulk photovolt…

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The two-dimensional (2D) bulk photovoltaic effect (BPVE) is a cornerstone for future highly efficient 2D solar cells and optoelectronics. The ferromagnetic semiconductor 2H-FeCl2 is shown to realize a new type of BPVE in which spatial…

材料科学 · 物理学 2023-06-16 Liang Liu , Xiaolin Li , Luping Du , Xi Zhang

The bulk photovoltaic effect is a photocurrent generation from alternating electric field, which is a promising candidate for future efficient solar cell technology. It is the second-order optical current, which is the injection current or…

介观与纳米尺度物理 · 物理学 2025-05-22 Motohiko Ezawa

Broadband, efficient and fast conversion of light to electricity is crucial for sensing and clean energy. Here we reveal the largest observed bulk photo-voltaic effect (BPVE), an intrinsic mechanism predicted to be ultrafast and exceed the…

The bulk photovoltaic effect (BPVE) leads to directed photo-currents and photo-voltages in bulk materials. Unlike photo-voltages in p-n junction solar cells that are limited by carrier recombination to values below the bandgap energy of the…

应用物理 · 物理学 2023-03-17 Andreas Pusch , Udo Römer , Dimitrie Culcer , Nicholas J. Ekins-Daukes

Two-dimensional ferroelectrics have recently emerged as a promising avenue for next-generation optoelectronic and photovoltaic devices. Due to the intrinsic absence of inversion symmetry, 2D ferroelectrics exhibit bulk photovoltaic effect…

材料科学 · 物理学 2025-12-08 Francesco Delodovici , Brahim Dkhil , Charles Paillard

Bulk photovoltaic (BPVE) effect in crystals lacking inversion symmetry offers great potential for optoelectronic applications due to its unique properties such as above bandgap photovoltage and switchable photocurrent. Because of their…

材料科学 · 物理学 2021-10-27 Amr Abdelsamie , Lu You , Le Wang , Shuzhou Li , Mingqiang Gu , Junling Wang

We calculate the bulk photovoltaic response of the ferroelectrics BaTiO$_3$ and PbTiO$_3$ from first principles by applying "shift current" theory to the electronic structure from density functional theory. The first principles results for…

材料科学 · 物理学 2015-06-04 Steve M. Young , Andrew M. Rappe

Noncentrosymmetric bulk crystals generate photocurrent without any bias voltage. One of the dominant mechanisms, shift current, comes from a quantum interference of electron wave functions being distinct from classical current caused by…

材料科学 · 物理学 2018-12-17 M. Nakamura , H. Hatada , Y. Kaneko , N. Ogawa , Y. Tokura , M. Kawasaki

Spontaneous polarization and bulk photovoltaic effect (BPVE) are two concomitant physical properties in ferroelectric materials. The flipping of ferroelectric order usually accompanies with the switching of BPVE as both of them are reversed…

材料科学 · 物理学 2022-07-04 Rui-Chun Xiao , Yang Gao , Hua Jiang , Wei Gan , Changjin Zhang , Hui Li

The bulk photovoltaic effect (BPVE) offers a promising avenue to surpass the efficiency limitations of current solar cell technology. However, disentangling intrinsic and extrinsic contributions to photocurrent remains a significant…

The bulk photovoltaic effect is an experimentally verified phenomenon by which a direct charge current is induced within a non-centrosymmetric material by light illumination. Calculations of its intrinsic contribution, the shift current,…

材料科学 · 物理学 2023-08-21 M. A. García-Blázquez , J. J. Esteve-Paredes , A. J. Uría , J. J. Palacios

This paper presents a study of dc photocurrents in biased insulators to the third order in the electric field. We find three photocurrents which are characterized by physical divergences of the third-order free-electron polarization…

介观与纳米尺度物理 · 物理学 2019-08-07 Benjamin M. Fregoso

The bulk photovoltaic effect generates intrinsic photocurrents in materials without inversion symmetry. Shift current is one of the bulk photovoltaic phenomena related to the Berry phase of the constituting electronic bands: photo-excited…

材料科学 · 物理学 2020-07-17 Banasree Sadhukhan , Yang Zhang , Rajyavardhan Ray , Jeroen van den Brink

Photovoltaic effect, e.g., solar cells, converts light into DC electric current. This phenomenon takes place in various setups such as in noncentrosymmetric crystals and semiconductor pn junctions. Recently, we proposed a theory for…

强关联电子 · 物理学 2020-10-23 Masahiro Sato , Hiroaki Ishizuka

A recent scientific debate has arisen: Which processes underlie the actual ground of the valley Hall effect (VHE) in two-dimensional materials? The original VHE emerges in samples with ballistic transport of electrons due to the anomalous…

介观与纳米尺度物理 · 物理学 2021-02-03 I. Vakulchyk , V. M. Kovalev , I. G. Savenko

The bulk photovoltaic effect provides a fundamental pathway for direct light-to-current conversion in quantum materials. However, these nonlinear currents are often strictly constrained or forbidden by crystal symmetries, hindering their…

介观与纳米尺度物理 · 物理学 2026-05-25 Zhuocheng Lu , Zhuang Qian , Zhichao Guo , Likun Shi , Shi Liu , Hua Wang , Kai Chang

The rectified bulk photovoltaic effect (BPVE) in noncentrosymmetric semiconductors, also called shift current, is considered promising for optoelectronic devices, terahertz emission and possibly solar energy harvesting. A clear…

材料科学 · 物理学 2025-02-11 Urmimala Dey , Jeroen van den Brink , Rajyavardhan Ray

We study the bulk photovoltaic effect (BPVE) in Dirac and Weyl semimetals under two-frequency light irradiation. We show that the BPVE emerges for centrosymmetric Dirac and Weyl semimetals in the presence of light fields with frequencies…

介观与纳米尺度物理 · 物理学 2025-01-15 Yuya Ikeda , Sota Kitamura , Takahiro Morimoto

Bulk photovoltaic (BPV) effect, a second order nonlinear process that generates static current under light irradiation, requires centrosymmetric broken systems as its application platform. In order to realize measurable BPV photocurrent in…

材料科学 · 物理学 2023-01-05 Xingchi Mu , Qianqian Xue , Yan Sun , Jian Zhou

The bulk photovoltaic effect exhibited by the non-centrosymmetric system gains research interest due to the observed large open-circuit voltage. The ferroelectric systems exhibiting anomalous photovoltaic effect are mostly crystallized with…