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Polaritons are unique hybrid light-matter states that offer an alternative way to manipulate chemical processes and change material properties. In this work we theoretically demonstrate that singlet fission dynamics can be accelerated under…

化学物理 · 物理学 2021-10-06 Clàudia Climent , David Casanova , Johannes Feist , Francisco J. García-Vidal

We show strong coupling between antiferromagnetic magnons and microwave cavity photons at both high and externally controllable magnon frequencies. Using the fully quantum mechanical path-integral method, we study an antiferromagnetic…

介观与纳米尺度物理 · 物理学 2025-09-03 Henrik T. Kaarbø , Henning G. Hugdal , Sol H. Jacobsen

A light-matter hybrid quasiparticle, called a polariton, is formed when molecules are strongly coupled to an optical cavity. Recent experiments have shown that polariton chemistry can manipulate chemical reactions. Polariton chemistry is a…

化学物理 · 物理学 2024-01-11 Xinyang Li , Nicholas Lubbers , Sergei Tretiak , Kipton Barros , Yu Zhang

We propose a scheme to efficiently couple a single quantum dot electron spin to an optical nano-cavity, which enables us to simultaneously benefit from a cavity as an efficient photonic interface, as well as to perform high fidelity (nearly…

We propose an approach to generate strong quantum entanglement by the controllable four wave mixing mechanism in a single cavity, weak coupling optomechanical system. The optomechanical system is driven by a strong two tone pump field and a…

量子物理 · 物理学 2019-11-27 Xiang You , Yongmin Li

Purcell-enhanced emission from a coupled emitter-cavity system is a fundamental manifestation of cavity quantum electrodynamics. Starting from a theoretical description we derive a scheme for photon emission from an emitter coupled to a…

量子物理 · 物理学 2020-08-26 Thomas D. Barrett , Thomas H. Doherty , Axel Kuhn

We have studied the coherent excitation of a strongly coupled QD/photonic crystal cavity system. Time-resolved reflectivity measurements show the vacuum Rabi oscillation of the dot in the cavity. Next, we considered the resonant driving of…

Here we present the theoretical foundation of the strong coupling phenomenon between quantum emitters and propagating surface plasmons observed in two-dimensional metal surfaces. For that purpose, we develop an ab-initio quantum framework…

介观与纳米尺度物理 · 物理学 2013-04-11 A. Gonzalez-Tudela , P. A. Huidobro , L. Martin-Moreno , C. Tejedor , F. J. Garcia-Vidal

Strong interaction between light and a single quantum emitter is essential to a great number of applications, including single photon sources. Microcavities and plasmonic antennas have been used frequently to enhance these interactions…

光学 · 物理学 2016-12-01 Hugo Michiel Doeleman , Ewold Verhagen , A. Femius Koenderink

Strong light-matter coupling occurs when the coupling strength between a confined electromagnetic mode and a molecular resonance exceeds losses to the environment. The study of strong coupling has been motivated by applications such as…

介观与纳米尺度物理 · 物理学 2022-04-27 Philip A. Thomas , Kishan S. Menghrajani , William L. Barnes

We investigate the transmission spectrum of an optical cavity coupled with four-level atoms. Multiple normal-mode splitting peaks of the strongly coupled atom-cavity system are obtained as single cavity mode couples three separated atomic…

量子物理 · 物理学 2019-01-03 Zheng Tan , Liyong Wang , Min Liu , Yifu Zhu , Jin Wang , Mingsheng Zhan

Strong light-matter coupling is a quantum process in which light and matter are coupled together, generating hybridized states. This is similar to the notion of molecular hybridization, but one of the components is light. Here, we utilized…

应用物理 · 物理学 2024-02-20 Jhuma Dutta , Pooja Bhatt , Kuljeet Kaur , Daniel E. Gómez , Jino George

We present a detailed study of the electroluminescence of intersubband devices operating in the light-matter strong coupling regime. The devices have been characterized by performing angle resolved spectroscopy that shows two distinct light…

介观与纳米尺度物理 · 物理学 2012-12-27 Pierre Jouy , Angela Vasanelli , Yanko Todorov , Luca Sapienza , Raffaele Colombelli , Ulf Gennser , Carlo Sirtori

We study photon emission by an ensemble of two-level systems, with strong inhomogeneous broadening and coupled to a cavity mode whose frequency has linear time-dependence. The analysis shows that, regardless the distribution of energy level…

介观与纳米尺度物理 · 物理学 2019-09-25 C. Sun , V. Y. Chernyak , A. Piryatinski , N. A. Sinitsyn

We study the emission from a molecular photonic cavity formed by two proximal photonic crystal defect cavities containing a small number (<3) of In(Ga)As quantum dots. Under strong excitation we observe photoluminescence from the bonding…

Plasmonic nanocavities enable access to the quantum properties of matter, but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role…

量子物理 · 物理学 2024-11-13 Angus Crookes , Ben Yuen , Angela Demetriadou

Silicon is vital to the computing industry due to the high quality of its native oxide and well-established doping technologies. Isotopic purification has enabled quantum coherence times on the order of seconds, thereby placing silicon at…

介观与纳米尺度物理 · 物理学 2017-03-10 X. Mi , J. V. Cady , D. M. Zajac , P. W. Deelman , J. R. Petta

Using far field optical lithography, a single quantum dot is positioned within a pillar microcavity with a 50 nm accuracy. The lithography is performed in-situ at 10 K while measuring the quantum dot emission. Deterministic spectral and…

材料科学 · 物理学 2009-01-05 A. Dousse , L. Lanco , J. Suffczynski , E. Semenova , A. Miard , A. Lemaitre , I. Sagnes , C. Roblin , J. Bloch , P. Senellart

This chapter introduces cavity-based light-matter quantum interfaces, with a single atom or ion in strong coupling to a high-finesse optical cavity. We discuss the deterministic generation of indistinguishable single photons from these…

量子物理 · 物理学 2015-02-25 Axel Kuhn

Standard cavity cooling of atoms or dielectric particles is based on the action of dispersive optical forces in high-finesse cavities. We investigate here a complementary regime characterized by large cavity losses, resembling the standard…

量子物理 · 物理学 2024-08-21 Julian Lyne , Nico S. Bassler , Seong eun Park , Guido Pupillo , Claudiu Genes