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The interplay between exctions and vibrations is considered to be a key factor in determining the exciton transfer properties in light-harvesting exciton transfer complexes. Here we study this interplay theoretically in a model for exciton…

介观与纳米尺度物理 · 物理学 2018-05-25 Omer Goldberg , Yigal Meir , Yonatan Dubi

Vibrational energy transfer from photo-excited single-wall carbon nanotubes (SWCNTs) to coupled proteins is a key to engineer thermally induced biological reactions such as photothermal therapy. Here, we explored vibrational energy transfer…

The Davydov model of energy transfer in molecular chains is reconsidered assuming the distance dependence of the exciton hopping term. New equations of motion for phonons and excitons are derived within the coherent state approximation.…

凝聚态物理 · 物理学 2009-10-28 E. A. Bartnik , J. A. Tuszynski , D. Sept

Using methods of condensed matter and statistical physics, we examine the transport of excitons through the Fenna-Matthews-Olson (FMO) complex from a receiving antenna to a reaction center. Writing the equations of motion for the exciton…

生物物理 · 物理学 2016-02-23 Lev Mourokh , Franco Nori

Understanding how the effectiveness of natural photosynthetic energy harvesting systems arises from the interplay between quantum coherence and environmental noise represents a significant challenge for quantum theory. Recently it has begun…

生物物理 · 物理学 2015-06-16 E. K. Irish , R. Gómez-Bombarelli , B. W. Lovett

The transport of energy inside protein $\alpha$-helices is studied by deriving a system of quantum equations of motion from the Davydov Hamiltonian with the use of the Schr\"odinger equation and the generalized Ehrenfest theorem.…

软凝聚态物质 · 物理学 2018-11-26 Danko D. Georgiev , James F. Glazebrook

Vibrational heat transport in molecular junctions is a central issue in different contemporary research areas like Chemistry, material science, mechanical engineering, thermoelectrics and power generation. Our model system consists of a…

统计力学 · 物理学 2025-07-04 Jayasmita Behera , Malay Bandyopadhyay

The role of noise in the transport properties of quantum excitations is a topic of great importance in many fields, from organic semiconductors for technological applications to light-harvesting complexes in photosynthesis. In this paper we…

量子物理 · 物理学 2016-11-22 Stefano Iubini , Octavi Boada , Yasser Omar , Francesco Piazza

We study the electronic transport in a molecular junction in which each site is coupled to a local phonon bath using the non-equilibrium Green's function method. We observe the length period of the oscillatory conductance in odd-numbered…

强关联电子 · 物理学 2011-08-12 Ya-Lin Lo , Shih-Jye Sun , Ying-Jer Kao

Problems of heat transport are ubiquitous to various technologies such as power generation, cooling, electronics, and thermoelectrics. In this paper we advocate for the application of the quantum self-consistent reservoir method, which is…

介观与纳米尺度物理 · 物理学 2019-01-30 Roya Moghaddasi Fereidani , Dvira Segal

Dynamics of the Davydov's soliton in an external oscillating in time magnetic field is studied analytically. It is shown that in a field perpendicular to the molecular chain axis, soliton wavefunction is a product of the electron plane wave…

软凝聚态物质 · 物理学 2024-08-15 Larissa Brizhik

The influence of an external oscillating in time magnetic field on the dynamics of the Davydov's soliton is investigated. It is shown that it essentially depends not only on the amplitude and frequency of the magnetic field, but also on the…

软凝聚态物质 · 物理学 2024-02-15 Larissa Brizhik

The conversion of an absorbed photon from the exciton energy into the reaction centre in the photosynthetic complex has a near unit efficiency. It is becoming clear that any classical model, where the exciton hopping is modeled by a…

量子物理 · 物理学 2010-06-21 Vlatko Vedral , Tristan Farrow

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

量子物理 · 物理学 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

Heat dissipation is ubiquitous in living systems, which constantly convert distinct forms of energy into each other. The transport of thermal energy in liquids and even within proteins is well understood but kinetic energy transfer across a…

软凝聚态物质 · 物理学 2026-01-07 Brandon Neff , Matthias Heyden

Strong coupling between excitons and confined modes of light presents a promising pathway to tunable and enhanced energy transport in organic materials. By forming hybrid light-matter quasiparticles, exciton-polaritons, electronic…

化学物理 · 物理学 2024-11-01 Niclas Krupp , Gerrit Groenhof , Oriol Vendrell

Self-assembled supramolecular aggregates are excellent candidates for the design of efficient excitation transport devices. Both artificially prepared and natural photosynthetic aggregates in plants and bacteria present an important degree…

量子物理 · 物理学 2017-09-04 Alejandro D. Somoza , Ke-Wei Sun , Rafael A. Molina , Yang Zhao

Light-harvesting and excitation energy transfer in photosynthesis generally involve chlorophyll-molecules, maintained by their host proteins at short distances from each other, this resulting in excitonic coupling. The transfer of…

We consider the reduced dynamics of a molecular chain weakly coupled to a phonon bath. With a small and constant inhomogeneity in the coupling, the excitation relaxation rates are obtained in closed form. They are dominated by transitions…

统计力学 · 物理学 2021-04-16 B. A. Tay

A communication protocol is proposed in which quantum state transfer is mediated by a vibrational exciton. We consider two distant molecular groups grafted on the sides of a lattice. These groups behave as two quantum computers where the…

量子物理 · 物理学 2015-06-03 Vincent J. C. Pouthier
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