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The issue of the stability of Pickering emulsions is tackled at a mesoscopic level using dissipative particle dynamics simulations within the Adiabatic Biased Molecular Dynamics framework. We consider the early stage of the coalescence…

软凝聚态物质 · 物理学 2017-02-08 François Sicard , Alberto Striolo

The stability of shapes formed by three viscoelastic droplets during their arrested coalescence has been investigated using micromanipulation experiments. Addition of a third droplet to arrested droplet doublets is shown to be controlled by…

Combining high-speed photography with electric current measurement, we investigate the electrocoalescence of Pickering emulsion droplets. Under high enough electric field, the originally-stable droplets coalesce via two distinct approaches:…

软凝聚态物质 · 物理学 2013-03-01 Guo Chen , Peng Tan , Shuyu Chen , Jiping Huang , Weijia Wen , Lei Xu

We study the stability of a model Pickering emulsion system. A special counter-flow microfluidics set-up was used to prepare monodisperse Pickering emulsions, with oil droplets in water. The wettability of the monodisperse silica…

软凝聚态物质 · 物理学 2015-04-17 S. Fouilloux , A. Thill , J. Daillant , F. Malloggi

We present a quantitative confocal-microscopy study of the transient and final microstructure of particle-stabilised emulsions formed via demixing in a binary liquid. To this end, we have developed an image-analysis method that relies on…

软凝聚态物质 · 物理学 2010-11-04 Job H J Thijssen , Paul S Clegg

Drop coalescence is central to diverse processes involving dispersions of drops in industrial, engineering and scientific realms. During coalescence, two drops first touch and then merge as the liquid neck connecting them grows from…

Droplet coalescence is ubiquitous in nature and the same time key to various technologies, such as inkjet printing. Here, we report on the coalescence of polymer droplets with different chain lengths coalescing on substrates of different…

软凝聚态物质 · 物理学 2023-09-21 Soheil Arbabi , Panagiotis E. Theodorakis

A mixture of hard-sphere particles and model emulsion droplets is studied with a Brownian dynamics simulation. We find that the addition of nonwetting emulsion droplets to a suspension of pure hard spheres can lead to both gas-liquid and…

软凝聚态物质 · 物理学 2015-03-13 Andrea Fortini

The stable configurations formed by two viscoelastic, ellipsoid-shaped droplets during their arrested coalescence has been investigated using micromanipulation experiments. Ellipsoidal droplets are produced by millifluidic emulsification of…

软凝聚态物质 · 物理学 2018-08-14 Chen Hao , Zhaoyu Xie , Timothy J. Atherton , Patrick T. Spicer

Phase separation in passive systems leads to uncontrolled droplet growth, limiting structural control in soft materials and cells. We identify a generic mechanism to arrest coarsening based on chemical interconversion between molecular…

软凝聚态物质 · 物理学 2026-03-19 Florian Raßhofer , Erwin Frey

The dynamical perspectives of bubble in a liquid droplet on smooth solid substrate can be revealed by investigating interfacial self-assembly phenomena. Moreover, the complexity in such system can be scaled down into a transparent immobile…

软凝聚态物质 · 物理学 2018-11-19 Mayuri Bora , Sushant K. Behera , Pritam Deb

There is a large debate on the destabilization mechanism of emulsions. We present a simple technique using mechanical compression to destabilize oil-in-water emulsions. Upon compression of the emulsion, the continuous aqueous phase is…

The coalescence of droplets plays a crucial role in nature and modern technology. Various experimental and theoretical studies explored droplet dynamics in 3D and on 2D solid or liquid substrates. In this paper, we demonstrate the…

软凝聚态物质 · 物理学 2023-01-05 Christoph Klopp , Alexey Eremin

Drying a droplet of colloidal dispersion can result in complex pattern formation due to both development and deformation of a skin at the drop surface. The present study focus on the drying process of droplets of colloidal dispersions in a…

软凝聚态物质 · 物理学 2012-11-08 François Boulogne , Frédérique Giorgiutti-Dauphiné , Ludovic Pauchard

The coalescence of water drops on a substrate is studied experimentally. We focus on the rapid growth of the bridge connecting the two drops, which very quickly after contact ensues from a balance of surface tension and liquid inertia. For…

流体动力学 · 物理学 2013-07-30 A. Eddi , K. G. Winkels , J. H. Snoeijer

Particle-stabilized emulsions are commonly used in various industrial applications. These emulsions can present in different forms, such as Pickering emulsions or bijels, which can be distinguished by their different topologies and…

软凝聚态物质 · 物理学 2015-02-10 Stefan Frijters , Florian Günther , Jens Harting

The thermodynamic stability of emulsions of liquid crystal in water (glycerol) matrices is demonstrated for a wide range of materials and concentrations. Coalescence is prevented by an energy barrier for a topological ring defect formation…

mtrl-th · 物理学 2009-10-28 E. M. Terentjev

The breakup and coalescence of drops are elementary topological transitions in interfacial flows. The breakup of a drop changes dramatically when polymers are added to the fluid. With the strong elongation of the polymers during the…

流体动力学 · 物理学 2022-01-26 Pim J. Dekker , Michiel A. Hack , Walter Tewes , Charu Datt , Ambre Bouillant , Jacco H. Snoeijer

We investigate the 3D structure and drying dynamics of complex mixtures of emulsion droplets and colloidal particles, using confocal microscopy. Air invades and rapidly collapses large emulsion droplets, forcing their contents into the…

We consider an emulsion whose droplets contain a trapped species (insoluble in the continuous phase), and study the emulsion's stability against coarsening via Lifshitz-Slyozov dynamics (Ostwald Ripening). Extending an earlier treatment by…

软凝聚态物质 · 物理学 2007-05-23 A. J. Webster , M. E. Cates
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