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The high-quality structures containing semiconducting transition metal dichalcogenides (S-TMDs) monolayer (MLs) required for optical and electrical studies are achieved by their encapsulation in hexagonal BN (hBN) flakes. To examine the…

介观与纳米尺度物理 · 物理学 2023-08-14 A. O. Slobodeniuk , M. R. Molas

Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

Monolayers (MLs) of MoS2 and WSe2 are 2D semiconductors with strong, direct optical transitions that are governed by tightly Coulomb bound eletron-hole pairs (excitons). The optoelectronic properties of these transition metal…

材料科学 · 物理学 2015-03-06 G. Wang , X. Marie , I. Gerber , T. Amand , D. Lagarde , L. Bouet , M. Vidal , A. Balocchi , B. Urbaszek

We have experimentally determined the energies of the ground and first four excited excitonic states of the fundamental optical transition in monolayer WS2, a model system for the growing class of atomically thin two-dimensional…

We analyze the dielectric-function spectra of low dimensional transition metal dichalcogenides (TMDCs) using a fully analytical model of the complex dielectric function that is applicable in fractional dimensional space. We extract the…

材料科学 · 物理学 2018-12-04 A. Thilagam

We derive an analytical expression for $s$-state exciton energies in monolayer transition-metal dichalcogenides (TMDCs): $E_{\text{ns}}=-{\text{Ry}}^*\times P_n/{(n-1/2+0.479\, r^*_0/\kappa)^2}$, $n=1,2,...$, where $r^*_0$ and $\kappa$ are…

We report 65 tesla magneto-absorption spectroscopy of exciton Rydberg states in the archetypal monolayer semiconductor WSe$_2$. The strongly field-dependent and distinct energy shifts of the 2s, 3s, and 4s excited neutral excitons permits…

介观与纳米尺度物理 · 物理学 2018-02-07 Andreas V. Stier , Nathan P. Wilson , Kirill A. Velizhanin , Junichiro Kono , Xiaodong Xu , Scott A. Crooker

In semiconductor physics, many essential optoelectronic material parameters can be experimentally revealed via optical spectroscopy in sufficiently large magnetic fields. For monolayer transition-metal dichalcogenide semiconductors, this…

介观与纳米尺度物理 · 物理学 2020-08-20 M. Goryca , J. Li , A. V. Stier , T. Taniguchi , K. Watanabe , E. Courtade , S. Shree , C. Robert , B. Urbaszek , X. Marie , S. A. Crooker

We investigate excitonic transitions in a h-BN encapsulated monolayer $\textrm{MoS}_2$ phototransistor by photocurrent spectroscopy at cryogenic temperature (T = 5 K). The spectra presents excitonic peaks with linewidths as low as 8 meV,…

Exciton spectra of monolayer transition metal dichalcogenides (TMDs) in various dielectric environments are studied. The screened hydrogen model (SHM) [Phys. Rev. Lett. 116, 056401 (2016)] is examined by comparing its exciton spectra with…

介观与纳米尺度物理 · 物理学 2019-02-20 Jian-zhong Zhang , Jin-zhong Ma

We report the experimental observation of radiative recombination from Rydberg excitons in a two-dimensional semiconductor, monolayer WSe2, encapsulated in hexagonal boron nitride. Excitonic emission up to the 4s excited state is directly…

The results of magneto-optical spectroscopy investigations of excitons in a CVD grown monolayer of WSe2 encapsulated in hexagonal boron nitride are presented. The emission linewidth for the 1s state is of 4:7 meV, close to the narrowest…

介观与纳米尺度物理 · 物理学 2019-07-24 A. Delhomme , G. Butseraen , B. Zheng , L. Marty , V. Bouchiat , M. R. Molas , A. Pan , K. Watanabe , T. Taniguchi , A. Ouerghi , J. Renard , C. Faugeras

Reduced exciton mass, polarizability, and dielectric constant of the surrounding medium are essential properties for semiconducting materials, and they have been extracted recently from the magnetoexciton energies. However, the acceptable…

介观与纳米尺度物理 · 物理学 2023-05-24 Duy-Nhat Ly , Dai-Nam Le , Duy-Anh P. Nguyen , Ngoc-Tram D. Hoang , Ngoc-Hung Phan , Hoang-Minh L. Nguyen , Van-Hoang Le

The dielectric environment of atomically-thin monolayer (ML) of semiconducting transition metal dichalcogenides affects both the electronic band gap and the excitonic binding energy in the ML. We investigate the effect of the environment on…

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

介观与纳米尺度物理 · 物理学 2018-04-18 Roland Gillen , Janina Maultzsch

We present low temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field $B$ applied to monolayers of different semiconducting transition metal dichalcogenides. For…

介观与纳米尺度物理 · 物理学 2017-01-18 M. R. Molas , C. Faugeras , A. O. Slobodeniuk , K. Nogajewski , M. Bartos , D. M. Basko , M. Potemski

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

Rydberg excitons, the solid-state counterparts of Rydberg atoms, have sparked considerable interest in harnessing their quantum application potentials, whereas a major challenge is realizing their spatial confinement and manipulation.…

Two-dimensional (2D) heterostructures (HS) formed by transition-metal dichalcogenide (TMDC) monolayers offer a unique platform for the study of intralayer and interlayer excitons as well as moir\'e-pattern-induced features. Particularly,…

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