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We have performed polarized Raman scattering measurements on WTe$_2$, for which an extremely large positive magnetoresistance has been reported recently. We observe 5 A$_1$ phonon modes and 2 A$_2$ phonon modes out of 33 Raman active modes,…

材料科学 · 物理学 2015-02-27 W. -D. Kong , S. -F. Wu , P. Richard , C. -S. Lian , J. -T. Wang , C. -L. Yang , Y. -G. Shi , H. Ding

The vibrational structure of chromium germanium telluride (Cr$_2$Ge$_2$Te$_6$, CGT) is investigated and a strong spin-phonon coupling is revealed. The measured high-resolution Raman scattering (RS) spectra are composed of the 10…

We report a comprehensive investigation of the lattice dynamics of URu$_2$Si$_2$ as a function of temperature using Raman scattering, optical conductivity and inelastic neutron scattering measurements as well as theoretical {\it ab initio}…

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

强关联电子 · 物理学 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

强关联电子 · 物理学 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

The infrared (IR) active phonons in multiferroic TbMn$_2$O$_5$ are studied as a function of temperature. Most of the symmetry allowed IR modes polarized along the \textit{a} and \textit{b} crystal axes are observed and the behavior of…

材料科学 · 物理学 2007-10-23 R. Valdés Aguilar , A. B. Sushkov , S. Park , S-W. Cheong , H. D. Drew

Near normal incident far-infrared reflectivity spectra of [111] dysprosium titanate (Dy2Ti2O4) single crystal have been measured at different temperatures. Seven phonon modes (eight at low temperature) are identified at frequency below 1000…

材料科学 · 物理学 2009-11-11 C. Z. Bi , J. Y. Ma , B. R. Zhao , Z. Tang , D. Yin , C. Z. Li , D. Z. Yao , J. Shi , X. G. Qiu

We report on an extended fluctuation regime in the spin dimer system Sr3Cr2O8 based on anomalies in Raman active phonons and magnetic scattering. The compound has two characteristic temperatures, TS = 275 K, related to a Jahn-Teller…

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

材料科学 · 物理学 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

In this work, we investigate the local structural distortion of the double perovskite Ba$_2$YMoO$_6$ by means of infrared transmission spectroscopy. At 300 K, three bands are observed at $\sim$ 255.1 cm$^{-1}$, $\sim$ 343.4 cm$^{-1}$, and…

强关联电子 · 物理学 2013-04-05 Zhe Qu , Youming Zou , Shile Zhang , Langsheng Ling , Lei Zhang , Yuheng Zhang

We investigate the tunability of the structural, electronic and magneto transport properties of polycrystalline Sr2IrO4 sample. The extent of bifurcation of the magnetisation curves during the field cooled and zero field cooled cycles…

强关联电子 · 物理学 2022-09-07 Priyamedha Sharma , Saurabh Singh , Kentaro Kuga , Tsunehiro Takeuchi , R. Bindu

The doping and temperature dependent optical conductivity spectra of the quasi-two-dimensional Ca_{2-x}Sr_xRuO_4 (0.0=<x=<2.0) system were investigated. In the Mott insulating state, two electron correlation-induced peaks were observed…

强关联电子 · 物理学 2009-11-07 J. S. Lee , Y. S. Lee , T. W. Noh , S. -J. Oh , Jaejun Yu , S. Nakatsuji , H. Fukazawa , Y. Maeno

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

强关联电子 · 物理学 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

The intermediate valence (IV) compound YbAl$_3$ exhibits nonintegral valence (Yb 4$f^{14-n_f}$ (5d6s)$^z$ where z = 2+n$_f$ = 2.75) in a moderately heavy (m* = 20-30me) ground state with a large Kondo temperature (T$_K$ ~ 500-600K). We have…

Probing phonons, quasi-particle excitations and their coupling has enriched our understanding of these 2D materials and proved to be crucial for developing their potential applications. Here, we report comprehensive temperature, 4-330 K,…

材料科学 · 物理学 2022-03-14 Deepu Kumar , Vivek Kumar , Rahul Kumar , Mahesh Kumar , Pradeep Kumar

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

强关联电子 · 物理学 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

The strongly correlated insulator Ca$_{2}$RuO$_4$ is considered as a paradigmatic realization of both spin-orbital physics and a band-Mott insulating phase, characterized by orbitally selective coexistence of a band and a Mott gap. We…

We present a detailed temperature dependent Raman light scattering study of optical phonons in Ba{1-x}K{x}Fe{2}As{2} (x ~ 0.28, superconducting Tc ~ 29 K), Sr{1-x}K{x}Fe{2}As{2} (x ~ 0.15, Tc ~ 29 K) and non-superconducting BaFe{2}As{2}…

超导电性 · 物理学 2009-08-18 M. Rahlenbeck , G. L. Sun , D. L. Sun , C. T. Lin , B. Keimer , C. Ulrich

Clusters of single spins form the relevant spin entities in the formation of long-range magnetic order in spin cluster Mott insulators. Such type of spin order bears resemblance to molecular crystals, and we therefore may expect a…

强关联电子 · 物理学 2020-01-08 R. B. Versteeg , C. Boguschewski , P. Becker , P. H. M. van Loosdrecht

In this study, we propose that the signatures of spin fractionalization in quantum magnets can be identified through a detailed analysis of the temperature dependence of the asymmetric Fano lineshape of optical phonons overlapping with a…

强关联电子 · 物理学 2024-10-15 Swetlana Swarup , Susmita Singh , Natalia B. Perkins