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We report a comprehensive Raman study of the phonon behaviour in PdSe$_2$ in the temperature range of 5 K to 300 K. A remarkable change in the Raman spectrum is observed at 120 K: a significant enhancement of the out-of-plane phonon…

We report an infrared spectroscopy study of the antiferromagnetic (AFM) insulator EuZn$_2$As$_2$ over a broad frequency range, spanning temperatures both above and below the AFM transition $T_{\rm N} \simeq$ 20 K. The optical response…

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge…

The temperature dependence of phonon excitations and the presence of spin phonon coupling in polycrystalline Pr2NiMnO6 samples were studied using micro-Raman spectroscopy and magnetometry. Magnetic properties show a single…

材料科学 · 物理学 2011-01-17 K. D. Truong , M. P. Singh , S. Jandl , P. Fournier

Antiferromagnetic materials with strong spin-phonon coupling have the potential for spintronic applications. Here, we report the structural, magnetic, and vibrational properties of 12R-BaTi0.4Mn0.6O3. Temperature-dependent magnetization…

材料科学 · 物理学 2021-10-27 Bommareddy Poojitha , Anjali Rathore , Surajit Saha

We studied the optical properties of antiferromagnetic ZnCr2Se4 by infrared spectroscopy up to 28,000 cm-1 and for temperatures from 5 to 295 K. At the magnetic phase transition at 21 K, one of the four phonon modes reveals a clear…

强关联电子 · 物理学 2009-04-01 T. Rudolf , Ch. Kant , F. Mayr , M. Schmidt , V. Tsurkan , J. Deisenhofer , A. Loidl

Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J$_{eff}=1/2$ Mott insulating iridate Sr$_2$IrO$_4$. Comparisons are drawn between the correlated magnetism in this single…

Magneto Raman scattering study of the E$_{2g}$ optical phonons in multi-layer epitaxial graphene grown on a carbon face of SiC are presented. At 4.2K in magnetic field up to 33 T, we observe a series of well pronounced avoided crossings…

材料科学 · 物理学 2015-05-13 C. Faugeras , M. Amado , P. Kossacki , M. Orlita , M. Sprinkle , C. Berger , W. A. de Heer , M. Potemski

We utilize near-infrared femtosecond pulses to investigate coherent phonon oscillations of Ca2RuO4. The coherent Ag phonon mode of the lowest frequency changes abruptly not only its amplitude but also the oscillation-phase as the spin order…

强关联电子 · 物理学 2019-04-24 Min-Cheol Lee , Choong H. Kim , Inho Kwak , C. W. Seo , C. H. Sohn , F. Nakamura , C. Sow , Y. Maeno , E. -A. Kim , T. W. Noh , K. W. Kim

Polarized Raman scattering and infrared reflection spectra of hexagonal HoMnO$_3$ single crystals in the temperature range 10-300 K are reported. Group-theoretical analysis is performed and scattering selection rules for the second order…

强关联电子 · 物理学 2009-11-10 A. P. Litvinchuk , M. N. Iliev , V. N. Popov , M. M. Gospodinov

We report the evolution of the Raman active A_g phonon modes in the charge-ordered manganite Pr_{0.63}Ca_{0.37}MnO_{3} as a function of temperature from 300K to 25K. Our studies reveal that the linewidths of A_g(2) and A_g(4) phonons…

强关联电子 · 物理学 2009-11-07 Rajeev Gupta , G. Venketeswara Pai , A. K. Sood , T. V. Ramakrishnan , C. N. R. Rao

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

强关联电子 · 物理学 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

Polarized Raman-scattering spectra of non-superconducting, single-crystalline FeTe are investigated as function of temperature. We have found a relation between the magnitude of ordered magnetic moments and the linewidth of A1g phonons at…

We report plane-polarized Raman scattering spectra of iron oxypnictide superconductor NdFeAsO$_{1-x}$F$_x$ single crystals with varying fluorine $x$ content. The spectra exhibit sharp and symmetrical phonon lines with a weak dependence on…

超导电性 · 物理学 2009-11-13 Y. Gallais , A. Sacuto , M. Cazayous , P. Cheng , L. Fang , H. H. Wen

We report point-contact measurements of anisotropic magnetoresistance (AMR) in a single crystal of antiferromagnetic (AFM) Mott insulator Sr2IrO4. The point-contact technique is used here as a local probe of magnetotransport properties on…

介观与纳米尺度物理 · 物理学 2014-12-03 Cheng Wang , Heidi Seinige , Gang Cao , Jian-Shi Zhou , John B. Goodenough , Maxim Tsoi

Materials which possess coupling between different degrees of freedom such as charge, spin, orbital and lattice are of tremendous interest due to their potential for device applications. It has been recently realized that some of manganite…

材料科学 · 物理学 2021-10-27 Bommareddy Poojitha , Surajit Saha

Following previous works reporting an anomalous behavior of several zone-center optical phonons across the magnetic transition of square lattice iridates Sr2IrO4 and Sr3Ir2O7, we have investigated the lattice dynamics as a function of…

强关联电子 · 物理学 2022-02-02 K. Sen , R. Heid , S. M. Souliou , D. Boll , A. Bosak , N. H. Sung , J. Bertinshaw , H. Gretarsson , B. J. Kim , F. Weber , M. Le Tacon

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

材料科学 · 物理学 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Inelastic neutron scattering is used to measure the temperature dependent phonon dispersion in Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ ($x=0.4$, 0.6). The in-plane $\Sigma_{4}$ octahedral tilt mode softens significantly at the zone boundary of the high…

强关联电子 · 物理学 2015-05-13 R. G. Moore , M. D. Lumsden , M. B. Stone , Jiandi Zhang , Y. Chen , J. W. Lynn , R. Jin , D. Mandrus , E. W. Plummer

We employ polarization-resolved Raman spectroscopy and first-principles phonon calculations to study the lattice dynamics and spin-phonon coupling in the kagome spin ice compound HoAgGe. Upon cooling, HoAgGe shows transitions from a…

强关联电子 · 物理学 2025-03-11 Shangfei Wu , Lingxiao Zhao , Wei Song , Mingshu Tan , Feng Jin , Tianping Ying , Jia-Xin Yin , Qingming Zhang