相关论文: Imaging the Renner-Teller effect using laser-induc…
We propose a new approach, based on statistical mechanics, to predict the saturated state of a single-pass, high-gain free-electron laser (FEL). In analogy with the violent relaxation process in self-gravitating systems and in the Euler…
By analyzing ``exact'' theoretical results from solving the time-dependent Schr\"odinger equation of atoms in few-cycle laser pulses, we established the general conclusion that differential elastic scattering and photo-recombination cross…
The spectral and kinetic properties of intrinsic luminescence from (Y$_2$Sc$_1$)$_{0.(3)}$(Sc)[Si]O$_5$ crystal are studied. The emission is excited by electrons and gamma-quanta. The composition (Y$_2$Sc$_1$)$_{0.(3)}$(Sc)[Si]O$_5$ is the…
Broadband laser ultrasonics and two dimensional Fourier transformation are used to characterize the properties of varieties of foils and plates. Laser ultrasonics generation is achieved by use of a pulsed laser which deposits pulsed laser…
Two-dimensional electronic spectroscopy (2DES) provides rich information about how the electronic states of molecules, proteins, and solid-state materials interact with each other and their surrounding environment. Atomistic molecular…
The accurate calculation of excited state properties of interacting electrons in the condensed phase is an immense challenge in computational physics. Here, we use state-of-the-art equation-of-motion coupled-cluster theory with single and…
We have investigated the structural dynamics in photoexcited 1,2-diiodotetrafluoroethane molecules (C2F4I2) in the gas phase experimentally using ultrafast electron diffraction and theoretically using FOMO-CASCI excited state dynamics…
We present a theory for manipulation of d-wave interaction of cold atoms with two lasers strongly driving two photoassociative transitions. The theory predicts the occurrence of a coherence between two excited ro-vibrational bound states…
A barrier to realizing the potential of molecules for quantum information science applications is a lack of high-fidelity, single-molecule imaging techniques. Here, we present and theoretically analyze a general scheme for dispersive…
Machine learning (ML) has shown to advance the research field of quantum chemistry in almost any possible direction and has recently also entered the excited states to investigate the multifaceted photochemistry of molecules. In this paper,…
Using particle-in-cell simulations, we examine hot electron generation from electron plasma waves excited by stimulated Raman scattering and rescattering in the kinetic regime where the wavenumber times the Debye length (k\lambda_D) is…
In this article we analyze the Casimir-Polder interaction of atoms with a solid grating and an additional repulsive interaction between the atoms and the grating in the presence of an external laser source. The combined potential landscape…
Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…
We have performed X-ray two-photon photoelectron spectroscopy (XTPPS) using the Linac Coherent Light Source (LCLS) X-ray free-electron laser (FEL) in order to study double core-hole (DCH) states of CO2, N2O and N2. The experiment verifies…
Ladder-type two-photon excitation of an atom from a ground state $|g\rangle$, to an intermediate excited state $|e\rangle$, and, finally, to a Rydberg state $|r\rangle$, has a variety of uses from quantum information to sensing. A common…
Recent reviews in ultrafast electron diffraction (UED) have claimed that relativistic electrons exhibit enhanced elastic scattering efficiency, frequently quantified as a \gamma^2 increase in the differential cross section. These claims,…
Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray…
Transition metal dichalcogenide (TMD) materials have attracted substantial interest due to their remarkable excitonic, optical, electrical, and mechanical properties, which are highly dependent on their crystal structure. Controlling the…
The excitation of soft dipole modes in light nuclei via inelastic electron scattering is investigated. I show that, under the proposed conditions of the forthcoming electron-ion colliders, the scattering cross sections have a direct…
We study nonlinear optical effects in the laser excitation of Rydberg states. $5S_{1/2}$ and $5P_{3/2}$ levels of $^{85}$Rb are strongly coupled by a strong laser field and probed by a weak laser tuned to the $5P_{3/2} - 44D$ Rydberg…