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The recent accessibility of high quality, charge neutral monolayer transition metal dichalcogenides with narrow exciton linewidths at the homogeneous limit provides an ideal platform to study excitonic many-body interactions. In particular,…

The family of 2D layered semiconductors, including transition metal chalcogenides (TMCs) of the form MX (M=Ga, In; X=S, Se, Te) exhibit exceptional nonlinear optical properties. The energetically most favorable crystal ordering for…

材料科学 · 物理学 2024-10-10 Dmitry Skachkov , Dirk R. Englund , Michael N. Leuenberger

Nonlinear electromagnetic response functions have reemerged as a crucial tool for studying quantum materials. Most attention has been paid to responses to spatially uniform electric fields, relevant to optical experiments in conventional…

介观与纳米尺度物理 · 物理学 2024-03-28 Robert C. McKay , Fahad Mahmood , Barry Bradlyn

Higgs Effective Field Theory can be used to study vector-boson elastic scattering at the high energies relevant for the LHC. For most of the parameter space, the scattering is strongly interacting, with the minimal Standard Model being a…

高能物理 - 唯象学 · 物理学 2018-08-15 Rafael L. Delgado , Antonio Dobado , Felipe J. Llanes-Estrada

Nonlinear optical responses are becoming increasingly relevant for characterizing the symmetries and quantum geometry of electronic phases in materials. Here, we develop an expanded diagrammatic scheme for calculating spatially dispersive…

介观与纳米尺度物理 · 物理学 2023-08-16 Steven Gassner , Eugene J. Mele

Calculation of the coherent nonlinear response of a system is essential to correctly interpret results from advanced techniques such as two-dimensional coherent spectroscopy (2DCS). Usually, even for the simplest systems, such calculations…

光学 · 物理学 2025-09-03 Rishabh Tripathi , Krishna K. Maurya , Pradeep Kumar , Bhaskar De , Rohan Singh

We compare the optical absorption of extended systems using the density-density and current-current linear response functions calculated within many-body perturbation theory. The two approaches are formally equivalent for a finite momentum…

材料科学 · 物理学 2017-04-26 D. Sangalli , A. Berger , C. Attaccalite , M. Gruning , P. Romaniello

We present a computational study of static and dynamic linear polarizabilities in solution. We use different theoretical approaches to describe solvent effects, ranging from quantum mechanics/molecular mechanics (QM/MM) to quantum embedding…

化学物理 · 物理学 2022-12-07 Linda Goletto , Sara Gómez , Josefine H. Andersen , Henrik Koch , Tommaso Giovannini

The nonlinear optical behavior of quantum systems plays a crucial role in various photonic applications. This study introduces a novel framework for understanding these nonlinear effects by incorporating gauge-covariant formulations based…

综合物理 · 物理学 2025-03-11 Jingxu Wu , Chenjia Li

We present three schemes to go beyond the electric-dipole approximation in X-ray absorption spectroscopy calculations within a four-component relativistic framework. The first is based on the full semi-classical light-matter interaction…

化学物理 · 物理学 2021-07-02 Nanna Holmgaard List , Timothé Romain Léo Melin , Martin van Horn , Trond Saue

We present a comprehensive theoretical framework for calculating the linear and nonlinear optical responses of time-periodic quantum systems. Using density matrix evolution in the Floquet basis and adopting the length gauge, our approach…

材料科学 · 物理学 2025-03-10 S. Sajad Dabiri , Reza Asgari

Detecting inhomogeneities in the electrical conductivity is a special case of the inverse problem in electrical impedance tomography, that leads to fast direct reconstruction methods. One such method can, under reasonable assumptions,…

数值分析 · 数学 2018-08-16 Henrik Garde

We present a general method for incorporating the electromagnetic interaction into descriptions of hadronic processes based on four-dimensional scattering integral equations. The method involves the idea of gauging the scattering equations…

核理论 · 物理学 2009-10-30 A. N. Kvinikhidze , B. Blankleider

We present a new exciton-based formalism for calculating the coherent response of asymmetric semiconductor multiple quantum well structures to ultra-short optical pulses valid to infinite order in the optical field and including the…

介观与纳米尺度物理 · 物理学 2009-11-10 M. Hawton , M. M. Dignam

The linear response of an isolated, homogeneous granular fluid to small spatial perturbations is studied by methods of non-equilibrium statistical mechanics. The long wavelength linear hydrodynamic equations are obtained, with formally…

软凝聚态物质 · 物理学 2009-11-11 James Dufty , Aparna Baskaran , J. Javier Brey

We present a general formulation to calculate the dynamic optical conductivity, beyond the linear response regime, of any electronic system whose quasiparticle dispersion is described by a two band model. Our phenomenological model is based…

介观与纳米尺度物理 · 物理学 2017-04-19 Ashutosh Singh , Tuhina Satpati , Kirill I. Bolotin , Saikat Ghosh , Amit Agarwal

Excitonic effects in the linear optical response of semiconductors are well-known and the subject of countless experimental and theoretical studies. For the technologically important second order nonlinear response, however, description of…

强关联电子 · 物理学 2007-05-23 Thomas G. Pedersen , Horia D. Cornean

We present a general method based on nonlinear response theory to obtain effective interactions between ions in an electron gas which can also be applied to other systems where an adiabatic separation of time-scales is possible. Nonlinear…

材料科学 · 物理学 2007-10-05 Simon Gravel , N. W. Ashcroft

In this paper, we propose a gauge-invariant way to define and calculate the effective mass for quasiparticles in systems with gauge interactions, and apply it to a model closely related to the half-filled Landau level problem. Our model is…

介观与纳米尺度物理 · 物理学 2008-02-03 A. Raghav Chari , F. D. M. Haldane , Kun Yang

We solve the two-band model for the transport across a junction between a semimetal and an excitonic insulator. We analyze the current in terms of two competing terms associated with neutral excitons and charged carriers, respectively. We…

强关联电子 · 物理学 2007-05-23 Massimo Rontani , L. J. Sham