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Integrating 2D materials into high-quality optical microcavities opens the door to fascinating many-particle phenomena including the formation of exciton-polaritons. These are hybrid quasi-particles inheriting properties of both the…

介观与纳米尺度物理 · 物理学 2024-01-10 Beatriz Ferreira , Roberto Rosati , Jamie M. Fitzgerald , Ermin Malic

The photoluminescence (PL) and absorption experiments have been performed in GaSe slab with incident light polarized perpendicular to c-axis of sample at 10K. An obvious energy difference of about 34meV between exciton absorption peak and…

介观与纳米尺度物理 · 物理学 2016-03-08 Chengrong Wei , Xi Chen , Dian Li , Huimin Su , Jun-Feng Dai

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

We control the thickness of GaSe on the level of individual layers and study the corresponding optical absorption via highly sensitive differential transmission measurements. Suppression of excitonic transitions is observed when the number…

介观与纳米尺度物理 · 物理学 2019-07-17 Arne Budweg , Dinesh Yadav , Alexander Grupp , Alfred Leitenstorfer , Maxim Trushin , Fabian Pauly , Daniele Brida

We use linear response theory in order to compute the light absorption spectrum, in the terahertz band, of a polariton system composed by excitons in a quantum dot very strongly coupled to the lowest photon mode of a thin micropillar. In a…

介观与纳米尺度物理 · 物理学 2013-10-08 Carlos Andres Vera-Ciro , Alain Delgado , Augusto Gonzalez

We present first-principles calculations of the optical response of monolayer molybdenum disulfide employing the GW-Bethe Salpeter equation (GW-BSE) approach including self-energy, excitonic, and electron-phonon effects. We show that…

材料科学 · 物理学 2014-06-30 Diana Y. Qiu , Felipe H. da Jornada , Steven G. Louie

We measure the optical absorption spectra and optical conductivities of excitons and trions in monolayers of metal dichalcogenide MoS$_{2}$ and compare the results with theoretical models. Our results show that the Wannier-Mott model for…

介观与纳米尺度物理 · 物理学 2014-06-04 Changjian Zhang , Haining Wang , Weimin Chan , Christina Manolatou , Farhan Rana

To fully explore exciton-based applications and improve their performance, it is essential to understand the exciton behavior in anisotropic materials. Here, we investigate the optical properties of anisotropic excitons in GeS encapsulated…

Recent experimental measurements of light absorption in few-layer black phosphorus (BP) reveal a series of high and sharp peaks, interspersed by pairs of lower and broader features. Here, we propose a theoretical model for these excitonic…

介观与纳米尺度物理 · 物理学 2021-05-12 A. Chaves , G. O. Sousa , K. Khaliji , D. R. da Costa , G. A. Farias , Tony Low

Spatially structured light fields applied to semiconductor quantum dots yield fundamentally different absorption spectra than homogeneous beams. In this paper, we theoretically discuss the resulting spectra for different light beams using a…

介观与纳米尺度物理 · 物理学 2020-11-04 M. Holtkemper , G. F. Quinteiro , D. E. Reiter , T. Kuhn

We examine the absorption spectrum of electromagnetic radiation from excitons, where an exciton in the $1s$ state absorbs a photon and makes a transition to the $2p$ state. We demonstrate that the absorption spectrum depends strongly on the…

凝聚态物理 · 物理学 2009-10-31 K. Johnsen , G. M. Kavoulakis

Biased bilayer graphene, with its easily tunable band gap, presents itself as the ideal system to explore the excitonic effect in graphene based systems. In this paper we study the excitonic optical response of such a system by combining a…

介观与纳米尺度物理 · 物理学 2022-01-20 J. C. G. Henriques , Itai Epstein , N. M. R. Peres

We investigate the absorption and emission of a 25 nm ZnSe layer, which was grown on a GaAs buffer and cladded by ZnSSe layers. Due to the coupling of light with the exciton resonances, polariton modes propagate through the ZnSe layer.…

强关联电子 · 物理学 2008-06-02 M. Seemann , F. Kieseling , H. Stolz , M. Florian , G. Manzke , K. Henneberger , D. Hommel

We compare first-principle band gaps and optical absorption spectra of single- and double-layer fluorographene with bulk graphite fluoride. The electronic properties are calculated using the many-body GW approximation and the optical…

材料科学 · 物理学 2014-10-24 František Karlický , Michal Otyepka

The photoluminescence spectrum of a single-layer boron nitride remains elusive, marked by enigmatic satellites that hint at a significant but unidentified exciton-phonon coupling.Here, by employing a first principles approach based on the…

材料科学 · 物理学 2024-06-03 Giovanni Marini , Matteo Calandra , Pierluigi Cudazzo

Exciton-polaritons (EPs) arising from strong light-matter coupling offer new pathways for controlling optoelectronic properties. While typically requiring closed optical cavities for strong coupling, we demonstrate that 2D metal-organic…

光学 · 物理学 2025-12-11 Bongjun Choi , Adam D. Alfieri , Wangleong Chen , Deep Jariwala

The effect of a magnetic field on the optical absorption in semiconductors has been measured experimentally and modeled theoretically for various systems in previous decades. We present a new first-principles approach to systematically…

介观与纳米尺度物理 · 物理学 2020-06-03 Thorsten Deilmann , Peter Krüger , Michael Rohlfing

We discuss the linear and two-photon spectroscopic selection rules for spin-singlet excitons in monolayer transition-metal dichalcogenides. Our microscopic formalism combines a fully $k$-dependent few-orbital band structure with a many-body…

材料科学 · 物理学 2015-08-12 Timothy C. Berkelbach , Mark S. Hybertsen , David R. Reichman

Due to high binding energy and oscillator strength, excitons in thin flakes of transition metal dichalcogenides constitute a perfect foundation for realizing a strongly coupled light-matter system. In this paper we investigate mono- and…

The optical properties of particularly the tungsten-based transition-metal dichalcogenides are strongly influenced by the presence of dark excitons. Recently, theoretical predictions as well as indirect experimental insights have shown that…

介观与纳米尺度物理 · 物理学 2019-12-25 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman
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