相关论文: Efficient excitation of nonlinear phonons via chir…
The non-equilibrium dynamics of matter excited by light may produce electronic phases that do not exist in equilibrium, such as laser-induced high-transition-temperature superconductivity. Here we simulate the dynamics of a metal driven at…
We examine generation dynamics of coherent phonons (CPs) in both of polar and non-polar semiconductors -- such as GaAs and Si -- based on a polaronic-quasiparticle (PQ) model. In the model concerned, the PQ operator is composed of two kinds…
Information technology demands high-speed optoelectronic devices, but going beyond the one terahertz (THz) barrier is challenging due to the difficulties associated with generating, detecting, and processing high-frequency signals. Here, we…
We study the direct laser drive of infrared-active phonons that are quadratically coupled to a spinless fermion chain. Feedback is incorporated by phonon dressing of the electronic dispersion, which enables effective non-linearities in the…
To enhance the efficiency of next-generation ferroelectric (FE) electronic devices, new techniques for controlling ferroelectric polarization switching are required. While most prior studies have attempted to induce polarization switching…
Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…
Nonlinear phononics provides a powerful ultrafast route to control lattice excitations, enabling access to hidden quantum orders, phononic computing, and quantum transduction. However, dynamic control of anharmonic phonon interactions…
Ultrafast laser excitation provides a means to transiently realize long-range ordered electronic states of matter that are hidden in thermal equilibrium. Recently, this approach has unveiled a variety of thermally inaccessible ordered…
One route to the control of quantum magnetism at ultrafast timescales is magnetophononics, the modulation of magnetic interactions by coherently driven lattice excitations. Theoretical studies of a gapped quantum magnet subject to…
Recent terahertz-pump second-harmonic-generation(SHG)-probe measurements of quantum paraelectrics observed a significant long-lived non-oscillatory SHG component following an ultrafast resonant excitation of the soft mode, which was…
Absorbing airborne noise at frequencies below 300 Hz is a particularly vexing problem due to the absence of natural sound absorbing materials at these frequencies. The prevailing solution for low-frequency sound absorption is the use of…
Selective excitation of coherent high-amplitude vibrations of atoms in a solid can induce exotic nonequilibrium states, in which the character of interactions between electronic, magnetic and lattice degrees of freedom is considerably…
We present the results of pressure-dependent far-infrared reflectivity measurements on the multiferroic perovskite BiFeO3 at room temperature. The observed behavior of the infrared-active phonon modes as a funtion of pressure clearly…
Light has a wavelength that is usually longer than the size of the unit cell of crystals. Hence, even intense light pulses are not expected to break the translation symmetry of materials. However, certain materials, including KTaO$_3$,…
The element specificity of soft X-ray spectroscopy makes it an ideal tool for analyzing the microscopic origin of ultrafast dynamics induced by localized optical excitation in metal-insulator heterostructures. Using [Fe/MgO]$_n$ as a model…
Far and mid infrared optical pulses have been shown to induce non-equilibrium unconventional orders in complex materials, including photo-induced ferroelectricity in quantum paraelectrics, magnetic polarization in antiferromagnets and…
Understanding surface collective dynamics in quantum materials is crucial for advancing quantum technologies. For example, surface phonon modes in quantum paraelectrics are thought to play an essential role in facilitating interfacial…
We show that phononic frequency conversion can be enhanced by orders of magnitude in piezoelectric systems by heterogeneous integration of high-mobility semiconductor films. A lithium niobate and indium gallium arsenide heterostructure is…
The ultrafast switching of magnetization in multiferroic materials by a femtosecond laser could provide various advantages in photonics and magnonics. An efficient approach to control the light matter interaction is the modulation of…
A two-phonon system with lowest-order coupling of form $Q_RQ_{IR}^2$ is studied by perturbation method, and analytic results for both phonon displacements and frequencies are obtained. The frequency renormalization of infrared (IR) active…