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Manipulating the atomic and electronic structure of matter with strong terahertz (THz) fields while probing the response with ultrafast pulses at x-ray free electron lasers (FELs) has offered unique insights into a multitude of physical…

We investigate the vibrational and magnetic properties of thin layers of chromium tribromide (CrBr$_3$) with a thickness ranging from three to twenty layers (3~L to 20~L) revealed by the Raman scattering (RS) technique. Systematic…

The band structure of bilayer graphene is tunable by introducing a relative twist angle between the two layers, unlocking exotic phases, such as superconductor and Mott insulator, and providing a fertile ground for new physics. At…

介观与纳米尺度物理 · 物理学 2021-07-28 Matthew C. DeCapua , Yueh-Chun Wu , Takashi Taniguchi , Kenji Watanabe , Jun Yan

The equilibrium optical phonons of graphene are well characterized in terms of anharmonicity and electron-phonon interactions, however their non-equilibrium properties in the presence of hot charge carriers are still not fully explored.…

Terahertz driven magnetization dynamics are explored in the orthoferrite DyFeO3. A high-field, single cycle THz pulse is used to excite magnon modes in the crystal together with other resonances. Both quasi-ferromagnetic and…

材料科学 · 物理学 2017-06-07 A. H. M. Reid , Th. Rasing , R. V. Pisarev , H. A. Dürr , M. C. Hoffmann

A fundamental understanding of the interplay between lattice structure, polarization and electrons is pivotal to the optical control of ferroelectrics. The interaction between light and matter enables the remote and wireless control of the…

Optical rectification of ultrashort laser pulses in LiNbO3 by tilted-pulse-front excitation is a powerful way to generate near single-cycle terahertz (THz) pulses. Motivated by various applications, calculations were carried out to optimize…

Terahertz (THz) radiation is a powerful probe of low-energy excitations in all phases of matter. However, it remains a challenge to find materials that efficiently generate THz radiation in a broad range of frequencies following optical…

Polarized Raman, IR and time-domain THz spectroscopy of orthorhombic lead zirconate single crystals yielded a comprehensive picture of temperature-dependent quasiharmonic frequencies of its low-frequency phonon modes. It is argued that…

Optical resonances in nanostructures enable strong enhancement of nonlinear processes at the nanoscale, such as second-harmonic generation (SHG), with high-$Q$ modes providing intensified light--matter interactions and sharp spectral…

Terahertz near fields of gold metamaterials resonant at a frequency of $0.88\,\rm THz$ allow us to enter an extreme limit of non-perturbative ultrafast THz electronics: Fields reaching a ponderomotive energy in the keV range are exploited…

Electron-electron thermalization and electron-phonon relaxation processes in laser-excited solids are often assumed to occur on different timescales. This is true for the majority of the conduction band electrons in a metal. However,…

介观与纳米尺度物理 · 物理学 2019-06-05 Sebastian T. Weber , Baerbel Rethfeld

Ferroelectric control of interfacial magnetism has attracted much attention. However, the coupling of these two functionalities has not been understood well at the atomic scale. The lack of scientific progress is mainly due to the limited…

Light and matter can intertwine to create entirely new quantum states in the so-called strong-coupling regime, allowing unprecedented control over electromagnetic waves. In this work, strong-coupling mediated polaritonic states are…

The terahertz (THz) frequency range, bridging the gap between microwave and infrared frequencies, presents unparalleled opportunities for advanced imaging, sensing, communications, and spectroscopy applications. Terahertz photonics, in…

Noncontacting and nondestructive control of geometric phase in conventional semiconductors plays a pivotal role in various applications. In the current work, we present a theoretical and computational investigation on terahertz (THz)…

材料科学 · 物理学 2025-04-03 H. Cui , J. Zhou

We present, to the best of our knowledge, the highest average power from a laser-driven single-cycle THz source demonstrated so far, using optical rectification in the titled pulse-front geometry in cryogenically cooled lithium niobate,…

光学 · 物理学 2024-08-08 Tim Vogel , Samira Mansourzadeh , Clara Jody Saraceno

The three dimensional vibrations in a periodically poled ZX-cut Lithium Niobate thin bar with 0.3-mm long domains are considered. The acoustical vibrations may be excited by the 1) longitudinal acousto-electric current when a radio…

材料科学 · 物理学 2016-10-25 Igor Ostrovskii , Andriy Nadtochiy , Lucien Cremaldi

We investigate by near-forward Raman scattering a presumed reinforcement of the (A-C,B-C)-mixed phonon-polariton of a A1-xBxC zincblende alloy when entering its longitudinal optical (LO-)regime near the Brillouin zone centre {\Gamma}, as…

We demonstrate a table-top high-field terahertz (THz) source based on optical rectification of a collimated near-infrared pulse in gallium phosphide (GaP) to produce peak fields exceeding 300 kV/cm with a spectrum centered at 2.6 THz. The…