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We have performed a first-principles study of the structural and vibrational properties of the three low-pressure (cubic, tetragonal, and especially monoclinic) phases of ZrO2, with special attention to the computation of the zone-center…

材料科学 · 物理学 2009-11-07 Xinyuan Zhao , David Vanderbilt

We report a polarized Raman study of Weyl semimetal TaAs. We observe all the optical phonons, with energies and symmetries consistent with our first-principles calculations. We detect additional excitations assigned to multiple-phonon…

材料科学 · 物理学 2015-08-12 H. W. Liu , P. Richard , Z. D. Song , L. X. Zhao , Z. Fang , G. -F. Chen , H. Ding

We investigated microscopic lattice states in the donor-acceptor ionic Mott insulator, TTF-BA, by $^{79}$Br-NQR spectroscopy to explore cross-correlated fluctuations between spin, charge and lattice. A ferroelectric transition with lattice…

强关联电子 · 物理学 2021-08-11 Keishi Sunami , Tomohiro Baba , Kazuya Miyagawa , Sachio Horiuchi , Kazushi Kanoda

We observe intense pulses of far-infrared electromagnetic radiation emitted from arrays of InAs nanowires. The THz radiation power efficiency of these structures is about 15 times higher compared to a planar InAs substrate. This is…

Driving materials using light with more than one frequency component is an emerging technique, enabled by advanced pulse-shaping capabilities in recent years. Here, we translate this technique to lattice vibrations, by exciting multicolor…

材料科学 · 物理学 2025-04-07 Omer Yaniv , Dominik M. Juraschek

Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…

We experimentally determine the lattice dynamics of black phosphorus layered crystals through a combination of x-ray diffuse scattering and inelastic x-ray scattering, and we rationalize our experimental findings using $\textit{ab initio}$…

Magnetized charge-neutral graphene supports collective hybrid electronic excitations - polaritons - which have quantum origin. In contrast to polaritons in doped graphene, which arise from intraband electronic transitions, those in…

The piezoelectric (PZ) polarization effect enhances the phonon group velocity in wurtzite nitrides. This enhancement influences the phonon relaxation rates. We calculate the modified phonon relaxation rates in binary wurtzite nitrides (GaN,…

材料科学 · 物理学 2015-05-30 Bijay Kumar Sahoo

A key challenge in spintronics is to efficiently generate and manipulate spin current for information processing. Here we study ultrashort spin transport and associated terahertz (THz) emission in a hybrid structure comprising gold…

介观与纳米尺度物理 · 物理学 2025-05-26 H. Y. Yuan , Rembert A. Duine

Hybrid organic-inorganic halide perovskites have shown remarkable optoelectronic properties (1-3), believed to originate from correlated motion of charge carriers and the polar lattice forming large polarons (4-7). Few experimental…

Ultrafast optical excitations trigger in materials a range of dynamics. An interesting range of dynamics is the ones that unfold within the picosecond timescale, corresponding to the THz frequency range. Within this short timescale, the…

光学 · 物理学 2023-09-27 Yingshu Yang , Stefano Dal Forno , Marco Battiato

We use Raman-assisted tunneling in an optical superlattice to generate large tunable effective magnetic fields for ultracold atoms. When hopping in the lattice, the accumulated phase shift by an atom is equivalent to the Aharonov-Bohm phase…

In ferroelectric materials, an electric field has been shown to change the phonon dispersion sufficiently to alter the lattice thermal conductivity, opening the possibility that a heat gradient could drive a polarization flux, and…

材料科学 · 物理学 2025-01-08 Delaram Rashadfar , Brandi L. Wooten , Joseph P. Heremans

The unique optoelectronic properties of graphene [1] make it an ideal platform for a variety of photonic applications [2], including fast photodetectors [3], transparent electrodes [4], optical modulators [5], and ultra-fast lasers [6].…

介观与纳米尺度物理 · 物理学 2012-10-02 L. Vicarelli , M. S. Vitiello , D. Coquillat , A. Lombardo , A. C. Ferrari , W. Knap , M. Polini , V. Pellegrini , A. Tredicucci

Despite extensive research interests in perovskite oxides, low energy consumption, non-destructive and maneuverable methods for phase transition in perovskite oxides are still the under its exploration, and the underlying mechanisms remain…

材料科学 · 物理学 2023-08-10 Cong Zhou , Jian Zhou

Using femtosecond laser machining, we have fabricated photonic bandgap materials that influence propagation of phonon-polaritons in ferroelectric crystals. Broadband polaritons were generated with impulsive stimulated Raman scattering…

光学 · 物理学 2007-05-23 David W. Ward , Eric R. Statz , Thomas Feurer , Keith A. Nelson

We study the enhancement of third harmonic generation in indium tin oxide nanolayers coupled to Tamm plasmon polaritons (TPPs). The TPPs are excited at the interface between a thin gold mirror and a silicon dioxide/silicon nitride…

光学 · 物理学 2025-02-03 Tornike Shubitidze , Smridhi Chawla , Luca Dal Negro

High-quality microresonators can greatly enhance light-matter interactions and are excellent platforms for studying nonlinear optics. Wavelength conversion through nonlinear processes is the key to many applications of integrated optics.…

光学 · 物理学 2024-06-27 Yuxuan He , Xiongshuo Yan , Jiangwei Wu , Xiangmin Liu , Yuping Chen , Xianfeng Chen

THz pulses are generated from femtosecond pulse-excited ferromagnetic/nonmagnetic spintronic heterostructures via inverse spin Hall effect. The contribution from ultrafast demagnetization/remagnetization is extremely weak, in the…

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