相关论文: Experimentally Exploring the Interatomic Potential…
In stimulated Raman scattering, two incident optical waves induce a force oscillating at the difference of the two light frequencies. This process has enabled important applications such as the excitation and coherent control of phonons and…
Coherent manipulation of magnetism through the lattice provides unprecedented opportunities for controlling spintronic functionalities on the ultrafast timescale. Such nonthermal control conventionally involves nonlinear excitation of…
To date, two types of coupling between electromagnetic radiation and a crystal lattice have been identified experimentally. One is direct, for infrared (IR)-active vibrations that carry an electric dipole. The second is indirect, it occurs…
We simulate propagation of phonon-polaritons (admixtures of polar lattice vibrations and electromagnetic waves) in ferroelectric LiNbO3 with a model that consists of a spatially periodic array of harmonic oscillators coupled to THz…
Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…
Free-space super-strong terahertz (THz) electromagnetic fields offer multifaceted capabilities for reaching extreme nonlinear THz optics, accelerating and manipulating charged particles, and realizing other fascinating applications.…
We investigate the out-of-equilibrium lattice dynamics in the spin-ladder system $\alpha'$-NaV$_2$O$_5$ using intense terahertz (THz) pump and near-infrared (NIR) probe spectroscopy. When quasi-single-cycle THz pulses interact with…
Important advances have recently been made in the search for materials with complex multi-phase landscapes that host photoinduced metastable collective states with exotic functionalities. In almost all cases so far, the desired phases are…
Lead halide perovskites (LHPs) have emerged as an excellent class of semiconductors for next-generation solar cells and optoelectronic devices. Tailoring physical properties by fine-tuning the lattice structures has been explored in these…
The toroidal dipole excitation is an important field for metamaterial research because of their low-loss attribute. In this study, we demonstrate numerically and experimentally, a unique polarization independent terahertz metamaterial that…
Hybrid lattice-light modes, known as phonon-polaritons, represent the backbone of advanced protocols based on THz pumping of infrared modes. Here we provide a theoretical framework able to capture the different roles played by…
Using time resolved ultrafast spectroscopy, we have demonstrated that the far infrared (FIR) excitations in ferroelectric crystals may be modified through an arsenal of control techniques from the fields of guided waves, geometrical and…
The interaction of a single-cycle THz electric field with the topological insulator $\mathrm{MnBi}_2\mathrm{Te}_4$ triggers strongly anharmonic lattice dynamics, promoting fully coherent energy transfer between the otherwise non-interacting…
We use the frozen phonon method to calculate the anharmonic potential energy surface and to model the ultrafast ferroelectric polarization reversal in LiNbO3 driven by intense pulses of THz light. Before stable switching of the polarization…
A Terahertz (THz) laser with strong strength could excite more than one phonons and induce a transient lattice distortion termed as nonlinear phononics. This process allows dynamic control of various physical properties, including…
Ionic conduction in solids that exceeds 1 mS/cm is predicted to involve coupled phonon-ion interactions in the crystal lattice. Here, we use theory and experiment to measure the possible contribution of coupled phonon-ion hopping modes…
Strain engineering has been extended recently to the ultrafast timescales, driving metal-insulator phase transitions and the propagation of ultrasonic demagnetization fronts. However, the non-linear lattice dynamics underpinning interfacial…
Achieving parametric excitation in an oscillating physical system involves periodically adjusting one of its parameters to modulate the oscillator's natural frequency. This phenomenon has been observed in numerous systems within physics and…
Polaritons in metals, semimetals, semiconductors, and polar insulators, with their extreme confinement of electromagnetic energy, provide many promising opportunities for enhancing typically weak light-matter interactions such as multipolar…
Driving coherent lattice motion with THz pulses has emerged as a novel pathway for achieving dynamic stabilization of exotic phases that are inaccessible in equilibrium quantum materials. In this work, we present a previously unexplored…