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Monolayers of transition metal dichalcogenides (TMDs) have recently emerged as a promising optoelectronic platform. To leverage their full potential, however, it is important to understand and engineer the properties of the different…

The spectral and spatiotemporal dynamics of photoluminescence in monolayers of transition metal dichalcogenide WSe$_2$ obtained by mechanical exfoliation on a Si/SiO$_2$ substrate is studied over a wide range of temperatures and excitation…

介观与纳米尺度物理 · 物理学 2021-02-03 M. A. Akmaev , M. V. Kochiev , A. I. Duleba , M. V. Pugachev , A. Yu. Kuntsevich , V. V. Belykh

We present the first measurements of the electroluminescence response to the emission of single electrons in a two-phase noble gas detector. Single ionization electrons generated in liquid xenon are detected in a thin gas layer during the…

We have combined spatially-resolved steady-state micro-photoluminescence ($\mu$PL) with time-resolved photoluminescence (TRPL) to investigate the exciton diffusion in a WSe$_2$ monolayer encapsulated with hexagonal boron nitride (hBN). At…

介观与纳米尺度物理 · 物理学 2018-05-09 F. Cadiz , C. Robert , E. Courtade , M. Manca , L. Martinelli , T. Taniguchi , K. Watanabe , T. Amand , A. C. H. Rowe , D. Paget , B. Urbaszek , X. Marie

Measurements of double photoelectron emission (DPE) probabilities as a function of wavelength are reported for Hamamatsu R8778, R8520, and R11410 VUV-sensitive photomultiplier tubes (PMTs). In DPE, a single photon strikes the PMT…

仪器与探测器 · 物理学 2015-09-30 C. H. Faham , V. M. Gehman , A. Currie , A. Dobi , P. Sorensen , R. J. Gaitskell

Monolayer transition metal dichalcogenides offer the possibility of optical control of the valley degree of freedom. In order to asses the potential of these materials in applications, detailed knowledge of the valley dynamics is essential.…

介观与纳米尺度物理 · 物理学 2015-07-03 A. A. Mitioglu , L. Klopotowski , D. K. Maude , G. Deligeorgis , S. Anghel , L. Kulyuk , P. Plochocka

Single layers of WS2 are direct gap semiconductors with high photoluminescence (PL) yield holding great promise for emerging applications in optoelectronics. The spatial confinement in a 2D monolayer together with the weak dielectric…

介观与纳米尺度物理 · 物理学 2017-05-09 I. Paradisanos , S. Germanis , N. T. Pelekanos , C. Fotakis , E. Kymakis , G. Kioseoglou , E. Stratakis

We studied multi-exciton dynamics in monolayer WSe2 using nonlinear photoluminescence (PL) spectroscopy and Monte Carlo simulations. We observed strong nonlinear saturation behavior of exciton PL with increasing excitation power density,…

介观与纳米尺度物理 · 物理学 2014-11-05 Shinichiro Mouri , Yuhei Miyauchi , Minglin Toh , Weijie Zhao , Goki Eda , Kazunari Matsuda

Optical interband transitions in monolayer transition metal dichalcogenides such as WSe2 and MoS2 are governed by chiral selection rules. This allows efficient optical initialization of an electron in a specific K-valley in momentum space.…

介观与纳米尺度物理 · 物理学 2014-09-09 G. Wang , L. Bouet , D. Lagarde , M. Vidal , A. Balocchi , T. Amand , X. Marie , B. Urbaszek

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

材料科学 · 物理学 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

This letter reports a time resolved pump-probe reflectance spectroscopic study on moir\'e excitons in a twisted monolayer WS2/WSe2 heterostructure. By probing at the resonant energies of intralayer excitons, we observed their distinct…

介观与纳米尺度物理 · 物理学 2024-10-08 Feng Kai , Xiong Wang , Yiqin Xie , Yuhui Yang , Kenji Watanabe , Takashi Taniguchi , Hongyi Yu , Wang Yao , Xiaodong Cui

We explore the optical dipole orientation of single photon emitters in monolayer MoS2 as produced by a focused helium ion beam. The single photon emitters can be understood as single sulfur vacancies. The corresponding far-field…

In atomically thin two-dimensional semiconductors such as transition metal dichalcogenides (TMDs), controlling the density and type of defects promises to be an effective approach for engineering light-matter interactions. We demonstrate…

介观与纳米尺度物理 · 物理学 2018-08-15 Galan Moody , Kha Tran , Xiaobo Lu , Travis Autry , James M. Fraser , Richard P. Mirin , Li Yang , Xiaoqin Li , Kevin L. Silverman

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

材料科学 · 物理学 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

介观与纳米尺度物理 · 物理学 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

In the archetypal monolayer semiconductor WSe$_2$, the distinct ordering of spin-polarized valleys (low-energy pockets) in the conduction band allows for studies of not only simple neutral excitons and charged excitons (i.e., trions), but…

材料科学 · 物理学 2022-08-15 Dinh Van Tuan , Su-Fei Shi , Xiaodong Xu , Scott A. Crooker , Hanan Dery

Transition metal dichalcogenide (TMDC) heterostructures have unique properties that depend on the twisting angle and stacking order of two or more monolayers. However, their practical applications are limited by the low photoluminescence…

Unconventional emissions from exciton and trion in monolayer WS2 are studied by photoexcitation. Excited by 532nm laser beam, the carrier species in the monolayer WS2 are affected by the excess electrons escaping from photoionization of…

介观与纳米尺度物理 · 物理学 2016-08-08 Ke Wei , Yu Liu , Hang Yang , Xiangai Cheng , Tian Jiang

We present optical spectroscopy (photoluminescence and reflectance) studies of thin layers of the transition metal dichalcogenide WSe2, with thickness ranging from mono- to tetra-layer and in the bulk limit. The investigated spectra show…

介观与纳米尺度物理 · 物理学 2015-03-06 Ashish Arora , Maciej Koperski , Karol Nogajewski , Jacques Marcus , Clement Faugeras , Marek Potemski

Two-dimensional semiconductors exhibit pronounced many-body effects and intense optical responses due to strong coulombic interactions. Consequently, subtle differences in photoexcitation conditions can strongly influence how the material…