相关论文: Tuning nonradiative lifetimes via molecular aggreg…
We analyze the electric dipole moments (PDMs) and static electric dipole polarizabilities of the alkali--alkaline-earth (Alk-AlkE) dimers by employing finite-field coupled-cluster methods, both in the frameworks of non-relativistic and…
We calculate Coulomb scattering lifetimes of electrons in two-subband quantum wires and in double-layer quantum wells by obtaining the quasiparticle self-energy within the framework of the random-phase approximation for the dynamical…
We assess the accuracy of vibrational damping rates of diatomic adsorbates on metal surfaces as calculated within the local-density friction approximation (LDFA). An atoms-in-molecules (AIM) type charge partitioning scheme accounts for…
We study the impact of an environment on the electromagnetic responses of a molecule in the presence of a dielectric medium. By applying the dipole-dipole coupling between the molecule's and the environment's degrees of freedom, we can…
The quantum nonlinear dimer consisting of an electron shuttling between the two sites and in weak interaction with vibrations, is studied numerically under the application of a DC electric field. A field-induced resonance phenomenon between…
The behavior of levels near the threshold of the lower continuum in superheavy H-like atoms with $Z\alpha >1$, caused by the interaction $\Delta U_{AMM}$ of the electron's magnetic anomaly (AMM) dynamically screened at small distances $ \ll…
The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by…
Negative differential resistance - a decrease in current with increasing bias voltage - is a counter-intuitive effect that is observed in various molecular junctions. Here, we present a novel mechanism that may be responsible for such an…
The lifetime of interatomic Coulombic decay (ICD) [L. S. Cederbaum et al., Phys. Rev. Lett. 79, 4778 (1997)] in Ne_2 is determined via an extreme ultraviolet pump-probe experiment at the Free-Electron Laser in Hamburg. The pump pulse…
A new algorithm based on auxiliary differential equation and finite difference time domain method (ADE-FDTD method) is presented to model a waveguide whose active layer is constituted of a silica matrix doped with rare-earth and silicon…
Nanophotonics offers a promising range of applications spanning from the development of efficient solar cells to quantum communications and biosensing. However, the ability to efficiently couple fluorescent emitters with nanostructured…
A mixed quantum-classical approach to simulate the coupled dynamics of electrons and nuclei in nanoscale molecular systems is presented. The method relies on a second order expansion of the Lagrangian in time-dependent density functional…
The interaction of condensed phase systems with external electric fields is crucial in myriad processes in nature and technology ranging from the field-directed motion of cells (galvanotaxis), to energy storage and conversion systems…
Many soft-matter and biophysical systems are composed of monomers which reversibly assemble into rod-like aggregates. The aggregates can then order into liquid-crystal phases if the density is high enough, and liquid-crystal ordering…
Atoms coupled to the same environment interfere with each other to yield super- or sub-radiance. Specifically, atoms in subradiant states are promising candidates for long-lifetime qubits and quantum memory because of the immunity to the…
We investigate the effect of nonrelativistic motion on the emission dynamics of a dipole emitter moving next to a reflecting interface. Within the formalism of macroscopic QED, we obtain a general equation of motion for the dipole amplitude…
We develop a new nonrelativistic effective field theory of $\rho$NRQCD [1] to describe the finite lifetime effects in the threshold production of top quark-antiquark pairs. The theory is based on the expansion in a parameter…
The v = 1 -> 0 radiative lifetime of NH (X triplet-Sigma-, v=1,N=0) is determined to be tau_rad,exp. = 37.0 +/- 0.5 stat +2.0 / -0.8 sys miliseconds, corresponding to a transition dipole moment of |mu_10| = 0.0540 + 0.0009 / -0.0018 Debye.…
Effects of various nuclear interaction potentials on the decay lifetimes and the turning points of the WKB action integral has been studied. The microscopic nuclear potential obtained by folding in the density distribution functions of the…
We study the role of static and dynamical Coulomb correlation effects on the electronic and magnetic properties of individual Mn, Fe and Co adatoms deposited on the CuN surface. For these purposes, we construct a realistic Anderson model,…