相关论文: Electronic ground state of Ni$_2^+$

The translational motion of molecular ions can be effectively cooled sympathetically to translational temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The ro-vibrational degrees of freedom,…

To determine the state of spin polarization of the 3D electron gas at very low densities and zero temperature, we calculate the energy versus spin polarization using Diffusion Quantum Monte Carlo methods with backflow wavefunctions and…

The magnetic ground state is crucial for the applications of the two-dimension magnets as it decides fundamental magnetic properties of the material, such as magnetic order, magnetic transition temperature, and low-energy excitation of the…

The effect of Ir substitution for Os in CeOs2Al10, with an unusually high Neel temperature of T~28.5K, has been studied by high-resolution neutron diffraction and magnetization measurements. A small amount of Ir (~ 8%) results in a…

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

We used a solid-state reaction method to prepare Sn$_{1-x}$Ni$_x$O$_2$ with $x$ = 0, 0.05, 0.1, 0.15 polycrystalline compounds. A rutile phase with tetragonal crystal structure was confirmed by X-ray diffraction. At room temperature, the…

We theoretically investigate the ground state spin of a polynuclear transition-metal complex as a function of the number of added electrons taking into account strong electron correlations. Our phenomenological model of the so-called…

The low temperature properties of the Kagome-type system Co3V2O8 have been studied by powder neutron diffraction both in zero field and in applied magnetic field of up to 8 T. Below 6 K, the zero-field ground state is ferromagnetic with the…

The $\mathrm{X}^+\ ^2\Sigma_u^+$ ground electronic state of the Mg$_2^+$ ion has been studied by pulsed-field-ionization zero-kinetic-energy (PFI-ZEKE) photoelectron spectroscopy. Rotationally cold Mg$_2$ molecules produced in a…

Recent neutron diffraction and NMR studies suggest that the incommensurately modulated spin cycloid structure of BiFeO3 is stable down to 4.2 K, whereas DC [M(T)] and AC [\c{hi} ({\omega}, T)] magnetization, and caloric studies have…

The electronic and magnetic properties of neutral substitutional transition-metal dopants in dia- mond are calculated within density functional theory using the generalized gradient approximation to the exchange-correlation potential. Ti…

Muon spin rotation/relaxation spectroscopy %(supported by magnetization measurements) has been employed to study electron localization around a donor center - the positive muon - in the 3d magnetic spinel semiconductor CdCr$_2$Se$_4$ at…

We identify a solid-state quantum emitter whose room-temperature radiative decay is mediated by a nearly equal mixture of isotropic electric dipole (ED) and magnetic dipole (MD) transitions. Using energy-momentum spectroscopy, we…

4$d$ transition metal oxide (TMO) offers an intriguing puzzle for their electronic and magnetic ground state. They are in the cross-over regime of strong spin orbit interaction (SOI) and electron-electron correlation ($U$) with quenched…

We study the magnetic susceptibility of mixed-valent La2-xSrxCoO4 single crystals in the doping range of 0.5<= x <= 0.8 for temperatures up to 1000 K. The magnetism below room temperature is described by paramagnetic Co2+ in the high-spin…

We present theoretical evidence, based on total-energy first-principles calculations, of the existence of spin-polarized states well localized at and extended along the edges of bare zigzag boron nitride nanoribbons. Our calculations…

We evaluate the charge and longitudinal spin response functions of a two-dimensional electron gas with $e^2/r$ interactions in an arbitrary state of spin polarization, using a structurally self-consistent approach to treat exchange and…

We show that the low-temperature physics of molecular nanomagnets, contrary to the prevailing one-molecule picture, must be determined by the long-range magnetic ordering due to many-body dipolar interactions. The calculations here…

The spin states at the surface of epitaxial thin films of hematite, both undoped and doped with 1% Ti, Sn or Zn, respectively, were probed with x-ray magnetic linear dichroism (XMLD) spectroscopy. Morin transitions were observed for the…

Dimers are the smallest chemical objects that show magnetic anisotropy. We focus on 3$d$ and 4$d$ transition metal dimers that have magnetic ground states in most cases. Some of these magnetic dimers have a considerable barrier against…