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Molecular dynamics simulations have been employed to study the formation of a physical (thermoreversible) gel by amphiphilic A-B-A triblock copolymers in aqueous solution. In order to mimic the structure of hydrogel-forming polypeptides…

软凝聚态物质 · 物理学 2007-05-23 Lei Guo , Erik Luijten

We model the mechanics of associating trivalent dendrimer network glasses with a focus on their energy dissipation properties. Various combinations of sticky bond (SB) strength and kinetics are employed. The toughness (work-to-fracture) of…

软凝聚态物质 · 物理学 2015-06-16 Arvind Srikanth , Robert S. Hoy , Berend C. Rinderspacher , Jan W. Andzelm

Hydrogen bonding plays a role in the microphase separation behavior of many block copolymers, such as those used in lithography, where the stronger interactions due to H-bonding can lead to a smaller period for the self-assembled…

软凝聚态物质 · 物理学 2018-05-28 E. Patyukova , T. Rottreau , R. Evans , P. D. Topham , M. J. Greenall

Many biological systems can form strong adhesion to various materials with complex shapes. The adhesion is further switchable between strongly adhering and completely non-adhering in a simple and fast manner. By contrast, no engineering…

软凝聚态物质 · 物理学 2025-03-11 Qianfeng Yin , Yilmaz Arin Manav , Yichen Wan , Benyamin Davaji , Ruobing Bai

The influence of structural constraints on the relaxation dynamics of three polyurea networks with varying degree of crosslinking, has been studied by means of a thorough analysis of broadband dielectric spectroscopy measurements. Two…

软凝聚态物质 · 物理学 2018-10-03 Nerea Sebastián , Christophe Contal , Antoni Sánchez-Ferrer , Marco Pieruccini

Reconfigurable metamaterials require constituent nanostructures to demonstrate switching of shapes with external stimuli. For generality, such nanostructures would touch and stick to other surfaces in one of its configurations. Yet, a…

Soft materials possessing tunable rheological properties are desirable in applications ranging from 3D printing to biological scaffolds. Here, we use a telechelic, triblock copolymer polystyrene-b-poly(ethylene oxide)-b-polystyrene (SEOS)…

软凝聚态物质 · 物理学 2023-05-05 Daniel P. Keane , Colby J. Constantine , Matthew D. Mellor , Ryan Poling-Skutvik

Various adhesion mechanisms that have been understood in the field of synthetic adhesives are described and these are linked with situations relevant to fouling issues. The review mainly deals with mechanical aspects of adhesion phenomena,…

软凝聚态物质 · 物理学 2016-04-13 Cyprien Gay

In this study we have investigated into the entanglement effect and crosslinking effect in long-chain SBR rubber polymer system to model the mechanical hyperelastic behavior. The discussed methodologies are developed by a dissipative…

材料科学 · 物理学 2021-03-24 Shashank Mishra , Soumyadipta Maiti , Prashant Pandey , Beena Rai

The wide adoption of thermoplastic composites to reduce weight in structural parts requires reliable numerical methods to account for debonding between overmolded parts. Although cohesive elements are effective for debonding, the need for…

计算工程、金融与科学 · 计算机科学 2026-03-31 Sérgio G. F. Cordeiro , Boyang Chen , Frans P. van der Meer

Using typical experimental techniques it is difficult to separate the effects of carrier density and disorder on the superconducting transition in two dimensions. Using a simple fabrication procedure based on metal layer dewetting, we have…

介观与纳米尺度物理 · 物理学 2012-07-03 B. M. Kessler , C. O. Girit , A. Zettl , V. Bouchiat

Polymer melts with chains undergoing reversible crosslinking have distinctively favorable dynamic properties, e.g., self healing and reprocessability. In these situations there are two relevant elementary time scales: the segmental and the…

软凝聚态物质 · 物理学 2025-03-14 Rahul Karmakar , Srikanth Sastry , Sanat K. Kumar , Tarak K. Patra

Enormous enhancement in the viscosity of a liquid near its glass transition is generally connected to the growing many-body static correlations near the transition, often coined as `amorphous ordering'. Estimating the length scales of such…

Using a coarse-grained bead-spring model for semi-flexible macromolecules forming a polymer brush, structure and dynamics of the polymers is investigated, varying chain stiffness and grafting density. The anchoring condition for the grafted…

软凝聚态物质 · 物理学 2014-01-28 Andrey Milchev , Kurt Binder

In addition to the ubiquitous structural relaxation of viscous supercooled liquids, monohydroxy alcohols and several other hydrogen-bonded systems display a strong single-exponential electrical low-frequency absorption. So far, this…

软凝聚态物质 · 物理学 2014-09-23 C. Gainaru , R. Figuli , T. Hecksher , B. Jakobsen , J. C. Dyre , M. Wilhelm , R. Böhmer

The universality of the swelling of the radius of gyration of a homopolymer relative to its value in the $\theta$ state, independent of polymer-solvent chemistry, in the crossover regime between $\theta$ and athermal solvent conditions, is…

软凝聚态物质 · 物理学 2020-07-03 Aritra Santra , Kiran Kumari , R. Padinhateeri , B. Duenweg , J. Ravi Prakash

We use numerical simulations to show how noninteracting hard particles binding to a deformable elastic shell may self-assemble into a variety of linear patterns. This is a result of the nontrivial elastic response to deformations of shells.…

软凝聚态物质 · 物理学 2011-02-25 Andela Šarić , Angelo Cacciuto

Surface confined dehalogenation reactions are versatile bottom-up approaches for the synthesis of carbon-based nanostructures with predefined chemical properties. However, for devices generally requiring low conductivity substrates,…

We study the bending rigidity of highly charged stiff polyelectrolytes, for both a single chain and many chains forming a bundle. A theory is developed to account for the interplay between competitive binding of counterions and charge…

软凝聚态物质 · 物理学 2009-11-07 Bae-Yeun Ha , D. Thirumalai

We investigate the static and dynamic properties of dendrimers diffusing through a network of linear associative polymers using coarse-grained Brownian dynamics simulations. Both dendrimers and network chains are modelled as bead-spring…

软凝聚态物质 · 物理学 2025-11-26 Silpa Mariya , Jeremy J. Barr , P. Sunthar , J. Ravi Prakash