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We connect the configurational entropy of a liquid to the geometrical properties of its local energy landscape, using a high-temperature expansion. It is proposed that correlations between local structures arises from their overlap and,…

软凝聚态物质 · 物理学 2016-08-24 Pierre Ronceray , Peter Harrowell

We discuss the applicability of the pseudopotential-like self-interaction correction (pSIC) to the study of defect energetics and electronic structure of In2O3. Our results predict that substitutional (at oxygen sites) and interstitial (at…

材料科学 · 物理学 2016-06-24 Juan J. Meléndez , Małgorzata Wierzbowska

Structure prediction has become a key task of the modern atomistic sciences, and depends on the rapid and reliable computation of the energy landscape. First principles density functional based calculations are highly reliable, faithfully…

材料科学 · 物理学 2022-07-08 Chris J. Pickard

In this paper, density functional theory calculations are used to explore the electronic and atomic reconstruction at interfaces between III-III/I-V oxides. In particular, at these interfaces, two dimensional electron gases (2DEGs) with…

材料科学 · 物理学 2012-06-06 Valentino R. Cooper

Formulating a statistical mechanics for granular matter remains a significant challenge, in part, due to the difficulty associated with a complete characterization of the systems under study. We present a fully characterized model of a…

软凝聚态物质 · 物理学 2015-05-27 Richard K. Bowles , S. S. Ashwin

An atomistic effective Hamiltonian technique is used to investigate the finite-temperature energy storage properties of a ferroelectric nanocomposite consisting of an array of BaTiO$_{3}$ nanowires embedded in a SrTiO$_{3}$ matrix, for…

Various experimental techniques, have revealed that the predominant intrinsic point defects in BaF$_2$ are anion Frenkel defects. Their formation enthalpy and entropy as well as the corresponding parameters for the fluorine vacancy and…

材料科学 · 物理学 2017-04-11 Vassiliki Katsika-Tsigourakou , Efthimios S. Skordas

Density functional theory (DFT) is the de facto approach for predicting self-consistent-field electronic structures of ground-state configurations of complex atoms, molecules, and solids and providing their property data for materials…

材料科学 · 物理学 2024-01-30 Zi-Kui Liu

Motivated by gauge/gravity group in the low energy effective theory of the heterotic string theory and novel aspects of massive gravity in the context of lattice physics, the minimal coupling of Gauss-Bonnet-massive gravity with Born-Infeld…

高能物理 - 理论 · 物理学 2017-01-19 S. H. Hendi , B. Eslam Panah , S. Panahiyan

Firstly, we calculate quantitatively decrease of entropy by the known formulas in the ordering phenomena and nucleation of thermodynamics of microstructure. They show again that a necessary condition of decrease of entropy in isolated…

综合物理 · 物理学 2009-05-04 Yi-Fang Chang

Understanding the properties of Au$_{10}$ clusters entails identifying the lowest energy structure at cold and warm temperatures. While functional materials operate at finite temperatures, energy computations using density functional theory…

Density functional theory is used to explore the possibility of inducing impurity band ferromagnetism in monolayers of semiconducting MoS2 by introducing holes into the narrow Mo 4d band that forms the top of the valence band. A large out…

材料科学 · 物理学 2019-06-26 Yuqiang Gao , Nirmal Ganguli , Paul J. Kelly

Defects determine many important properties and applications of materials, ranging from doping in semiconductors, to conductivity in mixed ionic-electronic conductors used in batteries, to active sites in catalysts. The theoretical…

材料科学 · 物理学 2024-04-17 Irea Mosquera-Lois , Seán R. Kavanagh , Johan Klarbring , Kasper Tolborg , Aron Walsh

The nature of defects in amorphous materials, analogous to vacancies and dislocations in crystals, remains elusive. Here we explore their nature in a three-dimensional microscopic model glass-former which describes granular, colloidal,…

软凝聚态物质 · 物理学 2019-11-13 Camille Scalliet , Ludovic Berthier , Francesco Zamponi

The structural, electronic, mechanical and thermal properties of Ir$_{1-x}$Rh$_{x}$ alloys were studied systematically using ab initio density functional theory at different concentrations (x = 0.00, 0.25, 0.50, 0.75, 1.00). A Special…

材料科学 · 物理学 2015-06-15 S. Ahmed , M. Zafar , M. Shakil , M. A. Choudhary

Defects in the atomic lattice of solids are sometimes desired. For example, atomic vacancies, single ones or more elaborated defective structures, can generate localized magnetic moments in a non magnetic crystalline lattice. Increasing…

超导电性 · 物理学 2019-02-21 Pablo D. Esquinazi

While the effect of intrinsic defects on the electronic properties of half-Heusler compounds has been extensively discussed in literature, their effect on the lattice vibrations has received much less attention, due to the prohibitive…

材料科学 · 物理学 2024-12-17 M. Yazdani-Kachoei , B. Rabihavi , I. E. Brumboiu , S. Mehdi Vaez Allaei , I. Di Marco

A number of diverse bulk properties of the zincblende and wurtzite III-V nitrides AlN, GaN, and InN, are predicted from first principles within density functional theory using the plane-wave ultrasoft pseudopotential method, within both the…

材料科学 · 物理学 2009-10-31 A. Zoroddu , F. Bernardini , P. Ruggerone , V. Fiorentini

The pseudogap regime of high-temperature cuprates harbours diverse manifestations of electronic ordering whose exact nature and universality remain debated. Here, we show that the short-ranged charge order recently reported in the normal…

超导电性 · 物理学 2015-03-10 T. Wu , H. Mayaffre , S. Krämer , M. Horvatić , C. Berthier , W. N. Hardy , R. Liang , D. A. Bonn , M. -H. Julien

The recent observations of ferromagnetic order in several two-dimensional (2D) materials have generated an enormous interest in the physical mechanisms underlying 2D magnetism. In the present prospective article we show that Density…

材料科学 · 物理学 2020-02-18 Thomas Olsen