相关论文: Do ultrafast exciton-polaron decoherence dynamics …
Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…
Organic solar cells are a promising avenue for renewable energy, and our study introduces a comprehensive model to investigate exciton dissociation processes at the donor-acceptor interface. Examining quantum efficiency and emitted phonons…
Two dimensional semiconductors provide an ideal platform for exploration of linear exciton and polariton physics, primarily due to large exciton binding energy and strong light-matter coupling. These features, however, generically imply…
A general problem arising in computer simulations is the number of material and device parameters, which have to be determined by dedicated experiments and simulation-based parameter extraction. In this study we analyze measurements of the…
We present quantitative ultrafast interferometric pump-probe microscopy capable of tracking of photoexcitations with sub 10 nm spatial precision in three dimensions with 15 fs temporal resolution, through retrieval of the full transient…
We measure the dynamics of a non-classical optical field using two-time second-order correlations in conjunction with pulsed excitation. The technique quantifies single-photon purity and coherence during the excitation-decay cycle of an…
Excitons in atomically-thin semiconductors interact very strongly with electromagnetic radiation and are necessarily close to a surface. Here, we exploit the deep-subwavelength confinement of surface plasmon polaritons (SPPs) at the edge of…
We study photocurrent of exciton polaritons in inversion broken systems. We use an effective Hamiltonian and Green's function approaches to deduce the formula for polariton photocurrent. The obtained formula shows the polariton photocurrent…
We report on a theoretical study on the rise of strong peaks at the harmonics of the cyclotron resonance in the irradiated magnetoresistance in ultraclean two-dimensional electron systems. The motivation is the experimental observation of a…
Photosystem II is crucial for life on Earth as it provides oxygen as a result of photoinduced electron transfer and water splitting reactions. The excited state dynamics of the photosystem II-reaction center (PSII-RC) has been a matter of…
Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…
The concept of modifying molecular dynamics in strongly coupled exciton-polariton systems is an emerging topic in photonics due to its potential to produce customized chemical systems with tailored photophysical properties. However, before…
Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…
There have been experimental and theoretical studies on Photoluminescence (PL) from possible exciton superfluid in semiconductor electron-hole bilayer systems. However, the PL contains no phase information and no photon correlations, so it…
A simple model is constructed to describe dissociation of charge transfer excitons in bulk heterojunction solar cells, and its dependence on the physical parameters of the system. In bulk heterojunction organic photovoltaics (OPVs), exciton…
The elementary optical excitations of a two-dimensional electron or hole system have been identified as exciton-Fermi-polarons. Nevertheless, the connection between the bound state of an exciton and an electron, termed trion, and…
Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…
The photon-electron interactions are generally volatile and the intricate multiphysics details of photoexcited carrier dynamics are not yet distinguished. How to nonvolatile control the physical state through all-optical means and clarify…
We report on the dynamics of photodegradation and subsequent recovery of two-photon fluorescence in a dye-doped polymer. The energy dependence suggests that photo-degradation is a linear process while recovery is entropic. Such recovery…
We use nonlinear pump-probe spectroscopy to study optical excitations in a charge-tunable MoSe$_2$\WS$_2$ moir\'e heterostructure. An intense red-detuned laser pulse creates a photonic dressing of the material by introducing a large virtual…