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The extraction of photogenerated charge carriers and the generation of a photovoltage belong to the fundamental functionalities of any solar cell. These processes happen not instantaneously but rather come with finite time constants, e.g.,…

材料科学 · 物理学 2023-02-08 Lisa Krückemeier , Zhifa Liu , Thomas Kirchartz , Uwe Rau

To clarify the ultrafast temporal interplay of the different photocurrent mechanisms occurring in single InAs-nanowire-based circuits, an on-chip photocurrent pump-probe spectroscopy based on coplanar striplines was utilized. The data are…

In recent years the physics of two-dimensional semiconductors was revived by the discovery of the class of transition metal dichalcogenides. In these systems excitons dominate the optical response in the visible range and open many…

介观与纳米尺度物理 · 物理学 2021-02-26 Thilo Hahn , Jacek Kasprzak , Paweł Machnikowski , Tilmann Kuhn , Daniel Wigger

Nonlinear Compton scattering driven by ultraintense lasers presents a promising avenue for enhancing the photon energy, brilliance, and setup compactness of $\gamma$-ray sources. However, a significant challenge lies in achieving a high…

等离子体物理 · 物理学 2024-04-12 Xian-Zhang Wu , Yan-Fei Li , Yu-Tong Li

The ultrafast dynamics of photon-to-charge conversion in an organic light harvesting system is studied by femtosecond time-resolved X-ray photoemission spectroscopy (TR-XPS) at the free-electron laser FLASH. This novel experimental…

Optical excitation and control of excitonic wavepackets in organic molecules is the basis to energy conversion processes. To gain insights into such processes, it is essential to establish the relationship between the coherence timescales…

Fullerene complexes may play a key role in the design of future molecular electronics and nanostructured devices with potential applications in light harvesting using organic solar cells. Charge and energy flow in these systems is mediated…

We analyze Photo-Electron Spectra (PES) for a variety of excitation mechanisms from a simple mono-frequency laser pulse to involved combination of pulses as used, e.g., in attosecond experiments. In the case of simple pulses, the peaks in…

原子与分子团簇 · 物理学 2015-05-20 C. -Z. Gao , P. M. Dinh , P. -G. Reinhard , E. Suraud

We propose a new concept for the design of high-efficiency photocells based on ultra-thin (submicron) semiconductor films of controlled thickness. Using a microscopic model of a thin dielectric layer interacting with incident…

材料科学 · 物理学 2009-11-13 D. Mozyrsky , I. Martin

A typical signature of charge extraction in disordered organic systems is dispersive transport, which implies a distribution of charge carrier mobilities that negatively impact on device performance. Dispersive transport has been commonly…

2D materials are considered a key element in the development of next-generation electronics (nanoelectronics) due to their extreme thickness in the nanometer range and unique physical properties. The ultrafast dynamics of photoexcited…

介观与纳米尺度物理 · 物理学 2024-06-18 Yuri D Glinka

Research into the efficiency of photosynthetic light harvesting has focused on two factors: (1) entanglement of chromophores, and (2) environmental noise. While chromophores are conjugated $\pi$-bonding molecules with strongly correlated…

生物物理 · 物理学 2013-03-29 David A. Mazziotti

Organic solar cells (OSCs) based on non-fullerene acceptors can show high charge generation yields despite near-zero donor-acceptor energy offsets to drive charge separation and overcome the mutual Coulomb attraction between electron and…

Organic solar cells have the potential to be low-cost and efficient solar energy converters, with a promising energy balance. They are made from carbon-based semiconductors, which exhibit favourable light absorption and charge generation…

材料科学 · 物理学 2015-03-13 Carsten Deibel , Vladimir Dyakonov

The optical response of semiconducting monolayer transition-metal dichalcogenides (TMDCs) is dominated by strongly bound excitons that are stable even at room temperature. However, substrate-related effects such as screening and disorder in…

We investigate the dynamical formation of excitons from photoexcited electron-hole plasma and its subsequent decay dynamics in monolayer MoS2 grown by chemical vapor deposition using ultrafast pump and terahertz probe spectroscopy.…

材料科学 · 物理学 2014-10-14 Xuefeng Liu , Qingqing Ji , Zhihan Gao , Shaofeng Ge , Jun Qiu , Zhongfan Liu , Yanfeng Zhang , Dong Sun

F\"orster theory describes electronic exciton energy migration in molecular assemblies as an incoherent hopping process between donor and acceptor molecules. The rate is expressed in terms of the overlap integral between donor fluorescence…

化学物理 · 物理学 2018-10-17 Marco Schröter , Tõnu Pullerits , Oliver Kühn

The steady current induced by electromagnetic field in a 2D system with asymmetric scatterers is studied. The scatterers are assumed to be oriented cuts with one diffusive and another specular sides. Besides, the existence of isotropic…

介观与纳米尺度物理 · 物理学 2009-11-11 M. V. Entin , L. I. Magarill

We investigate the photon statistics of an ensemble of coherently driven non-interacting two-level atoms in the weak driving regime. As it turns out, the system displays unique emission characteristics that are strongly in contrast to the…

量子物理 · 物理学 2024-11-27 M. Bojer , A. Cidrim , P. P. Abrantes , R. Bachelard , J. von Zanthier

There is strong interest in designing and realizing optically-active semiconductor nanostructures of greater complexity for applications in fields ranging from biomedical engineering to quantum computing. While these increasingly complex…

介观与纳米尺度物理 · 物理学 2026-05-25 Jill M. Cleveland , Tory A. Welsch , Eric Y. Chen , D. Bruce Chase , Matthew F. Doty , Hanz Y. Ramírez-Gómez