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We present evidence of magnetic ordering in type-II (Zn, Mn) Te quantum dots. This ordering is attributed to the formation of bound magnetic polarons caused by the exchange interaction between the strongly localized holes and Mn within the…

介观与纳米尺度物理 · 物理学 2015-05-14 I. R. Sellers , R. Oszwaldowski , V. R. Whiteside , M. Eginligil , A. Petrou , I. Zutic , W-C. Chou , W. C. Fan , A. G. Petukhov , B. D. McCombe

Spatially indirect Type-II band alignment in magnetically-doped quantum dot (QD) structures provides unexplored opportunities to control the magnetic interaction between carrier wavefunction in the QD and magnetic impurities. Unlike the…

介观与纳米尺度物理 · 物理学 2018-01-17 P. Zhang , T. Norden , J. M. Pientka , R. Oszwałdowski , A. Najafi , B. Barman , Y. Tsai , W-C. Fan , W-C. Chou , J. E. Han , I. Žutić , B. D. McCombe , A. Petrou

The optically induced spin polarization in (Cd,Mn)Te/(Cd,Mn,Mg)Te diluted-magnetic-semiconductor quantum wells is investigated by means of picosecond pump-probe Kerr rotation. At 1.8 K temperature, additionally to the oscillatory signals…

介观与纳米尺度物理 · 物理学 2016-06-22 E. A. Zhukov , Yu. G. Kusrayev , K. V. Kavokin , D. R. Yakovlev , J. Debus , A. Schwan , I. A. Akimov , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer

We study the formation dynamics of a spontaneous ferromagnetic order in single self-assembled CdMnTe quantum dots. By measuring time-resolved photoluminescence, we determine the formation times for QDs with Mn ion contents x varying from…

Semiconductor quantum dots (QDs) doped with magnetic impurities have been a focus of continuous research for a couple of decades. A significant effort has been devoted to studies of magnetic polarons (MP) in these nanostructures. These…

材料科学 · 物理学 2023-07-19 D. Rederth , R. Oszwaldowski , A. G. Petukhov , J. Pientka

Wide quantum dots were fabricated from multiple quantum well structures based on Zn_{1-x}Mn_xTe/ZnTe (x = 0.076) dilute magnetic semiconductors and were investigated via photoluminescence (PL) in a magnetic field. Calculations taking into…

介观与纳米尺度物理 · 物理学 2015-06-25 Ivan J. Griffin , Peter J. Klar , Daniel Wolverson , J. John Davies , Bernard Lunn , Duncan E. Ashenford , Torsten Henning

We study the exciton magnetic polaron (EMP) formation in (Cd,Mn)Se/(Cd,Mg)Se diluted-magnetic-semiconductor quantum wells using time-resolved photoluminescence (PL). The magnetic field and temperature dependencies of this dynamics allow us…

We study the excitonic structure of CdSe/ZnSe self assembled quantum dots (SAQD) by magneto-photoluminescence (PL) spectroscopy. Using fixed 200 nm apertures through a metal film, we are able to probe single narrow (200 micro-eV)…

In semiconductors, quantum confinement can greatly enhance the interaction between band carriers (electrons and holes) and dopant atoms. One manifestation of this enhancement is the increased stability of exciton magnetic polarons in…

介观与纳米尺度物理 · 物理学 2017-04-27 W. D. Rice , W. Liu , V. Pinchetti , D. R. Yakovlev , V. I. Klimov , S. A. Crooker

In an effort to elucidate the spin (rather than charge) degrees of freedom in colloidal semiconductor nanocrystal quantum dots, we report on a series of static and time-resolved photoluminescence measurements of colloidal CdSe quantum dots…

材料科学 · 物理学 2007-05-23 Madalina Furis , Jennifer Hollingsworth , Victor I. Klimov , Scott A. Crooker

A trion magnetic polaron formed by the exchange interaction of a positively charged exciton (trion) with localized spins of Mn$^{2+}$ ions is found experimentally in a 4\,nm wide Cd$_{0.98}$Mn$_{0.02}$Te/Cd$_{0.78}$Mn$_{0.02}$Mg$_{0.2}$Te…

We propose a model of magnetic polaron formation in semiconductor quantum dots doped with magnetic ions. A wetting layer serves as a reservoir of photo-generated holes, which can be trapped by the adjacent quantum dots. For certain hole…

介观与纳米尺度物理 · 物理学 2012-10-25 J. M. Pientka , R. Oszwałdowski , A. G. Petukhov , J. E. Han , Igor Žutić

We show that through the resonant optical excitation of spin-polarized excitons into CdMnTe magnetic quantum dots, we can induce a macroscopic magnetization of the Mn impurities. We observe very broad (4 meV linewidth) emission lines of…

软凝聚态物质 · 物理学 2009-11-10 T. Gurung , S. Mackowski , H. E. Jackson , L. M. Smith , W. Heiss , J. Kossut , G. Karczewski

We demonstrate that resonant excitation of CdMnTe self-assembled quantum dots creates an ensemble of spin-polarized magnetic polarons at B=0 T. The strong spatial confinement characteristic of quantum dots significantly increases the…

软凝聚态物质 · 物理学 2009-11-10 S. Mackowski , T. Gurung , T. A. Nguyen , H. E. Jackson , L. M. Smith , G. Karczewski , J. Kossut

Magnetically doped nanostructures can significantly enhance the interaction between the band carriers and the dopant atoms. Motivated by the demonstration of the enhanced sp-d exchange interaction in quantum confined structures with the…

介观与纳米尺度物理 · 物理学 2023-01-02 Kalpana Panneerselvam , Bhaskaran Muralidharan

Photoluminescence (PL) and highly circularly-polarized magneto-PL (up to 50% at 6 T) from two-step bandgap InAs/InGaAs/InAlAs quantum wells (QWs) are studied. Bright PL is observed up to room temperature, indicating a high quantum…

We report on a magneto-photoluminescence (PL) study of Mn modulation-doped InAs/InGaAs/InAlAs quantum wells. Two PL lines corresponding to the radiative recombination of photoelectrons with free and bound-on-Mn holes have been observed. In…

We analyze, through resonant photoluminescence, the spin dynamics of an individual magnetic atom (Mn) coupled to a hole in a semiconductor quantum dot. The hybrid Mn-hole spin and the positively charged exciton in a CdTe/ZnTe quantum dot…

介观与纳米尺度物理 · 物理学 2017-06-21 A. Lafuente-Sampietro , H. Boukari , L. Besombes

We show that CdMnTe self-assembled quantum dots can be formed by depositing a submonolayer of Mn ions over a ZnTe surface prior to deposition of the CdTe dot layer. Single dot emission lines and strongly polarized quantum dot…

材料科学 · 物理学 2009-11-10 S. Mackowski , H. E. Jackson , L. M. Smith , J. Kossut , G. Karczewski , W. Heiss

We investigate the evolution of a photoexcitation in correlated materials over a wide range of time scales. The system studied is a one-dimensional model of a manganite with correlated electron, spin, orbital, and lattice degrees of…

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