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Two-dimensional bismuth (Bi) is a promising platform for quantum and energy technologies due to strong spin-orbit coupling, high thermoelectric efficiency, and magnetoresistance. However, scalable and flexible synthesis of high-quality Bi…

Bismuth telluride (Bi2Te3) and its alloys are the best bulk thermoelectric materials known today. The stacked quasi-two-dimensional (2D) layers of Bi2Te3 were also identified as topological insulators. In this paper we describe a method for…

介观与纳米尺度物理 · 物理学 2010-04-19 Desalegne Teweldebrhan , Vivek Goyal , Alexander A. Balandin

The success of topological insulators (TI) in creating devices with unique functionalities is directly connected to the ability of coupling their helical spin states to well defined perturbations. However, up to now, TI-based…

介观与纳米尺度物理 · 物理学 2015-03-12 Thomas Bathon , Paolo Sessi , Konstantin Kokh , Oleg Tereshchenko , Matthias Bode

Because of their loosely bound electrons, electrides offer physical properties useful in chemical synthesis and electronics. For these applications and others, nano-sized electrides offer advantages, but to-date no electride has been…

Based on first-principles calculations, we show that stoichiometric TaSe3, synthesized in space group P21/m, belongs to a three-dimensional (3D) strong topological insulator (TI) phase with Z2 invariants (1;100). The calculated surface…

材料科学 · 物理学 2018-11-07 Simin Nie , Lingyi Xing , Rongying Jin , Weiwei Xie , Zhijun Wang , Fritz B. Prinz

Topology optimization (TO) of 3D surface-enhanced Raman scattering (SERS) substrates faces challenges in managing field singularities and modeling orientation-averaged anisotropic molecules. We present 3D TO for manufacturable SERS…

We theoretically investigate the possibility of establishing ferromagnetism in the topological insulator Bi2Se3 via magnetic doping of 3d transition metal elements. The formation energies, charge states, band structures, and magnetic…

材料科学 · 物理学 2013-01-08 Jian-Min Zhang , Wenguang Zhu , Ying Zhang , Di Xiao , Yugui Yao

A theoretical study of the newly identified Ti5Al2C3 belonging to the MAX phases has been performed by using the first-principles pseudopotential plane-wave method within the generalized gradient approximation (GGA). The energy band…

材料科学 · 物理学 2012-06-19 M. S. Ali , A. K. M. A. Islam , M. A. Hossain

Designing metal-semiconductor junctions is essential for optimizing the performance of modern nanoelectronic devices. A widely used material is TiSi$_2$, which combines low electronic resistivity with good endurance. However, its multitude…

材料科学 · 物理学 2026-01-16 Lukas Hückmann , Jonathon Cottom , Jörg Meyer , Emilia Olsson

Topological insulators (TIs) are novel materials that manifest spin-polarized Dirac states on their surfaces or at interfaces made with conventional matter. We have measured the electron kinetics of bulk doped TI Bi$_2$Se$_3$ with angle…

Silicon telluride (Si2Te3) is a two-dimensional material with a unique variable structure where the silicon atoms form Si-Si dimers to fill the "metal" sites between the Te layers. The Si-Si dimers have four possible orientations: three…

材料科学 · 物理学 2020-01-29 Romakanta Bhattarai , Xiao Shen

As emerging atomically ultrathin metal compounds, MXenes show great promise for catalysts and nanoelectronics applications due to the abundant surface terminations and high metallic conductivity. However, the tendency of the interlayer…

材料科学 · 物理学 2022-10-18 Qiye Guan , Hejin Yan , Yongqing Cai

Topological insulators (TIs) have attracted much attention due to their spin-polarized surface and edge states, whose origin in symmetry gives them intriguing quantum-mechanical properties. Robust control over the chemical potential of TI…

介观与纳米尺度物理 · 物理学 2015-10-28 Andrew L. Yeats , Yu Pan , Anthony Richardella , Peter J. Mintun , Nitin Samarth , David D. Awschalom

Since the emergence of monolayer graphene as a promising two-dimensional material, many other monolayer and few-layer materials have been investigated extensively. An experimental study of few-layer Si2Te3 was recently reported, showing…

材料科学 · 物理学 2016-05-13 Yevgeniy Puzyrev , X. Shen , C. Combs , S. T. Pantelides

In this work we describe the synthesis and electrochemical properties of nitridated hierarchical TiO$_2$ nanotubes as an electrode for supercapacitors. The hierarchical TiO$_2$ nanostructures are formed by a controlled layer-by-layer TiO2…

化学物理 · 物理学 2020-04-28 Nhat Truong Nguyen , Selda Ozkan , Imgon Hwang , Xuemei Zhou , Patrik Schmuki

The colloidal synthesis of large thin two-dimensional (2D) nanosheets is fascinating but challenging, since the growth along the lateral and vertical dimensions need to be controlled independently. In-plane anisotropy in 2D nanosheets is…

材料科学 · 物理学 2019-03-15 Fu Li , Mohammad Mehdi Ramin Moayed , Eugen Klein , Rostyslav Lesyuk , Christian Klinke

The electrical and optoelectronic properties of transition-metal dichalcogenides (TMDs), such as MoS2, are highly dependent on carrier doping and layer thickness. The ability to selectively control these two critical characteristics is of…

材料科学 · 物理学 2023-01-26 Lei Zhang , Kun Liu , Fanyi Kong , Xue Han , Jianxun Dai , Mengmeng Wang , Changsen Sun , Huolin Huang , Lujun Pan , Dawei Li

Two-dimensional (2D) materials for their versatile band structures and strictly 2D nature have attracted considerable attention over the past decade. Graphene is a robust material for spintronics owing to its weak spin-orbit and hyperfine…

介观与纳米尺度物理 · 物理学 2017-01-30 Kuei-Lin Chiu , Yang Xu

We investigate the structure and electronic spectra properties of two-dimensional amorphous bismuthene structures and show that these systems are topological insulators. We employ realistic modeling of amorphous geometries together with…

材料科学 · 物理学 2021-03-01 Bruno Focassio , Gabriel R. Schleder , Marcio Costa , Adalberto Fazzio , Caio Lewenkopf

While topological superconductors are predicted to provide building blocks for fault-tolerant quantum computing, one of the remaining challenges is to find a convenient experimental platform that would allow patterning of circuits. We find…

介观与纳米尺度物理 · 物理学 2016-10-28 Jerome T. Mlack , Atikur Rahman , Gopinath Danda , Natalia Drichko , Sarah Friedensen , Marija Drndic , Nina Markovic