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The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

When doped with a high density of mobile charge carriers, monolayer transition-metal dichalcogenide (TMD) semiconductors can host new types of composite many-particle exciton states that do not exist in conventional semiconductors. Such…

介观与纳米尺度物理 · 物理学 2024-11-22 J. Choi , J. Li , D. Van Tuan , H. Dery , S. A. Crooker

Being motivated by recent achievements in the rapidly developing fields of optical bound states in the continuum (BICs) and excitons in monolayers of transition metal dichalcogenides, we analyze strong coupling between BICs in $\rm Ta_2O_5$…

介观与纳米尺度物理 · 物理学 2018-10-24 K. L. Koshelev , S. K. Sychev , Z. F. Sadrieva , A. A. Bogdanov , I. V. Iorsh

Excitons and their complexes govern optical-related behaviors in semiconductors. Here, using angle-resolved photoemission spectroscopy (ARPES), we have elucidated the light-matter interaction mediated by quasi-steady excitonic complexes…

Electric field-controlled, two-dimensional (2D) exciton dynamics in transition metal dichalcogenide monolayers is a current research focus in condensed matter physics. We have experimentally investigated the spectral and temporal properties…

介观与纳米尺度物理 · 物理学 2019-12-11 Michael Engel , Mathias Steiner

Hybrid structures incorpora1ng both III-nitride and Transi1on Metal Dichalcogenide (TMD) semiconductors have strong applica1on poten1al for light harves1ng and optoelectronics. Here we have inves1gated the proper1es of hybrid structures…

材料科学 · 物理学 2025-09-09 D. Chen , D. Lagarde , L. Hemmen , L. Lombez , P. Renucci , M. Mauguet , L. Ren , C. Robert , N. Grandjean , X. Marie

The common model to describe exciton-plasmon interaction phenomenologically is the coupled oscillator model. Originally developed for atomic systems rather than solid-state matter, this model treats both excitons and plasmons as single…

介观与纳米尺度物理 · 物理学 2024-10-23 Lara Greten , Robert Salzwedel , Diana Schutsch , Andreas Knorr

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

The manipulation of coupled quantum excitations is of fundamental importance in realizing novel photonic and optoelectronic devices. We use electroluminescence to probe plasmon-exciton coupling in hybrid structures consisting of a nanoscale…

All-solid-state strong light-matter coupling systems with large vacuum Rabi splitting are great important for quantum information application, such as quantum manipulation, quantum information storage and processing. The monolayer…

介观与纳米尺度物理 · 物理学 2017-04-27 Jinxiu Wen , Hao Wang , Huanjun Chen , Shaozhi Deng , Ningsheng Xu

Based on \emph{ab initio} theoretical calculations of the optical spectra of vertical heterostructures of MoSe$_2$ (or MoS$_2$) and WSe$_2$ sheets, we reveal two spin-orbit-split Rydberg series of excitonic states below the \textsl{A}…

介观与纳米尺度物理 · 物理学 2018-04-18 Roland Gillen , Janina Maultzsch

Trion states of three correlated particles (e.g., two electrons and one hole) are essential to understand the optical spectra of doped or gated nanostructures, like carbon nanotubes or transition-metal dichalcogenides. We develop a…

介观与纳米尺度物理 · 物理学 2016-06-22 Thorsten Deilmann , Matthias Drüppel , Michael Rohlfing

Monolayer transition metal dichalcogenides, coupled to metal plasmonic nanocavities, have recently emerged as new platforms for strong light-matter interactions. These systems are expected to have nonlinear optical properties that will…

We report the direct observation of quantum coupling in individual quantum dot molecules and its manipulation using static electric fields. A pronounced anti-crossing of different excitonic transitions is observed as the electric field is…

介观与纳米尺度物理 · 物理学 2007-05-23 H. J. Krenner , M. Sabathil , E. C. Clark , A. F. Kress , D. Schuh , M. Bichler , G. Abstreiter , J. J. Finley

Monolayers of transition-metal dichalcogenides (TMDs) are characterized by an extraordinarily strong Coulomb interaction giving rise to tightly bound excitons with binding energies of hundreds of meV. Excitons dominate the optical response…

材料科学 · 物理学 2018-05-30 Samuel Brem , Gunnar Berghaeuser , Malte Selig , Ermin Malic

Metal monochalcogenide GaSe is a classic layered semiconductor that has received increasing research interest due to its highly tunable electronic and optical properties for ultrathin electronics applications. Despite intense research…

材料科学 · 物理学 2024-05-14 Fanhao Jia , Zhao Tang , Greis J. Cruz , Weiwei Gao , Shaowen Xu , Wei Ren , Peihong Zhang

Heterostructures of two-dimensional transition metal dichalcogenides (TMDs) are emerging as a promising platform for investigating exotic correlated states of matter. Here, we propose to engineer Bose-Fermi mixtures in these systems by…

介观与纳米尺度物理 · 物理学 2024-08-01 Caterina Zerba , Clemens Kuhlenkamp , Ataç Imamoğlu , Michael Knap

We study a doped transition metal dichalcogenide (TMDC) monolayer in an optical microcavity. Using the microscopic theory, we simulate spectra of quasiparticles emerging due to the interaction of material excitations and a high-finesse…

材料科学 · 物理学 2024-07-23 Y. V. Zhumagulov , S. Chiavazzo , D. R. Gulevich , V. Perebeinos , I. A. Shelykh , O. Kyriienko

Excitons are composite bosons that can feature spin singlet and triplet states. In usual semiconductors, without an additional spin-flip mechanism, triplet excitons are extremely inefficient optical emitters. Transition metal…

Coupled two-dimensional electron-hole bilayers provide a unique platform to study strongly correlated Bose-Fermi mixtures in condensed matter. Electrons and holes in spatially separated layers can bind to form interlayer excitons, composite…