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Light-emitting diodes are of importance for lighting, displays, optical interconnects, logic and sensors. Hence the development of new systems that allow improvements in their efficiency, spectral properties, compactness and integrability…

The combination of repulsive and attractive Coulomb interactions in a quantum electron(e)-hole(h) fluid can give rise to novel correlated phases of multiparticle charge complexes such as excitons, trions and biexcitons. Here we report the…

Strong coupling between the electronic states of monolayer transition metal dichalcogenides (TMDC) such as MoS$_2$, MoSe$_2$, WS$_2$, or WSe$_2$, and a two-dimensional (2D) photonic cavity gives rise to several exotic effects. The Dirac…

介观与纳米尺度物理 · 物理学 2017-08-02 Amrit De , Roger Lake

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying…

介观与纳米尺度物理 · 物理学 2017-03-28 N. Lundt , A. Maryński , E. Cherotchenko , A. Pant , X. Fan , G. Sęk , S. Tongay , A. V. Kavokin , S. Höfling , C. Schneider

We study the neutral exciton energy spectrum fine structure and its spin dephasing in transition metal dichalcogenides such as MoS$_2$. The interaction of the mechanical exciton with its macroscopic longitudinal electric field is taken into…

介观与纳米尺度物理 · 物理学 2014-05-15 M. M. Glazov , T. Amand , X. Marie , D. Lagarde , L. Bouet , B. Urbaszek

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

The interaction of excitons with lattice vibrations underlies the scattering from bright to dark excitons as well as the coherent modulation of the exciton energy. Unlike the former mechanism, which involves phonons with finite momentum,…

介观与纳米尺度物理 · 物理学 2024-06-24 Enrico Perfetto , Kai Wu , Gianluca Stefanucci

Coulomb bound electron-hole pairs, excitons, govern the optical properties of semi-conducting transition metal dichalcogenides like MoS$_2$ and WSe$_2$. We study optical transitions at the K-point for 2H homobilayer MoS$_2$ in Density…

Excitons in two-dimensional semiconductors provide a novel platform for fundamental studies of many-body interactions. In particular, dipolar interactions between spatially indirect excitons may give rise to strongly correlated phases of…

介观与纳米尺度物理 · 物理学 2022-09-14 Rafał Ołdziejewski , Alessio Chiocchetta , Johannes Knörzer , Richard Schmidt

Tailoring and enhancing the interaction between light and matter is of great importance for both fundamental researches and future photonic and optoelectronic applications. Due to their high exciton oscillator strength and large exciton…

Recent advances in the field of vertically stacked 2D materials have revealed a rich exciton landscape. In particular, it has been demonstrated that out-of-plane electrical fields can be used to tune the spectral position of spatially…

介观与纳米尺度物理 · 物理学 2023-01-18 Joakim Hagel , Samuel Brem , Ermin Malic

Monolayer transition metal dichalcogenides (TMDs) host deeply bound excitons interacting with itinerant electrons, and as such they represent an exciting new quantum many-body Bose-Fermi mixture. Here, we demonstrate that electrons…

超导电性 · 物理学 2022-10-24 Aleksi Julku , Jami J. Kinnunen , Arturo Camacho-Guardian , Georg M. Bruun

The photoluminescence (PL) spectrum of transition metal dichalcogenides (TMDs) shows a multitude of emission peaks below the bright exciton line and not all of them have been explained yet. Here, we study the emission traces of…

Excitons in monolayer transition-metal dichalcogenides (TMDs) have garnered significant attention because of their large binding energies due to weakly screened Coulomb interaction, and direct bandgap at the K/K$^\prime$ point in the…

The optical properties of transition metal dichalcogenide monolayers such as the two-dimensional semiconductors MoS$_2$ and WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. The light emission yield depends on whether…

材料科学 · 物理学 2016-03-23 J. P. Echeverry , B. Urbaszek , T. Amand , X. Marie , I. C. Gerber

The optical responses of semiconducting transition metal dichalcogenides are dominated by excitons. Being able to strongly interact with light and other materials excitations, excitons in semiconductors are prototypes for investigating…

介观与纳米尺度物理 · 物理学 2021-01-28 Xuke Jiang , Masoud Taleb , Florian Diekmann , Kai Rossnagel , Nahid Talebi

Photoluminescence spectra, shows that monolayer Transition-metal dichalcogenides (MLTMDCs), possess charged exciton binding energies, conspicuously similar to the energy of optical phonons. This enigmatic coincidence has offered…

介观与纳米尺度物理 · 物理学 2020-09-16 Sabrine Ayari , Sihem Jaziri , Robson Ferreira , Gerald Bastard

The optical properties of particularly the tungsten-based transition-metal dichalcogenides are strongly influenced by the presence of dark excitons. Recently, theoretical predictions as well as indirect experimental insights have shown that…

介观与纳米尺度物理 · 物理学 2019-12-25 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Tungsten-based monolayer transition metal dichalcogenides host a long-lived dark exciton, an electron-hole pair in a spin-triplet configuration. The long lifetime and unique spin properties of the dark exciton provide exciting opportunities…

We investigate how many-electron excited states emerge in twisted MoSe2 homobilayers when the lattice reconstructions evolve. Notably, we identify a new trion resonance that arises in the transition regime of lattice reconstruction, where…