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The generation of energetic electron bunches by the interaction of a short, ultra-intense ($I>10^{19} \textrm{W/cm}^2$) laser pulse with "grating" targets has been investigated in a regime of ultra-high pulse-to-prepulse contrast…

We investigate the spectroscopic fingerprints of electron-plasmon coupling in integrated (PES) and angle-resolved photoemission spectroscopy (ARPES). To account for electron-plasmon interactions at a reduced computational cost, we derived…

强关联电子 · 物理学 2015-07-27 Fabio Caruso , Feliciano Giustino

Formation of nanoscale laser-induced periodic surface structures on thin metal films (of the size of the optical penetration depth) is a yet unexplored area that is expected to open new routes for laser patterning and a wealth of exciting…

Experiments on the excitation of propagating surface plasmons (SPs) by ultrashort, high intensity laser interaction with "grating" targets are reviewed. At intensities exceeding $10^{19}~\mbox{W cm}^{-2}$ on target, i.e. in the strongly…

等离子体物理 · 物理学 2019-05-01 A. Macchi , G. Cantono , L. Fedeli , F. Pisani , T. Ceccotti

Correlated transition metal oxides, such as cuprates, nickelates, and manganites, are typically considered "bad metals", where high electromagnetic losses suppress the conventional plasmonic effects observed in noble metals, 2D electron…

Harnessing the optical properties of noble metals down to the nanometer-scale is a key step towards fast and low-dissipative information processing. At the 10-nm length scale, metal crystallinity and patterning as well as probing of surface…

Electromagnetic hot-spots at ultra-narrow plasmonic nanogaps carry immense potential to drive detection limits down to few molecules in sensors based on surface enhanced Raman or Fluorescence spectroscopies. However, leveraging the EM…

The accurate calculation of laser energy absorption during femto- or picosecond laser pulse experiments is very important for the description of the formation of periodic surface structures. On a rough material surface, a crack or a step…

应用物理 · 物理学 2020-04-22 P. N. Terekhin , O. Benhayoun , S. T. Weber , D. S. Ivanov , M. E. Garcia , B. Rethfeld

Assemblies of plasmonic nanoparticles (NPs) support hybridized modes of localized surface plasmons (LSPs), which delocalize in geometrically well-ordered arrangements. Here, the hybridization behavior of LSPs in geometrically completely…

Nonlinear optical absorption of light by materials are weak due to its perturbative nature, although a strong nonlinear response is of crucial importance to applications in optical limiting and switching. Here we demonstrate experimentally…

Tapered metallic grooves have been shown to support plasmons -- electromagnetically coupled oscillations of free electrons at metal-dielectric interfaces -- across a variety of configurations and V-like profiles. Such plasmons may be…

介观与纳米尺度物理 · 物理学 2015-05-22 Cameron L. C. Smith , Nicolas Stenger , Anders Kristensen , N. Asger Mortensen , Sergey I. Bozhevolnyi

The ability to confine light into tiny spatial dimensions is important for applications such as microscopy, sensing and nanoscale lasers. While plasmons offer an appealing avenue to confine light, Landau damping in metals imposes a…

Surface plasmons have attracted growing interest from the photonics community due to their inherent ability to controllably confine light below the diffraction limit and their direct application in trapping and transporting matter at the…

Regular arrays of metal nanoparticles on metal films have tuneable optical resonances that can be applied for surface enhanced Raman scattering or biosensing. With the aim of developing more surface selective geometries we investigate…

介观与纳米尺度物理 · 物理学 2012-09-13 Andreas Hohenau , Joachim R. Krenn

We perform a comprehensive analysis of the spectrum of graphene plasmons which arise when a pair of sheets are confined between conducting materials. The associated enhanced local fields may be employed in the manipulation of light on the…

介观与纳米尺度物理 · 物理学 2017-09-05 Godfrey Gumbs , Dipendra Dahal , Antonios Balassis

A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

原子物理 · 物理学 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Chains of metallic nanoparticles sustain strongly confined surface plasmons with relatively low dielectric losses. To exploit these properties in applications,such as waveguides, the fabrication of long chains of low disorder and a thorough…

Plasmons --the collective oscillations of electrons in conducting materials-- play a pivotal role in nanophotonics because of their ability to couple electronic and photonic degrees of freedom. In particular, plasmons in graphene --the…

材料科学 · 物理学 2018-05-08 Renwen Yu , F. Javier García de Abajo

We propose a composite layered structure for tunable, low-loss plasmon resonances, which con- sists of a noble-metal thin film coated in graphene and supported on a hexagonal boron nitride (hBN) substrate. We calculate electron energy loss…

介观与纳米尺度物理 · 物理学 2016-05-20 L. Rast , T. J. Sullivan , V. K. Tewary

Porous nanosponges, percolated with a three-dimensional network of 10-nm sized ligaments, recently emerged as promising substrates for plasmon-enhanced spectroscopy and (photo-)catalysis. Experimental and theoretical work suggests surface…

介观与纳米尺度物理 · 物理学 2018-09-19 Jinhui Zhong , Abbas Chimeh , Anke Korte , Felix Schwarz , Juemin Yi , Dong Wang , Jinxin Zhan , Peter Schaaf , Erich Runge , Christoph Lienau