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The self-consistent field theory (SCFT) is a powerful framework for the study of the phase behavior and structural properties of many-body systems. In particular, polymeric SCFT has been successfully applied to inhomogeneous polymeric…

软凝聚态物质 · 物理学 2019-01-31 An-Chang Shi

Self-consistent field theory (SCFT) has proven to be a powerful tool for modeling equilibrium microstructures of soft materials, particularly for multiblock polymers. A very successful approach to numerically solving the SCFT set of…

软凝聚态物质 · 物理学 2017-01-04 David M. Ackerman , Kris Delaney , Glenn H. Fredrickson , Baskar Ganapathysubramanian

Self-consistent field theory (SCFT) is one of the useful methods to simulate phase separated structures of multi-component polymer systems. In this article, we propose an SCFT for semiflexible polymer melts, where the basic equations for…

软凝聚态物质 · 物理学 2025-03-04 Yutaka Oya , Toshihiro Kawakatsu

Self-consistent field theory (SCFT) is one of the most widely-used framework in studying the equilibrium phase behaviors of inhomogenous polymers. For liquid crystalline polymeric systems, the main numerical challenges of solving SCFT…

数值分析 · 数学 2024-09-16 Zhijuan He , Kai Jiang , Liwei Tan , Xin Wang

The phase behavior of asymmetrically interacting ABC star triblock copolymer melts is investigated by the self-consistent field theory (SCFT). Motivated by the experimental systems, in this study, we focus on the systems in which the…

软凝聚态物质 · 物理学 2015-08-25 Kai Jiang , Juan Zhang , Qin Liang

Block copolymers provide a wonderful platform in studying the soft condensed matter systems. Many fascinating ordered structures have been discovered in bulk and confined systems. Among various theories, the self-consistent field theory…

软凝聚态物质 · 物理学 2019-05-01 Huayi Wei , Ming Xu , Wei Si , Kai Jiang

Diblock copolymers blended with homopolymer may self-assemble into spherical, cylindrical or lamellar aggregates. Transitions between these structures may be driven by varying the homopolymer molecular weight or the molecular weight or…

统计力学 · 物理学 2011-06-28 M. J. Greenall , D. M. A. Buzza , T. C. B. McLeish

We present a self-consistent field theory (SCFT) study of spherical micelle formation in a blend of poly(styrene-butadiene) diblocks and homopolystyrene. The micelle core radii, corona thicknesses and critical micelle concentrations are…

软凝聚态物质 · 物理学 2011-06-28 M. J. Greenall , D. M. A. Buzza , T. C. B. McLeish

We present a self-consistent field theory (SCFT) of semiflexible (wormlike) diblock copolymers, each consisting of a rigid and a flexible part. The segments of the polymers are otherwise identical, in particular with regard to their…

软凝聚态物质 · 物理学 2009-11-07 Dominik Düchs , D. E. Sullivan

We review various methods to investigate the statics and the dynamics of collective composition fluctuations in dense polymer mixtures within fluctuating-field approaches. The central idea of fluctuating-field theories is to rewrite the…

软凝聚态物质 · 物理学 2007-05-23 Marcus Mueller , Friederike Schmid

Based on a functional-integral formalism, a generalization of the self-energy-functional theory (SFT) is proposed which is applicable to systems of interacting electrons with disorder. Similar to the pure case without disorder, a…

强关联电子 · 物理学 2013-05-29 Michael Potthoff , Matthias Balzer

Our work establishes the mathematical equivalence between polymer Self Consistent Field Theory and interfacial SAFT based classical Density Functional Theory by providing an explicit proof that SCFT is the mean field (MF) or saddle point…

介观与纳米尺度物理 · 物理学 2025-12-10 Maximo T. Estrada

We demonstrate in the present study that self-consistent calculations based on the self-energy functional theory (SFT) are possible for the electronic structure of realistic systems in the context of quantum chemistry. We describe the…

材料科学 · 物理学 2018-06-14 Taichi Kosugi , Hirofumi Nishi , Yoritaka Furukawa , Yu-ichiro Matsushita

The self-energy functional theory (SFT) is generalized to describe the real-time dynamics of correlated lattice-fermion models far from thermal equilibrium. This is achieved by means of a reformulation of the original equilibrium theory in…

强关联电子 · 物理学 2013-10-21 Felix Hofmann , Martin Eckstein , Enrico Arrigoni , Michael Potthoff

Constrained density functional theory (cDFT) is a versatile electronic structure method that enables ground-state calculations to be performed subject to physical constraints. It thereby broadens their applicability and utility. Automated…

其他凝聚态物理 · 物理学 2016-08-03 David D. O'Regan , Gilberto Teobaldi

Self-consistent field theory (SCFT) and strong segregation theory (SST) are used to explore the parameter space governing the self-assembly of cylinder forming block copolymers (BCPs) on a modulated substrate. The stability of in-plane…

材料科学 · 物理学 2018-11-16 Karim Gadelrab , Alfredo Alexander-Katz

The relation between saddle points of the potential of a classical many-particle system and the analyticity properties of its thermodynamic functions is studied. For finite systems, each saddle point is found to cause a nonanalyticity in…

统计力学 · 物理学 2011-11-09 Michael Kastner , Oliver Schnetz , Steffen Schreiber

We investigate the properties of a system of semi-diluted polymers in the presence of charged groups and counter-ions, by means of self-consistent field theory. We study a system of polyelectrolyte chains grafted to a similarly, as well as…

软凝聚态物质 · 物理学 2015-05-19 Gabriele Migliorini

The phase behavior of linear dendritic triblock copolymer melts(AB2C4) is studied by self-consistent-field theory (SCFT) in order to find the effects of branching on the phase behavior of ABC linear triblock copolymer melts. We focus on a…

软凝聚态物质 · 物理学 2023-09-19 Danyang Chen , Xiaowei Ning

We study a model of flexible block copolymers (BCPs) in which there is an enlthalpic preference for local alignment, among like-block segments. We describe a generalization of the self-consistent field theory (SCFT) of flexible BCPs to…

软凝聚态物质 · 物理学 2018-05-23 Christopher J. Burke , Gregory M. Grason
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