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Recent advances in scanning transmission electron microscopy (STEM) instrumentation have made it possible to focus electron beams with sub-atomic precision and to identify the chemical structure of materials at the level of individual…

材料科学 · 物理学 2017-03-08 T. Susi , J. C. Meyer , J. Kotakoski

Patterning of graphene into micro- and nano-ribbons allows for the tunability in emerging fields such as flexible electronic and optoelectronic devices, and is gaining interest for the production of more efficient reinforcement for…

Atomic resolution high angle annular dark field imaging of suspended, single-layer graphene, onto which the metals Cr, Ti, Pd, Ni, Al and Au atoms had been deposited was carried out in an aberration corrected scanning transmission electron…

介观与纳米尺度物理 · 物理学 2012-08-02 Quentin M. Ramasse , Recep Zan , Ursel Bangert , Danil W. Boukhvalov , Young-Woo Son , Konstantin S. Novoselov

This paper presents a detailed computational protocol for atomistic simulation of the formation and growth of metal-containing nanostructures during the Focused Electron Beam Induced Deposition (FEBID) process. The protocol is based upon…

We show that electron irradiation in a dedicated scanning transmission microscope can be used as a nano-electron-lithography technique allowing the controlled reshaping of single walled carbon and boron nitride nanotubes. The required…

材料科学 · 物理学 2008-01-16 Alberto Zobelli , Alexandre Gloter , Chris P. Ewels , Christian Colliex

In spite of years of intense research, graphene continues to produce surprising results. Recently, it was experimentally observed that under certain conditions graphene can self-drive its tearing and peeling from substrates. This process…

介观与纳米尺度物理 · 物理学 2018-01-17 Alexandre F. Fonseca , Douglas S. Galvao

Precision control of interfacial structures and electronic properties is the key to the realization of functional heterostructures. Here, utilizing the scanning tunneling microscope (STM) both as a manipulation and characterization tool, we…

介观与纳米尺度物理 · 物理学 2019-01-09 Chuanxu Ma , Zhongcan Xiao , Jingsong Huang , Liangbo Liang , Wenchang Lu , Kunlun Hong , Bobby G. Sumpter , J. Bernholc , An-Ping Li

The direct manipulation of individual atoms in materials using scanning probe microscopy has been a seminal achievement of nanotechnology. Recent advances in imaging resolution and sample stability have made scanning transmission electron…

The shape of metal nanoparticles embedded in dielectric matrices influences the optical properties of the composite material. Swift heavy ion irradiation can induce a controllable shape transformation in gold and other metals embedded in…

材料科学 · 物理学 2022-04-22 Aleksi A. Leino , Ville E. Jantunen , Flyura Djurabekova

We demonstrate anisotropic etching of single-layer graphene by thermally-activated nickel nanoparticles. Using this technique, we obtain sub-10nm nanoribbons and other graphene nanostructures with edges aligned along a single…

One-dimensional diffusion of Co ad-atoms on graphene nanoribbons has been induced and investigated by means of scanning tunnelling microscopy (STM). To this end, the nanoribbons and the Co ad-atoms have been imaged before and after…

介观与纳米尺度物理 · 物理学 2021-10-22 Tobias Preis , Sasha Vrbica , Jonathan Eroms , Jascha Repp , Jan M. van Ruitenbeek

Recent advances in scanning transmission electron microscopy (STEM) allow to observe solid-state transformations and reactions in materials induced by thermal stimulus or electron beam on the atomic level. However, despite the rate at which…

材料科学 · 物理学 2019-11-26 Maxim Ziatdinov , Ondrej Dyck , Stephen Jesse , Sergei V. Kalinin

Substituting heteroatoms and non-benzenoid carbons into nanographene structure offers an unique opportunity for atomic engineering of electronic properties. Here we show the bottom-up synthesis of graphene nanoribbons (GNRs) with embedded…

We report the electronic properties of two-dimensional systems made of graphene nanoribbons which are patterned with ad-atoms in two separated regions. Due to the extra electronic confinement induced by the presence of the impurities, we…

介观与纳米尺度物理 · 物理学 2015-09-25 J. W. González , L. Rosales , M. Pacheco , A. Ayuela

Photo-induced edge states in low dimensional materials have attracted considerable attention due to the tunability of topological properties and dispersion. Specifically, graphene nanoribbons have been predicted to host chiral edge modes…

介观与纳米尺度物理 · 物理学 2020-11-12 Yuan Chen , Yao Wang , Martin Claassen , Brian Moritz , Thomas P. Devereaux

We demonstrate that the sub-atomically focused beam of a scanning transmission electron microscope (STEM) can be used to controllably manipulate individual dopant atoms in a 2D graphene lattice. We demonstrate the manipulation of adsorbed…

材料科学 · 物理学 2018-08-06 Ondrej Dyck , Songkil Kim , Sergei V. Kalinin , Stephen Jesse

Graphene functionalized with catalytic transition metals offers high-performance gas sensing by coupling graphene's exceptional electronic transport properties with the metal's catalytic activity, yet the atomistic relationships connecting…

材料科学 · 物理学 2025-05-29 Akram Ibrahim , Ahmed M. Hafez , Mahmooda Sultana , Can Ataca

The practical realization of nano-scale electronics faces two major challenges: the precise engineering of the building blocks and their assembly into functional circuits. In spite of the exceptional electronic properties of carbon…

介观与纳米尺度物理 · 物理学 2008-07-09 Levente Tapaszto , Gergely Dobrik , Philippe Lambin , Laszlo P Biro

To clarify the yielding mechanism of small hydrocarbon molecules in chemical sputtering between hydrogen and graphene sheets, we made classical molecular dynamics simulation with modified Brenner's REBO potential which we proposed to deal…

材料科学 · 物理学 2007-05-23 Hiroaki Nakamura , Atsushi Ito

Directed atomic fabrication using an aberration-corrected scanning transmission electron microscope (STEM) opens new pathways for atomic engineering of functional materials. In this approach, the electron beam is used to actively alter the…