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We present a study the initial stages of ice growth on pristine and oxygen-functionalized highly oriented pyrolytic graphite (O-HOPG), combining low-temperature scanning tunneling microscopy (LT-STM) and machine-learning structural…

Coarse grained molecular dynamics simulations are presented in which the sensitivity of the ice nucleation rate to the hydrophilicity of a graphene nanoflake is investigated. We find that an optimal interaction strength for promoting ice…

材料科学 · 物理学 2015-06-01 Stephen J. Cox , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

We show a general two-step method to grow hydroxide and oxide nanocrystals of the iron family elements (Ni, Co, Fe) on graphene with two degrees of oxidation. Drastically different nanocrystal growth behaviors were observed on low-oxidation…

材料科学 · 物理学 2010-02-19 Hailiang Wang , Joshua Tucker Robinson , Georgi Diankov , Hongjie Dai*

Ice nucleation from vapor presents a variety of challenges across a wide range of industries and applications including refrigeration, transportation, and energy generation. However, a rational comprehensive approach to fabricating…

Deposition of water on aerosol particles contributes to ice cloud formation in the atmosphere with implications for the water cycle and climate on Earth. The heterogeneous ice nucleation process is influenced by physico-chemical properties…

化学物理 · 物理学 2013-09-13 Xiangrui Kong , Patrik U. Andersson , Erik S. Thomson , Jan B. C. Pettersson

Numerous studies have focused on a low surface energy coating and a micro/nanoscale surface texture to design functional surfaces that delay frost formation and reduce ice adhesion. However, the scientific challenges for in developing…

应用物理 · 物理学 2019-04-16 Yuehan Yao , Emma Feldman , Kyoo-Chul Park

The non-wetting phenomena of water on certain solid surfaces have been under intensive study for decades, but the nature of hydrophobic/water interfaces remains controversial. Here a water/graphite interface is investigated with…

软凝聚态物质 · 物理学 2012-04-02 Ing-Shouh Hwang , Chih-Wen Yang , Yi-Hsien Lu

We report a versatile water-based method for transferring nanostructures onto surfaces of various shapes and compositions. The transfer occurs through the intercalation of a layer of water between a hydrophilic substrate and a hydrophobic…

介观与纳米尺度物理 · 物理学 2010-07-27 Grégory F. Schneider , Victor E. Calado , Henny Zandbergen , Lieven M. K. Vandersypen , Cees Dekker

Adsorbed layers of water are ubiquitously present at surfaces and fill in microscopic pores, playing a central role in many phenomena in such diverse fields as materials science, geology, biology, tribology, nanotechnology. Despite such…

介观与纳米尺度物理 · 物理学 2015-03-26 G. Algara-Siller , O. Lehtinen , F. C. Wang , R. R. Nair , U. Kaiser , H. A. Wu , I. V. Grigorieva , A. K. Geim

Experimental investigations of hydrophobic/water interfaces often return controversial results, possibly due to the unknown role of gas accumulation at the interfaces. Here, during advanced atomic force microscopy of the initial evolution…

介观与纳米尺度物理 · 物理学 2015-12-29 Ing-Shouh Hwang , Chung-Kai Fang , Hsien-Chen Ko , Chih-Wen Yang , Yi-Hsien Lu

Ice accumulation hinders the performance of, and poses safety threats for infrastructure both on the ground and in the air. Previously, rationally designed superhydrophobic surfaces have demonstrated some potential as a passive means to…

软凝聚态物质 · 物理学 2018-09-10 Thomas Vasileiou , Thomas M. Schutzius , Dimos Poulikakos

We report here a fully atomistic molecular dynamics study on the dynamics of impact of water nanodroplets (100 {\AA} of diameter) at high velocities (from 1 up to 15 {\AA}/ps) against graphene targets. Our results show that tuning graphene…

材料科学 · 物理学 2018-08-28 Ygor M. Jaques , Douglas S. Galvao

Molten metallic nanoparticles have recently been used to construct graphene nanostructures with crystallographic edges. The mechanism by which this happens, however, remains unclear. Here, we present a simple model that explains how a…

介观与纳米尺度物理 · 物理学 2010-08-16 Sujit S. Datta

The performance of graphene oxide(GO)-based materials strongly depends on the lateral size and size distribution of GO nanosheets. Various methods are employed to prepare GO nanosheets with a narrow size distribution. One of the promising…

软凝聚态物质 · 物理学 2019-03-26 Xin Xu , Luofu Liu , Hongya Geng , Jianjun Wang , Jiajia Zhou , Ying Jiang , Masao Doi

The unique and remarkable properties of graphene can be exploited as the basis to a wide range of applications. However, in spite of years of investigations there are some important graphene properties that are not still fully understood,…

介观与纳米尺度物理 · 物理学 2016-02-08 Ygor M. Jaques , Gustavo Brunetto , Douglas S. Galvao

The issue of ice accumulation at low-temperature circumstances causes multiple problems and serious damages in many civil infrastructures which substantially influence human daily life. However, despite the significant consideration in…

化学物理 · 物理学 2020-11-24 Amir Afshar , Dong Meng

The growth of single and multilayer graphene nano-flakes on MgO and ZrO2 at low temperatures is shown through transmission electron microscopy. The graphene nano-flakes are ubiquitously anchored at step edges on MgO (100) surfaces. Density…

What makes a material a good ice nucleating agent? Despite the importance of heterogeneous ice nucleation to a variety of fields, from cloud science to microbiology, major gaps in our understanding of this ubiquitous process still prevent…

化学物理 · 物理学 2016-11-29 Martin Fitzner , Gabriele C Sosso , Stephen J Cox , Angelos Michaelides

The wetting properties of graphene have proven controversial and difficult to assess. The presence of a graphene layer on top of a substrate does not significantly change the wetting properties of the solid substrate, suggesting that a…

软凝聚态物质 · 物理学 2017-02-10 Bijoyendra Bera , Noushine Shahidzadeh , Himanshu Mishra , Daniel Bonn

Surface icing affects the safety and performance of numerous processes in technology. Previous studies mostly investigated freezing of individual droplets. The interaction among multiple droplets during freezing is investigated less,…

软凝聚态物质 · 物理学 2019-01-23 Gustav Graeber , Valentin Dolder , Thomas M. Schutzius , Dimos Poulikakos
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