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The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are…

原子物理 · 物理学 2017-02-22 S. Schippers , A. L. D. Kilcoyne , R. A. Phaneuf , A. Müller

We investigate positron scattering upon endohedrals and compare it with electron-endohedral scattering. We show that the polarization of the fullerene shell considerably alters the polarization potential of an atom, stuffed inside a…

原子物理 · 物理学 2017-08-02 M. Ya. Amusia , L. V. Chernysheva

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

原子物理 · 物理学 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

Dynamically rich nature of the high-order harmonic generation process lends itself to a variety of ways to increase photon yield and extend the harmonic cut-off frequency. We show here that high-harmonic generation from an atom confined…

原子物理 · 物理学 2019-12-25 T. Topcu , E. A. Bleda , Z. Altun

Effects of the interchannel coupling on the spin polarization of energetic photoelectrons emitted from atomic Ne valence subshells are examined. Like previously obtained results for cross sections and angular distributions, the…

原子物理 · 物理学 2021-06-08 Himadri S. Chakraborty , Pranawa C. Deshmukh , Steven T. Manson

The electron-phonon and Coulomb interactions inC$_{60}$, and larger fullerene spheres are analyzed. The coupling between electrons and intramolecular vibrations give corrections $\sim 1 - 10$ meV to the electronic energies for C$_{60}$, and…

凝聚态物理 · 物理学 2009-10-22 F. Guinea , J. Gonzalez , M. A. H. Vozmediano

Photons strongly coupled to material systems constitute a novel system for studying the dynamics of non-equilibrium quantum many-body systems. We give a fully analytical description of the dynamics of photons coupled to a one-dimensional…

量子物理 · 物理学 2023-01-04 Björn Schrinski , Anders S. Sørensen

The photoelectric effect describes the ejection of an electron upon absorption of one or several photons. The kinetic energy of this electron is determined by the photon energy reduced by the binding energy of the electron and, if strong…

We provide the initial insight into the angle-differential photodetachment spectra of fullerene anions beyond the dipole approximation by utilizing a broadly used modelling of C$_{n}$. In the model, the C$_{n}$ cage is approximated by a…

原子物理 · 物理学 2018-10-02 V K Dolmatov , A Edwards , C G Lane

In this paper we present a mathematical analysis of the photoelectric effect for one-electron atoms in the framework of non-relativistic QED. We treat photo-ionization as a scattering process where in the remote past an atom in its ground…

数学物理 · 物理学 2015-05-14 Marcel Griesemer , Heribert Zenk

We demonstrate that the Auger decay rate in an endohedral atom is very sensitive to the atom's location in the fullerene cage. Two additional decay channels appear in an endohedral system: (a) the channel due to the change in the electric…

原子与分子团簇 · 物理学 2015-05-20 Andrey V. Korol , Andrey V. Solov'yov

Massively parallel ionization of many atoms in a cluster or bio-molecule is identified as new phenomenon of light-matter interaction which becomes feasible through short and intense FEL pulses. Almost simultaneously emitted from the…

原子与分子团簇 · 物理学 2012-04-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

The endohedral fullerene Er3N@C80 shows characteristic 1.5 micron photoluminescence at cryogenic temperatures associated with radiative relaxation from the crystal-field split Er3+ 4I13/2 manifold to the 4I15/2 manifold. Previous…

Hartree-Fock atom in a strong electric static field is considered. It is demonstrated that exchange between outer and inner electrons, taken into account by the so-called Fock term affects strongly the long-range behavior of the inner…

原子物理 · 物理学 2015-05-13 M. Ya. Amusia

We study the ground state structure and aspects of photoionization dynamics of the $Na_{20}@C_{240}$ endofullerene. The structure shows effects from the electronic coupling between the nested cluster and the fullerene cage. They include the…

原子与分子团簇 · 物理学 2024-12-20 Rasheed Shaik , Hari R. Varma , Mohamed El-Amine Madjet , Fulu Zheng , Himadri S. Chakraborty

We investigate here the fast electron scattering upon endohedral atoms that present a fullerene CN staffed by an atom A, A@CN. We calculate the inelastic scattering cross-section expressing it via generalized oscillator strengths (GOS)…

原子与分子团簇 · 物理学 2012-03-06 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We demonstrate for the first time that the effect of fullerene shell upon photoionization of the "caged" atom in an endohedral can result in formation of Giant Endohedral Resonances or GER. This is illustrated by the concrete case of Xe@C60…

化学物理 · 物理学 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

The present paper explores possible features of electron elastic scattering off endohedral fullerenes $A$@C$_{60}$. It focuses on how dynamical polarization of the encapsulated atom $A$ by an incident electron might alter scattering off…

原子物理 · 物理学 2015-11-03 V. K. Dolmatov , M. Ya. Amusia , L. V. Chernysheva

We demonstrate rather interesting manifestations of co-existence of resonance features in characteristics of the photoionization of 3d-electrons in Xe, Cs and Ba endohedral atoms. It is shown that for all of the considered atoms the…

原子物理 · 物理学 2009-11-13 M. Ya. Amusia , A. S. Baltenkov , L. V. Chernysheva

Electron-electron interactions and correlations form the basis of difficulties encountered in the theoretical solution of problems dealing with multi-electron systems. Accurate treatment of the electron-electron problem is likely to unravel…

量子物理 · 物理学 2022-03-24 E. O. Jobunga